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In view of the climate emergency, it is necessary to model and forecast road transport emissions for implementing more effective climate policy. This paper fills an important research gap by quantifying the challenges, barriers and remedies of achieving road transport emission reduction and air quality improvement in developing countries. It contributes to the debate on top-down and bottom-up approaches to reconcile carbon and other transport related emissions. China and India are chosen as case studies. Using various official statistics and proxy variables, we estimate and compare the road transport carbon emissions of the two countries systematically from 2009 to 2020. Insights from detailed mode-specific estimations of the bottom-up approach are valuable for targeted policies and measures. An analysis of the major components of road transport carbon emissions points to strategies of promoting electric vehicles, reducing transport demand, accelerating modal shift to low-carbon modes, and cleaner electricity to achieve climate policy. [ABSTRACT FROM AUTHOR]