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The resonant nature and geometric scalability make metamaterials an ideal platform for an enhanced light–matter interaction over a broad frequency range. The mid-infrared (IR) spectral range is of great importance for vibrational spectroscopy of molecules, while IR metamaterials created from lithography-based planar nanostructures have been used to demonstrate enhanced molecular detection. Compared with visible and near-infrared, the relative long wavelengths of IR light make it possible to achieve three-dimensional (3D) IR metamaterials via the state-of-the-art 3D fabrication techniques. Here, we design and fabricate a 3D printed plasmonic metamaterial absorber (MMA), and by performing Fourier-transform IR spectroscopy, we demonstrate that a series of molecular fingerprint vibrations of glycine can be significantly enhanced by the high absorption mode supported by the 3D meta-atoms of the MMA. The observed enhanced IR detection can also be partially attributed to the improved accessibility offered by the 3D architecture of the MMA. In particular, due to capillary forces during the drying process, the microscale 3D printed features lead to selective analyte deposition in high-field regions, which provides another degree of freedom in the design of the 3D printed structures for surface-enhanced IR detection. Our study shows the flexibility of metastructures based on advanced 3D printing technology in tailoring the interaction between IR light and materials on a subwavelength scale. [ABSTRACT FROM AUTHOR]

The resonance based strong light-matter interaction in metamaterials offers unprecedented opportunities to manipulate polarization of electromagnetic waves. In this work, we fabricate a three-dimensional (3D) metamaterial consisting of 90°-twisted split-tube resonators using a 3D printing technique and demonstrate the corresponding asymmetric transmission for linearly polarized electromagnetic waves in the Ku band with near-unity polarization conversion efficiency. Experimental results reveal a 90° polarization rotation and an incident polarization angle dependent asymmetric transmission at a frequency around 15.2 GHz. The experimental results are in good agreement with simulations. Possessing the merits of both flexibility of response tailoring and ease of fabrication, the proposed 3D-printed metamaterials have great potential for compact polarization-control devices exhibiting unidirectional transmission at both microwave and terahertz frequencies. [ABSTRACT FROM AUTHOR]

A tunable isotropic negative effective permeability is experimentally demonstrated in a three-dimensional (3D) dielectric composite consisting of dielectric ceramic cube arrays by temperature changing. It shows that a strong subwavelength magnetic resonance can be excited in dielectric cubes corresponding to the first Mie resonance mode and can be continuously and reversibly adjusted from 13.65 to 19.28 GHz with the temperature changing from -15 to 35 °C. Accordingly, negative permeability can be performed in the frequency range of about 6 GHz by adjusting the temperature. It provides a convenient route to design adaptive metamaterials and 3D invisible cloak. [ABSTRACT FROM AUTHOR]

An electrically tunable negative permeability metamaterial consisting of a periodic array of split ring resonators infiltrated with nematic liquid crystals is demonstrated. It shows that the transmitted resonance dip of the metamaterial can be continuously and reversibly adjusted by an applied electric field, and the maximum shift is about 210 MHz with respect to the resonance frequency around 11.08 GHz. Numerical simulation shows that the permeability is negative near the resonance frequency, and the frequency range with negative permeability can be dynamically adjusted and widened by about 200 MHz by the electric field. It provides a convenient means to design adaptive metamaterials. [ABSTRACT FROM AUTHOR]