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1. Palladacycle-CatalyzedAsymmetric Intermolecular Constructionof Chiral Tertiary P-Heterocycles by Stepwise Addition of H–P–HBonds to Bis(enones).

Author

Huang, Yinhua, Pullarkat, Sumod A., Teong, Siewping, Chew, Renta Jonathan, Li, Yongxin, and Leung, Pak-Hing

Subjects
*PALLADIUM catalysts, *PALLADACYCLES, *ASYMMETRY (Chemistry), *HETEROCYCLIC compounds, *CHIRALITY, *ADDITION reactions, *CARBONYL compounds, *CHEMICAL bonds
Abstract

A palladacycle-catalyzed diastereo- and enantioselectivestepwisedouble hydrophosphination of bis(enones) with PhPH2hasbeen developed, allowing intermolecular construction of chiral tertiarybulky P-heterocycles in one pot in high yields. A catalytic cyclefor the reaction is proposed as well. [ABSTRACT FROM AUTHOR]

Published
2012
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