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Carbon dioxide (CO2) is the most important long-lived greenhouse gas and can be retrieved using solar absorption spectra recorded by a ground-based Fourier-transform infrared spectrometer (FTIR). In this study, we investigate the CO2 retrieval strategy using the Network for the Detection of Atmospheric Composition Change–Infrared Working Group (NDACC–IRWG) type spectra between August 2018 and April 2022 (~4 years) at Xianghe, China, aiming to find the optimal observed spectra, retrieval window, and spectroscopy. Two spectral regions, near 2600 and 4800 cm−1, are analyzed. The differences in column-averaged dry-air mole fraction of CO2 (XCO2) derived from spectroscopies (ATM18, ATM20, HITRAN2016, and HITRAN2020) can be up to 1.65 ± 0.95 ppm and 7.96 ± 2.02 ppm for NDACC-type 2600 cm−1 and 4800 cm−1 retrievals, respectively, which is mainly due to the CO2 differences in air-broadened Lorentzian HWHM coefficient (γair) and line intensity (S). HITRAN2020 provides the best fitting, and the retrieved CO2 columns and profiles from both 2600 and 4800 cm−1 are compared to the co-located Total Column Carbon Observing Network (TCCON) measurements and the greenhouse gas reanalysis dataset from the Copernicus Atmosphere Monitoring Service (CAMS). The amplitude of XCO2 seasonal variation derived from the NDACC-type (4800 cm−1) is closer to the TCCON measurements than that from the NDACC-type (2600 cm−1). Moreover, the NDACC-type (2600 cm−1) retrievals are strongly affected by the a priori profile. For tropospheric XCO2, the correlation coefficient between NDACC-type (4800 cm−1) and CAMS model is 0.73, which is higher than that between NDACC-type (2600 cm−1) and CAMS model (R = 0.56). [ABSTRACT FROM AUTHOR]

Nighttime light data can characterize urbanization, economic development, population density, energy consumption and other human activities. Additionally, carbon dioxide (CO2) emissions are closely related to the scope and intensity of human activities. In this study, we assess the utility of nighttime light data as a powerful tool to reflect CO2 emissions from energy consumption, analyze the uncertainty associated with different nighttime light data for modeling CO2 emissions, and provide guidance and a reference for modeling CO2 emissions based on nighttime light data. In this paper, Mainland China was taken as a case study, and nighttime light datasets (the Defense Meteorological Satellite Program's Operational Linescan System (DMSP-OLS) nighttime light data and the Suomi National Polar-Orbiting Partnership Visible Infrared Imaging Radiometer Suite (NPP-VIIRS) nighttime light data) as well as a global gridded CO2 emissions dataset (PKU-CO2) were used to perform simple regressions at provincial, prefectural and 0.1° × 0.1° grid levels, respectively. The analyses are aimed at exploring the accuracy and uncertainty of DMSP-OLS and NPP-VIIRS nighttime light data in modeling CO2 emissions at different spatial scales. The improvement of nighttime light index and the potential factors influencing the effects of modeling CO2 emissions based on nighttime light datasets were also explored. The results show that DMSP-OLS is superior to NPP-VIIRS in modeling CO2 emissions at all spatial scales, and the bigger the scale, the more evident the advantages of DMSP-OLS. When modeling CO2 emissions with nighttime light datasets, not only the total amount of lights within a given statistical unit but also the agglomeration degree of lights should be taken into account. Furthermore, the geographical location and socio-economic conditions at the study site, such as gross regional product per capita (GRP per capita), population, and urbanization were shown to have an impact on the regression effect of the nighttime lights-CO2 emissions model. The regression effect was found to be better at higher latitude and longitude areas with higher GRP per capita and higher urbanization, while population showed little effect on the regression effect of the nighttime lights - CO2 emissions model. The limitation of this study is that the thresholds of potential factors are unclear and the quantitative guidance is insufficient. [ABSTRACT FROM AUTHOR]

The massive increase in the amount of greenhouse gases in the atmosphere, especially carbon dioxide (CO2), has had a significant impact on the global climate. Research has revealed that lakes play an important role in the global carbon cycle and that they can shift between the roles of carbon sources and sinks. This study used Landsat satellite images to analyze the spatiotemporal characteristics and factors influencing the CO2 changes in Chagan Lake in China. We conducted six water sampling campaigns at Chagan Lake in 2020–2021 and determined the partial pressure of carbon dioxide (pCO2) from 110 water samples. Landsat surface reflectance was matched with water sampling events within ±7 days of satellite overpasses, yielding 75 matched pairs. A regression analysis indicated strong associations between pCO2 and both the band difference model of the near-infrared band and green band (Band 5-Band 3, R2 = 0.83, RMSE = 27.55 μatm) and the exponential model [((exp(b3) − exp(b5))2/(exp(b3) + exp(b5))2, R2 = 0.82, RMSE = 27.99 μatm]. A comparison between the performances of a linear regression model and a machine learning model found that the XGBoost model had the highest fitting accuracy (R2 = 0.94, RMSE = 16.86 μatm). We used Landsat/OLI images acquired mainly in 2021 to map pCO2 in Chagan Lake during the ice-free period. The pCO2 in the surface water of Chagan Lake showed considerable spatiotemporal variability within a range of 0–200 μatm. pCO2 also showed significant seasonal variations, with the lowest and highest mean values in autumn (30–50 μatm) and summer (120–150 μatm), respectively. Spatially, the pCO2 values in the southeast of Chagan Lake were higher than those in the northwest. The CO2 fluxes were calculated based on the pCO2 and ranged from −3.69 to −2.42 mmol/m2/d, indicating that Chagan Lake was absorbing CO2 (i.e., it was a weak carbon sink). Temperature, chlorophyll a, total suspended matter, and turbidity were found to have reinforcing effects on the overall trend of pCO2, while the Secchi disk depth was negatively correlated with pCO2. The results of this study provide valuable insights for assessing the role of lakes in the carbon cycle in the context of climate change. [ABSTRACT FROM AUTHOR]

Coal-fired power plants, as major anthropogenic CO2 emission sources, constitute one of the largest contributors to global greenhouse gas emissions. Accurately calculating the dispersion process of CO2 emissions from these point sources is crucial, as it will aid in quantifying CO2 emissions using remote sensing measurements. Employing the Lagrangian Particle Dispersion Theory Model (LPDTM), our study involves modeling CO2 diffusion from point sources. Firstly, we incorporated high-resolution DEM (Digital Elevation Model) and artificial building elements obtained through the Adaptive Deep Learning Location Matching Method, which is involved in CO2 simulation. The accuracy of the results was verified using meteorological stations and aircraft measurements. Additionally, we quantitatively analyzed the influence of terrain and artificial building characteristics on high spatial resolution atmospheric CO2 diffusion simulations, revealing the significance of surface characteristics in dispersion modeling. To validate the accuracy of the LPDTM in high-resolution CO2 diffusion simulation, a comparative experiment was conducted at a power plant in Yangzhou, Jiangsu Province, China. The simulated result was compared with observation from aerial flights, yielding the R2 (Correlation Coefficient) of 0.76, the RMSE (Root Mean Square Error) of 0.267 ppm, and the MAE (Mean Absolute Error) of 0.2315 ppm for the comparison of 73 pixels where the plume intersected with flight trajectories. The findings demonstrate a high level of consistency between the modeled CO2 point source plume morphology and concentration quantification and the actual observed outcomes. This study carried out a quantitative assessment of the influence of surface features on high-resolution atmospheric CO2 point source diffusion simulations, resulting in an enhanced accuracy of the simulated CO2 concentration field. It offers essential technological and theoretical foundations for the accurate quantification of anthropogenic CO2 emissions using top-down approaches. [ABSTRACT FROM AUTHOR]

Humans have altered the earth in unprecedented ways, and these changes have profound implications for global climate change. However, the impacts of human pressures on carbon dioxide (CO2) emissions over long time scales have not yet been clarified. Here, we used the human footprint index (HF), which estimates the ecological footprint of humans in a given location, to explore the impacts of human pressures on CO2 emissions in China from 2000 to 2017. Human pressures (+13.6%) and CO2 emissions (+198.3%) in China are still on the rise during 2000–2017 and are unevenly distributed spatially. There was a significant positive correlation between human pressures and CO2 emissions in China, and northern China is the main driver of this correlation. The increase of CO2 emissions in China slowed down after 2011. Although human pressures on the environment are increasing, high-quality development measures have already had noticeable effects on CO2 emission reductions. [ABSTRACT FROM AUTHOR]

As one of the most influential greenhouse gases, carbon dioxide (CO2) has a profound impact on the global climate. The spaceborne integrated path differential absorption (IPDA) lidar will be a great sensor to obtain the columnar concentration of CO2 with high precision. This paper analyzes the performance of a spaceborne IPDA lidar, which is part of the Aerosol and Carbon Detection Lidar (ACDL) developed in China. The line-by-bine radiative transfer model was used to calculate the absorption spectra of CO2 and H2O. The laser transmission process was simulated and analyzed. The sources of random and systematic errors of IPDA lidar were quantitatively analyzed. The total systematic errors are 0.589 ppm. Monthly mean global distribution of relative random errors (RREs) was mapped based on the dataset in September 2016. Afterwards, the seasonal variations of the global distribution of RREs were studied. The global distribution of pseudo satellite measurements for a 16-day orbit repeat cycle showed relatively uniform distribution over the land of the northern hemisphere. The results demonstrated that 61.24% of the global RREs were smaller than 0.25%, or about 1 ppm, while 2.76% of the results were larger than 0.75%. The statistics reveal the future performance of the spaceborne IPDA lidar. [ABSTRACT FROM AUTHOR]

Atmospheric carbon dioxide (CO2) is recognized as the most important component of the greenhouse gases, the concentration of which has increased rapidly since the pre-industrial era due to anthropogenic emissions of greenhouse gases (GHG). The accurate monitoring of carbon dioxide is essential to study the global carbon cycle and radiation budget on Earth. The Aerosol and Carbon Detection Lidar (ACDL) instrument onboard the Atmospheric Environmental Monitoring Satellite (AEMS) was successfully launched in April 2022, which allows a new perspective to quantify the global spatial distribution of atmospheric CO2 with high accuracy. In this work, the impact of the Doppler shift on CO2 measurements for an integrated-path differential absorption (IPDA) light detection and ranging (lidar) system was evaluated to meet the weighted column-averaged mixing ratio of carbon dioxide (XCO2) measurement requirements of less than one part per million (ppm). The measurement uncertainties due to the Doppler shift were first evaluated in airborne IPDA observations. The result shows that most of the Doppler shift is in the range of 6–8 MHz, resulting in 0.26-0.39 ppm deviations in the XCO2 results. The deviations between the XCO2 retrievals and in situ measurements decreased to 0.16 ppm after the correction of the Doppler shift from 11:28:29 to 11:28:49 in the flight campaign. In addition, the online Doppler shift accounts for 98% of the deviations between XCO2 retrievals and in situ measurements. Furthermore, the impact of the Doppler shift on ACDL measurements is also assessed. The differences between the XCO2 retrievals with and without Doppler shift are used to quantify measurement uncertainties due to the Doppler effect. The simulations reveal that a pointing misalignment of 0.067 mrad can lead to a mean bias of about 0.30 ppm (0.072%) in the CO2 column. In addition, CO2 measurements are more sensitive to the Doppler shift at high altitudes for IPDA lidar, so the largest differences in the CO2 columns are found on the Qinghai–Tibet Plateau in China. [ABSTRACT FROM AUTHOR]

In view of global warming, caused by the increase in the concentration of greenhouse gases, China has proposed a series of carbon emission reduction policies. It is necessary to obtain the spatiotemporal distribution of carbon emissions accurately. Nighttime light data is recognized as an important basis for carbon emission estimation. A large number of research results show that there is a positive correlation between nighttime light intensity and carbon emission. However, in the current context of China's industrial reforms, this positive relationship may not be entirely correct. First, we correct the nighttime light data from different satellites and established a long-term series data set. Then, we verify the positive correlation between nighttime light and carbon emission. However, the time scale of emission data often lags, and the carbon concentration data are released earlier and are more accurate than emission data. Therefore, we propose to investigate the relationship between nighttime light and carbon concentration. It is found that there may be different correlations between nighttime light and the carbon concentration, due to different urban industrial structure and development planning. Therefore, by exploring the relationship between nighttime light and the carbon concentration, the existing carbon emission estimation model can be modified to improve the accuracy of the emission model. [ABSTRACT FROM AUTHOR]

Vegetation regulates the exchange of terrestrial carbon and water fluxes and connects the biosphere, hydrosphere, and atmosphere. Over the last four decades, vegetation greening has been observed worldwide using satellite technology. China has also experienced a notably widespread greening trend. However, the responsiveness of vegetation dynamics to elevated CO2 concentration, climate change, and human activities remains unclear. In this study, we attempted to explore the impact of natural (precipitation, air temperature), biogeochemical (CO2), and anthropogenic drivers (nighttime light, afforestation area) on changes in vegetation greenness in the Haihe River Basin (HRB) during 2002–2018 at the county-level. We further determined the major factors affecting the variation in satellite-derived normalized difference vegetation index (NDVI) from moderate resolution imaging spectroradiometer (MODIS) for each county. The results indicated that over 85% of the counties had a significantly increased NDVI trend, and the average linear trend of annual NDVI across the study region was 0.0037 per year. The largest contributor to the NDVI trend was CO2 (mean contribution 45%), followed by human activities (mean contribution of 27%). Additionally, afforestation was a pronounced driving force for NDVI changes in mountainous areas, resulting from ecosystem restoration efforts. Our findings emphasize the crucial role of CO2 fertilization in vegetation cover change, while considering CO2 concentration, climate change, and human activities, and shed light on the significant influences of afforestation programs on water resources, especially in mountainous areas. [ABSTRACT FROM AUTHOR]

The spaceborne double-pulse integrated-path differential absorption (IPDA) light detection and ranging (LIDAR) system was found to be helpful in observing atmospheric CO2 and understanding the carbon cycle. The airborne experiments of a scale prototype of China's planned spaceborne IPDA LIDAR was implemented in 2019. A problem with data inversion caused by the detector module nonlinearity was found. Through many experiments, the amplifier circuit board (ACB) of the detector module was proved to be the main factor causing the nonlinearity. Through amplifier circuit optimization, the original bandwidth of the ACB was changed to 1 MHz by using a fifth-order active filter. Compared with the original version, the linearity of optimized ACB is improved from 42.6% to 0.0747%. The optimized ACB was produced and its linearity was verified by experiments. In addition, the output waveform of the optimized ACB changes significantly, which will affect the random error (RE) of the optimized IPDA LIDAR system. Through the performance simulation, the RE of more than 90% of the global area is less than 0.728 ppm. Finally, the transfer model of the detector module was given, which will be helpful for the further optimization of the CO2 column-averaged dry-air mixing ratio (XCO2) inversion algorithm. [ABSTRACT FROM AUTHOR]