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The average Total Kinetic Energy (TKE ) release and fission-fragment yields in neutron-induced fission of 235 U and 238 U was measured using a Frisch-gridded ionization chamber. These observables are important nuclear data quantites that are relevant to applications and for informing the next generation of fission models. The measurements were performed a the Los Alamos Neutron Science Center and cover E n = 200 keV – 30 MeV. The double-energy (2E) method was used to determine the fission-fragment yields and two methods of correcting for prompt-neutron emission were explored. The results of this study are correlated mass and TKE data.

Background: Neutron-rich, even-mass chromium and iron isotopes approaching neutron number $N=40$ have been important benchmarks in the development of shell-model effective interactions incorporating the effects of shell evolution in the exotic regime. Odd-mass manganese nuclei have received less attention, but provide important and complementary sensitivity to these interactions.Purpose: We report the observation of two new $\ensuremath{\gamma}$-ray transitions in $^{63}\mathrm{Mn}$, which establish the $(9/{2}^{\ensuremath{-}})$ and $(11/{2}^{\ensuremath{-}})$ levels on top of the previously known $(7/{2}^{\ensuremath{-}})$ first-excited state. The lifetime for the $(7/{2}^{\ensuremath{-}})$ and $(9/{2}^{\ensuremath{-}})$ excited states were determined for the first time, while an upper limit could be established for the $(11/{2}^{\ensuremath{-}})$ level.Method: Excited states in $^{63}\mathrm{Mn}$ have been populated in inelastic scattering from a $^{9}\mathrm{Be}$ target and in the fragmentation of $^{65}\mathrm{Fe}$. $\ensuremath{\gamma}\ensuremath{\gamma}$ coincidence relationships were used to establish the decay level scheme. A Doppler line-shape analysis for the Doppler-broadened $(7/{2}^{\ensuremath{-}})\ensuremath{\rightarrow}5/{2}^{\ensuremath{-}}$, $(9/{2}^{\ensuremath{-}})\ensuremath{\rightarrow}(7/{2}^{\ensuremath{-}}),$ and $(11/{2}^{\ensuremath{-}})\ensuremath{\rightarrow}(9/{2}^{\ensuremath{-}})$ transitions was used to determine (limits for) the corresponding excited-state lifetimes.Results: The low-lying level scheme and the excited-state lifetimes were compared with large-scale shell-model calculations using different model spaces and effective interactions in order to isolate important aspects of shell evolution in this region of structural change.Conclusions: While the theoretical $(7/{2}^{\ensuremath{-}})$ and $(9/{2}^{\ensuremath{-}})$ excitation energies show little dependence on the model space, the calculated lifetime of the $(7/{2}^{\ensuremath{-}})$ level and calculated energy of the $(11/{2}^{\ensuremath{-}})$ level reveal the importance of including the neutron ${g}_{9/2}$ and ${d}_{5/2}$ orbitals in the model space. The LNPS effective shell-model interaction provides the best overall agreement with the new data.

The 9Be(28Mg,27Na) one-proton removal reaction with a large proton separation energy of Sp(28Mg)=16.79 MeV is studied at intermediate beam energy. Coincidences of the bound 27Na residues with protons and other light charged particles are measured. These data are analyzed to determine the percentage contributions to the proton removal cross section from the elastic and inelastic nucleon removal mechanisms. These deduced contributions are compared with the eikonal reaction model predictions and with the previously measured data for reactions involving the re- moval of more weakly-bound protons from lighter nuclei. The role of transitions of the proton between different bound single-particle configurations upon the elastic breakup cross section is also quantified in this well-bound case. The measured and calculated elastic breakup fractions are found to be in good agreement., Comment: Phys. Rev. C 2014 (accepted)

The study of fission fragment yields and how they behave as a function of excitation energy provides insight into the process in which they are formed. Fission yields are also important for nuclear applications, as they can be used as a diagnostic tool. A new instrument, SPIDER (Spectrometer for Ion DEtermination in fission Research), is being developed for measuring fission yields as a function of incident neutron energy at the Los Alamos Neutron Science Center. The instrument employs a time-of-flight mass spectrometry method in which the velocity and kinetic energy of the fragments are measured in order to determine their mass. Additionally, by using Bragg peak spectroscopy, the charge of the fragments can be identified. A prototype instrument has been developed and preliminary results indicate that ∼ 1 mass unit resolution is feasible using this approach. A larger detector array is currently being designed, and will be used at study fission yields from thermal neutron energies up to at least 20 MeV.