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Two kinds of cellulose/ZnO piezoelectric papers are prepared by crushing and dissolving methods. The papers are characterized by SEM and analyzed by a piezoelectric equipment. The differences in the structure and piezoelectric performance of the two kinds of papers are explored. The effects of ZnO add-on amount, thickness of the papers, and pressure on the piezoelectric properties are discussed and compared with a PVDF film. The mutts show that the fibers of the piezoelectric paper prepared by the dissolving method are smooth and tightly bounded to ZnO, which makes ZnO uniformly coat on the surface of the fibers. The higher the pressure, the higher the piezoelectric properties. The thicker the piezoelectric paper, the higher the piezoelectric properties. The piezoelectric paper with 20% ZnO added by the dissolving method has high piezoelectric properties, and the maximum output current is 52.36 nA/cm². The piezoelectric properties of the piezoelectric paper are comparable to the purchased PVDF film. [ABSTRACT FROM AUTHOR]