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In this study we assume that a gravitational curvature tensor, i.e. a tensor of third-order directional derivatives of the Earth's gravitational potential, is observable at satellite altitudes. Such a tensor is composed of ten different components, i.e. gravitational curvatures, which may be combined into vertical-vertical-vertical, vertical-vertical-horizontal, vertical-horizontal-horizontal and horizontal-horizontal-horizontal gravitational curvatures. Firstly, we study spectral properties of the gravitational curvatures. Secondly, we derive new quadrature formulas for the spherical harmonic analysis of the four gravitational curvatures and provide their corresponding analytical error models. Thirdly, requirements for an instrument that would eventually observe gravitational curvatures by differential accelerometry are investigated. The results reveal that measuring third-order directional derivatives of the gravitational potential imposes very high requirements on the accuracy of deployed accelerometers which are beyond the limits of currently available sensors. For example, for orbital parameters and performance similar to those of the GOCE mission, observing third-order directional derivatives requires accelerometers with the noise level of $${\sim}10^{-17}\,\hbox {m}\,\hbox {s}^{-2}$$ Hz $$^{-1/2}$$ . [ABSTRACT FROM AUTHOR]