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The goal of the work is to determine unknown parameters of reactor heating in the process of biomass solar pyrolysis. The lab-scale reactor is heated by a xenon lamp, but the fraction of heat absorbed by the reactor is unknown, as well as the heat transfer coefficient from the reactor walls to the nitrogen flowing through internal reactor channels, and the overall heat transfer coefficient through the external reactor walls to the surroundings. The missing parameters are impossible to measure, therefore they need to be determined by solving the inverse problem. As the problem is strongly ill-conditioned, since the quantities are directly dependent on each other, two different inverse algorithms were used to retrieve them, namely, the Levenberg-Marquardt method and the Metropolis-Hastings method. The effectiveness of both approaches was assessed and then they were applied to the real data. The inverse problem was implemented in the MatLab software, while validation of the mathematical model and optimisation procedure was carried out with a CFD model built in Ansys Fluent 19.2. Calculations showed that 14.4% of the lamp power penetrates inside the reactor and heat transfer coefficients to the flowing nitrogen equal 8.74 W/m2K and 0.965 W/m2K to the surroundings. • Two inverse algorithms were used: Levenberg-Marquardt and Metropolis-Hastings. • The validation was carried out with a 3D CFD model. • Calculations showed that only 14.4% of the lamp power penetrates inside the reactor. [ABSTRACT FROM AUTHOR]

The article presents a review of works on mathematical modelling of biomass pyrolysis process. Models types, number of dimensions, captured phenomena, type and dimensions of the reactors and biomass particles as well as models validation methods were analysed. Particular attention was paid to descriptions of chemical reactions, which are the essence of biomass thermal decomposition simulation. The article briefly describes the most important issues related to biomass pyrolysis and provides a review of commonly used methods of modelling this process with emphasis on solutions "ready to employ" in CFD modelling. A summary of other review papers on this topic is also provided. The problem of mathematical modelling in the context of "model - an engineering tool" was also discussed. Mathematical model for an engineering applications must be prepared with consideration of necessary consensus between the calculations accuracy, calculation time, preparation efforts and analysis requirements. Therefore, in pyrolysis modelling context, the inclusion of chemical reactions and changes of heat transport conditions were considered as priority, while taking into account moisture evaporation and bed shrinkage should be conditioned by their actual contribution in the calculations accuracy and by their influence on the calculations time. • A review of research on mathematical modelling of biomass pyrolysis is presented. • Captured phenomena, kinetic models, properties change, reactor types are summarized. • Compromise between model precision and calculations costs is discussed. [ABSTRACT FROM AUTHOR]