1. Superstrong, sustainable, origami wood paper enabled by dual-phase nanostructure regulation in cell walls.
- Author
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Jianfu Tang, Lianping Wu, Xueqin Fan, Xiaofei Dong, Xueqi Li, Yanjun Xie, Jian Li, Jiancun Rao, Teng Li, and Wentao Gan
- Abstract
Constructing a crystalline-amorphous hybrid structure is an effective strategy to overcome the conflict between the strength and toughness of materials. However, achieving such a material structure often involves complex, energy-intensive processing. Here, we leverage the natural wood featuring coexisting crystalline and amorphous regions to achieve superstrong and ultratough wood paper (W-paper) via a dual-phase nanostructure regulation strategy. After partially removing amorphous hemicellulose and eliminating most lignin, the treated wood can self-densify through an energy-efficient air drying, resulting in a W-paper with high tensile strength, toughness, and folding endurance. Coarse-grained molecular dynamics simulations reveal the underlying deformation mechanism of the crystalline and amorphous regions inside cell walls and the failure mechanism of the W-paper under tension. Life cycle assessment reveals that W-paper shows a lower environmental impact than commercial paper and common plastics. This dual-phase nanostructure regulation based on natural wood may provide valuable insights for developing high-performance and sustainable film materials. [ABSTRACT FROM AUTHOR]
- Published
- 2024
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