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Abstract: Every year during the winter and pre-monsoon periods most of the Indian peninsula, Bay of Bengal and the adjoining Indian Ocean are affected by a polluted regional haze, known as the South Asian Winter Haze (SAWH). This article is the first of a series of three papers collectively anticipated at the central idea of retrieving aerosol component type and effective radius of the SAWH by incorporating experimental data of ground-based solar radiometer into Mie theory, and validation by collocated in-situ measurements. The work presented in this paper provides an approach to retrieve optical depths and their spectral curvature for SAWH at a tropical coastal station, Visakhapatnam (17.7°N, 83.3°E). A dataset comprised of 92 wintertime atmospheric optical depths are obtained from spectral extinction measurements of direct solar flux by means of a Multi-Wavelength Solar Radiometer during the period of October 2002 to February 2004. The inter-channel correlations established a linear relation and the airmass conditions specific to this dataset suggested a two-component linear model; the stable and variable components of which are analysed to obtain the mentioned optical parameters. Results indicate that the spectral curvature is best represented by a Lorentz model with a central wavelength of 0.40425±0.02945μm, a width of 0.40382±0.10253μm, a constant of 0.92623±0.33793, and a wavelength independent component of 0.95778±0.15678. Resonance-like structure of the obtained spectral curvature resembles wavelength dependent extinction characteristic of absorbing soot particles; thereby supports the key findings from INDOEX campaign. [Copyright &y& Elsevier]

Abstract: The significant role of aerosol–cloud interaction during the large-scale drought producing breaks of 2009 Indian Summer Monsoon is investigated in the present paper. This mega drought had already been attributed to two long breaks, one in June and the other in July-August. While Central India (CI) and northern parts of the country experienced deficient rainfall, the rainfall over the southern Peninsular India (PI) remained close to normal. During the first break in June, which was associated with mid-latitude intrusion of dry air, the Twomey effect (positive aerosol indirect effect – AIE) was a dominant factor inhibiting efficient precipitation over CI region, as compared to that over PI. Moreover, the number of days that experienced significant (at 5% level of significance) positive AIE during the first break was more over CI compared to the same during the second break. The AIE on ice clouds was not as significant as that of the low-clouds. The resulting cloud properties during both break and active phases over CI differ significantly from that over PI for the corresponding periods. The positive AIE mentioned here is attributed to the large-scale deficit of moisture supply to the CI region due to dynamical reasons. However, it is shown that under ample availability of moisture, more aerosols could invigorate deep clouds over specific regions even during the break spells. [Copyright &y& Elsevier]

Abstract: Aerosol measurements over a tropical semi-arid site in Anantapur (14.62°N, 77.65°E, 331 m asl), India, provide the variabilities of aerosol characteristics for the period of January 2007–December 2008. The mean values of aerosol optical depth at 500 nm (AOD500 nm) over 2-year period are found to be 0.37 ± 0.11, 0.39 ± 0.13 and 0.30 ± 0.10 during winter, summer and monsoon seasons, respectively. A rather systematic variation is seen with AOD peaking in the month of March, falling off gradually to the lowest value in June and increasing slowly superposed with some modulations, which show a weak secondary peak in October. The mean and standard values of the Ångström exponent, α (turbidity coefficient, β), are found to be 1.06 ± 0.33 (0.17 ± 0.05) during winter, 0.97 ± 0.35 (0.22 ± 0.04) during summer and 0.85 ± 0.26 (0.16 ± 0.06) during monsoon. The frequency distribution of α is relatively broad with two modes for dusty (α < 1) and non-dusty (α > 1) situations. This frequency distribution of α reveals a great dispersion of a values in all seasons thus denoting variability in the aerosol-size distribution. In this study, spectral AOD and Ångström exponent data are analyzed to obtain information about the adequacy of the simple use of the Ångström exponent and its variation for characterizing optical properties of aerosols, and exploring possibilities for a more efficient characterization of them. Using the least-squares fit method, the Ångström parameter, α, is calculated in the spectral interval 380–850 nm, along with coefficients a1 and a2 of the second-order polynomial fit to the plotted logarithm of AOD versus the logarithm of wavelength. The correlations between the coefficients a1 and a2 with months and α are discussed in the paper. [Copyright &y& Elsevier]

The Indian summer monsoon (ISM) is largely influenced by intra-seasonal variability like break and active phases of monsoon. In the present study, different cloud and aerosol parameters are considered and analyzed to formulate a cloud-aerosol coupled index (CACI) that can aid in forecasting the break phase of ISM. The method of principal component analysis is implemented to identify the significant cloud and aerosol parameters during break and active phases of ISM. The threshold ranges of each parameter are evaluated by using the normal probability density function. The result reveals that for break phase, the significant parameters are cloud water path (CWP), cloud optical depth, aerosol index, zonal wind (ZW), and meridional wind (MW) at 850 hPa pressure level whereas for active phase, the parameters found to be important are aerosol optical depth, CWP, ZW, and MW at 850 hPa pressure level. The significantly correlated ( p < 0.05) parameters are taken for formulating CACI. The results show that no such significant correlation is possible with the parameters during active phase of ISM. The CACI is thus formulated to forecast the break phase of ISM. The result shows that the CACI is capable of forecasting the break phase of Indian summer monsoon over central India with 88 % certainty and 10 days lead time. The result is validated with the observations. [ABSTRACT FROM AUTHOR]

Atmospheric aerosol (PM10) measurements were made at a regional representative semi-arid urban site, Tirupati, India over one-year period i.e. from October, 2001 to September, 2002. The samples were collected on polyflex filters, and analyzed for the major water-soluble ions – F, Cl, NO3, SO4, Na, NH4, K, Ca and Mg, employing ion chromatograph. The average mass of PM10 is found to be 32.75 μg/m3 with a total water-soluble aerosol load (total anion + total cation) of 13.56 μg/m3. Composition of aerosol showed higher concentration of SO4 followed by Na, Ca and NO3. Very good correlation is observed between crustal ions Ca and Mg ( r=0.82) as well as between crustal and acidic ions; Ca and SO4 ( r=0.75) and NO3 ( r=0.67) and Mg and NO3 ( r=0.78) and SO4 ( r=0.73), suggest that the ionic composition was influenced by local terrestrial sources. The presence of SO4 and NO3 may be due to re-suspension of soil particles (formation by heterogeneous oxidation). Ca, Mg and Na are mainly soil derived ones. Correlation matrix with meteorological factors, as well as seasonal distribution of PM10 and its ionic components present a clear trend of higher concentrations during summer due to greater particle release and lowering atmospheric levels during the rainy season due to washout effect. ANOVA results showed the significant variation of composition from season to season. Paired comparisons (DMRT) revealed the occurrence of significant difference in pairs of mean concentration from season to season except within monsoon i.e. between S-W and N-E monsoon. [ABSTRACT FROM AUTHOR]