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Improving the carbon sequestration capacity (CSC) of an ecosystem by optimizing urban ecological networks is one of the effective ways to achieve the goal of "carbon neutrality" in the world. The contradiction between the irreplaceable ecological function and economic development of Yancheng City is prominent. Therefore, taking Yancheng City as an example, this paper adopted the morphological spatial pattern analysis–minimum cumulative resistance (MSPA-MCR) model to establish the ecological network of Yancheng City in 2020 and combined it with complex network theory to evaluate its ecological base, network quality, and CSC. The results show that the ecological network of Yancheng City has obvious characteristics of coastal cities. There is a significant positive correlation between CSC and the clustering efficiency of ecological sources, and improving the clustering efficiency of vegetation and water ecological nodes is conducive to enhancing the CSC of ecological networks. In terms of functional restoration of ecological networks, four types of 13 ecological stepping stones and 12 ecological corridors have been designed to strengthen the connectivity and balance of the network, and the improvement of network robustness before and after optimization verifies that the optimization scheme is reasonable and effective. This study improved the optimization method of ecological networks in Yancheng City based on enhancing the CSC of ecological nodes, which provided a theoretical framework and practical reference for the realization of global strategic goals of carbon neutrality. [ABSTRACT FROM AUTHOR]