Search

Neutrinoless double beta ($0\nu\beta\beta$) decay is a hypothetical rare nuclear transition ($T_{1/2}>10^{26}$ y). Its observation would provide an important insight about the nature of neutrinos (Dirac or Majorana particle) demonstrating that the lepton number is not conserved. This decay can be investigated with bolometers embedding the double beta decay isotope ($^{76}$Ge, $^{82}$Se, $^{100}$Mo, $^{116}$Cd, $^{130}$Te...), which perform as low temperature calorimeters (10 mK) detecting particle interactions via a small temperature rise read out by a dedicated thermometer. CROSS (Cryogenic Rare-event Observatory with Surface Sensitivity) aims at the development of bolometric detectors (Li$_{2}$MoO$_{4}$ and TeO$_{2}$) capable of discriminating surface $\alpha$ and $\beta$ interactions by exploiting superconducting properties of Al film deposited on the crystal surface. We report in this paper the results of tests on prototypes performed at CSNSM (Orsay, France) that showed the capability of a-few-$\mu$m-thick superconducting Al film deposited on crystal surface to discriminate surface $\alpha$ from bulk events, thus providing the detector with the required surface sensitivity capability. The CROSS technology would further improve the background suppression and simplify the detector construction with a view to future competitive double beta decay searches., Comment: Accepted for publication in J. Low Temp. Phys

The double-electron capture and the electron capture with positron emission in 168Yb have been investigated for the first time at the STELLA facility of the Gran Sasso underground laboratory (Italy) measuring 371 g of highly purified ytterbium oxide placed on the end-cap of a 465 cm3 ultra-low-background high purity Germanium detector (HPGe). No gamma associated to double beta processes in 168Yb have been observed after 2074 h of data taking. This has allowed setting the half-life limits on the level of lim ⁡ T 1 / 2 ∼ 10 14 – 10 18 yr at 90% C.L. Particularly, a lower half-life limit on a possible resonant neutrinoless double-electron capture in 168Yb to the ( 2 ) − 1403.7 keV excited state of 168Er is set as T 1 / 2 ≥ 1.9 × 10 18 yr at 90% C.L. Half-life limits T 1 / 2 2 ν ( 0 ν ) ≥ 4.5 ( 4.3 ) × 10 16 yr were set on the 2 ν ( 0 ν ) 2 β − decay of 176Yb to the 2 + 84.3 keV first excited level of 176Hf.

The development of low-threshold detectors for the study of coherent elastic neutrino-nucleus scattering and for the search for light dark matter necessitates methods of low-energy calibration. We suggest this can be provided by the nuclear recoils resulting from the $\gamma$ emission following thermal neutron capture. In particular, several MeV-scale single-$\gamma$ transitions induce well-defined nuclear recoil peaks in the 100 eV range. Using the FIFRELIN code, complete schemes of $\gamma$-cascades for various isotopes can be predicted with high accuracy to determine the continuous background of nuclear recoils below the calibration peaks. We present a comprehensive experimental concept for the calibration of CaWO$_4$ and Ge cryogenic detectors at a research reactor. For CaWO$_4$ the simulations show that two nuclear recoil peaks at 112.5 eV and 160.3 eV should be visible above background simply in the spectrum of the cryogenic detector. Then we discuss how the additional tagging for the associated $\gamma$ increases the sensitivity of the method and extends its application to a wider energy range and to Ge cryogenic detectors., Comment: 21 pages, 8 figures

Lithium magnesium molybdate (Li 2 Mg 2 (MoO 4 ) 3 ) crystals were grown by the low-thermal-gradient Czochralski method . Luminescence properties of the material (emission spectra, thermally stimulated luminescence, dependence of intensity on temperature, phosphorescence) have been studied under X-ray excitation in the temperature interval from 8 to 400 K, while at the same being operated as a scintillating bolometer at 20 mK for the first time. We demonstrated that Li 2 Mg 2 (MoO 4 ) 3 crystals are a potentially promising detector material to search for neutrinoless double beta decay of 100Mo.

The first direct search for the double electron capture ($2\epsilon$) and the electron capture with positron emission ($\epsilon\beta^+$) in $^{144}$Sm to the ground state and to the excited levels of $^{144}$Nd was realized by measuring - over 1899 h - a 342 g sample of highly purified samarium oxide (Sm$_2$O$_3$) with the ultra-low background HP-Ge $\gamma$ spectrometer GeCris (465 cm$^3$) at the STELLA facility of the Gran Sasso National Laboratory (LNGS). No effect was observed and half-life limits were estimated at the level of $T_{1/2} \sim (0.1-1.3) \times 10^{20}$ yr (90% C.L.). Moreover, for the first time half-life limits of the double beta ($2\beta^-$) decay of $^{154}$Sm to several excited levels of $^{154}$Gd have been set; they are at the level of $T_{1/2} \sim (0.06-8) \times 10^{20}$ yr (90% C.L.)., Comment: 20 pages, 7 figures and 4 tables

The first observation of coherent elastic neutrino-nucleus scattering (CE ν NS), reported by the COHERENT Collaboration in 2017, paved the way for a new generation of experiments using reactor ν e and aiming at precisely measuring this process. In this context, the BASKET (Bolometers At Sub-KeV Energy Thresholds) R&D project investigates the use of cryogenic detectors for a reactor CE ν NS experiment. This article reports on the first test of a Mo-doped lithium tungstate scintillating bolometer ( ⊘ 18 × 7 mm, 8 g), performed in an aboveground laboratory at CSNSM, Orsay (France). The detector bolometric performance (energy and time response, particle identification capabilities) and radiopurity have been studied and confirm the promising potential of lithium tungstate-based bolometric detectors for the measurement of CE ν NS at reactors.

International audience; We present a measurement of the cosmogenic activation in the germanium cryogenic detectors of the EDELWEISS III direct dark matter search experiment. The decay rates measured in detectors with different exposures to cosmic rays above ground are converted into production rates of different isotopes. The measured production rates in units of nuclei/kg/day are 82 $\pm$ 21 for $^3$H, 2.8 $\pm$ 0.6 for $^{49}$V, 4.6 $\pm$ 0.7 for $^{55}$Fe, and 106 $\pm$ 13 for $^{65}$Zn. These results are the most accurate for these isotopes. A lower limit on the production rate of $^{68}$Ge of 74 nuclei/kg/day is also presented. They are compared to model predictions present in literature and to estimates calculated with the ACTIVIA code.

Search for double $\beta$ decay of $^{136}$Ce and $^{138}$Ce was realized with 732 g of deeply purified cerium oxide sample measured over 1900 h with the help of an ultra-low background HPGe $\gamma$ detector with a volume of 465 cm$^3$ at the STELLA facility of the Gran Sasso National Laboratories of the INFN (Italy). New improved half-life limits on double beta processes in the cerium isotopes were set at the level of $\lim T_{1/2}\sim 10^{17}-10^{18}$~yr; many of them are even two orders of magnitude larger than the best previous results., Comment: 21 pages, 6 figures, 3 tables; version accepted for publication on Nucl. Phys. A

A large cylindrical cadmium molybdate crystal with natural isotopic abundance has been used to fabricate a scintillating bolometer. The measurement was performed above ground at milli-Kelvin temperature, with simultaneous readout of the heat and the scintillation light. The energy resolution as FWHM has achieved from 5 keV (at 238 keV) to 13 keV (at 2615 keV). We present the results of the α versus β / γ events discrimination. The low internal trace contamination of the CdMoO 4 crystal was evaluated as well. The detector performance with preliminary positive indications proves that cadmium molybdate crystal is a promising absorber for neutrinoless double beta decay scintillating bolometric experiments with 116 Cd and 100 Mo nuclides in the next-generation technique.

The EDELWEISS-III direct dark matter search experiment uses cryogenic HP-Ge detectors Fully covered with Inter-Digitized electrodes (FID). They are operated at low fields ($, 17 pages 12 figures, submitted to JINST, author list updated

The radioactive contamination of ZnWO4 crystal scintillators has been measured deep underground at the Gran Sasso National Laboratory (LNGS) of the INFN in Italy with a total exposure 3197 kg x h. Monte Carlo simulation, time-amplitude and pulse-shape analyses of the data have been applied to estimate the radioactive contamination of the ZnWO4 samples. One of the ZnWO4 crystals has also been tested by ultra-low background gamma spectrometry. The radioactive contaminations of the ZnWO4 samples do not exceed 0.002 -- 0.8 mBq/kg (depending on the radionuclide), the total alpha activity is in the range: 0.2 - 2 mBq/kg. Particular radioactivity, beta active 65Zn and alpha active 180W, has been detected. The effect of the re-crystallization on the radiopurity of the ZnWO4 crystal has been studied. The radioactive contamination of samples of the ceramic details of the set-ups used in the crystals growth has been checked by low background gamma spectrometry. A project scheme on further improvement of the radiopurity level of the ZnWO4 crystal scintillators is briefly addressed., Comment: 15 pages, 8 figures, 6 tables, submitted for publication

A sample of 100MoO3 powder with molybdenum enriched in 100Mo to 99.5% and mass of 1199 g was measured for 18120 h in a low-background set-up with 4 HP Ge detectors ( ≃ 225 cm 3 volume each one) deep underground (3600 m w.e.) at the Laboratori Nazionali del Gran Sasso of the INFN (Italy). The two γ quanta of 540 keV and of 591 keV emitted in the deexcitation process after a 2 β 2 ν decay of 100Mo to the 0 1 + excited level of 100Ru ( E exc = 1131 keV ) are observed in the accumulated data both in coincidence and in the 1-dimensional sum spectrum. The measured half life is: T 1 / 2 = 6.9 − 0.8 + 1.0 ( stat. ) ± 0.7 ( syst. ) × 10 20 yr , well in agreement with positive results obtained in previous experiments. Moreover, the limit on charge non-conserving β decay of 100Mo is also set: τ CNC > 4.5 × 10 19 yr at 90% C.L.; it corresponds to the limit on CNC admixture in weak currents: ϵ ν 2 2.9 × 10 − 21 .

A cadmium tungstate crystal scintillator enriched in 106 Cd was developed for an experiment to search for double beta processes in 106 Cd. With this aim samples of cadmium with natural isotopic composition and enriched in 106 Cd were purified by vacuum distillation. Cadmium tungstate compounds were synthesized from solutions. The absolute isotopic composition of the enriched cadmium was accurately determined as 66.4% by thermal ionisation mass-spectrometry. A 106 CdWO 4 crystal boule was grown by the low-thermal-gradient Czochralski technique. The total irrecoverable loss of the enriched cadmium in all the stages of the crystal scintillator production does not exceed 2.3%. The produced 106 CdWO 4 crystal scintillator with mass of 216 g exhibits good optical and scintillation properties.

Results are presented on our latest research, aimed at the development and study of oxide scintillation crystals (ZnWO4, ZnMoO4, PbWO4, PbMoO4, and MgWO4) with high scintillation yield and low intrinsic radioactivity. We report on the improvement of these properties for conventional scintillators, as well as on new promising crystals based on metal tungstates and molybdates. The results are discussed in view of applying these materials in cryogenic experiments searching for dark matter and/or neutrinoless double beta decay. © 2006 IEEE.

In June–August 2006 an expedition with the aim to look for archaeological lead with low levels of 210 Pb was organised by a Korean–Ukrainian collaboration on the shelf of the Black Sea, near the Crimean Peninsula. The first samples with ∼0.2 ton of total mass were found at a depth of 28 m among the relics of an ancient Greek ship. Their age has been dated to the first century BC. The element composition of the samples was measured by means of X-ray fluorescence and Inductively Coupled Plasma-Mass Spectrometry (ICP-MS) analyses. The radiopurity of the lead was tested using low-level and ultra-low-level γ-spectrometry at a surface laboratory in Kyiv, at the Solotvina Underground Laboratory (Ukraine), and deep underground at the Laboratori Nazionali del Gran Sasso (LNGS, Italy). The samples have been assessed at the LNGS also by means of α-spectroscopy. For all investigated radionuclides, only upper limits could be obtained. Limits on activities of radionuclides in the lead after melting were set at the level of −1 ( 60 Co), −1 ( 137 Cs), −1 ( 226 Ra), −1 ( 228 Th), −1 ( 40 K), −1 ( 210 Po), and −1 ( 210 Pb). Any 210 Pb present in the lead after it was produced ca. 2000 years ago has decayed away. Assuming secular equilibrium in the 238 U chain in the lead, the activity of 210 Pb due to 238 U can be restricted to −1 before melting, and −1 after melting.

Light output, α / β ratio, and pulse shape have been investigated at - 25 ∘ C with PbWO 4 crystal scintillators undoped, and doped by F, Eu, Mo, Gd and S. The fast 0.01– 0.06 μ s and middle 0.1– 0.5 μ s components of scintillation decay were observed for all the samples. Slow components of scintillation signal with decay times 1–3 and 13– 28 μ s with total intensity up to ≈ 50 % have been recognized for several samples doped by Molybdenum. We found some indications of a pulse-shape discrimination between α particles and γ quanta with PbWO 4 (Mo doped) crystal scintillators.

Some recent results obtained in the search for double beta decay in vari- ous isotopes obtained in experiments carried out at LNGS with the DAMA/R&D, DAMA/Ge set-up and the STELLA facility will be summarized.

ISBN: 978-0-7354-1333-7; International audience; The LUMINEU program aims at performing a pilot experiment on 0ν2β decay of 100 Mo using radiopure ZnMoO4 crystals enriched in 100 Mo operated as cryogenic scintillating bolometers. Large volume ZnMoO4 crystal scintillators (∼ 0.3 kg) were developed and tested showing high performance in terms of radiopurity, energy resolution and α/β particle discrimination capability. Zinc molybdate crystal scintillators enriched in 100 Mo were grown for the first time by the low-thermal-gradient Czochralski technique with a high crystal yield and an acceptable level of enriched molybdenum irrecoverable losses. A background level of ∼ 0.5 counts/(yr keV ton) in the region of interest can be reached in a large detector array thanks to the excellent detectors radiopurity and particle discrimination capability, suppression of randomly coinciding events by pulse-shape analysis, and anticoincidence cut. These results pave the way to future sensitive searches based on the LUMINEU technology, capable of approaching and exploring the inverted hierarchy region of the neutrino mass pattern.

Energy resolution, light yield, non-proportionality in the scintillation response, alpha/beta ratio, pulse shape for gamma rays and alpha particles were studied with CdWO4 crystal scintillators. Some indication for a difference in the emission spectra for gamma rays and alpha particles was observed. No dependence of CdWO4 pulse shape on emission spectrum wavelengths under laser, alpha particles and gamma ray excitation was observed. Dependence of scintillation pulse shape for gamma quanta and alpha particles and pulse-shape discrimination ability on temperature was measured in the range of 0-24 degrees., Comment: 22 pages, 14 figures, submitted to NIMA

Lead tungstate (PbWO4) crystal scintillators are discussed as an active shield and light guides in Cd-116 double-beta decay experiment with Cadmium tungstate (CdWO4) scintillators. Scintillation properties and radioactive contamination of PbWO4 scintillators were investigated. Energy resolution of CdWO4 detector, coupled to PbWO4 light guide, was tested. Efficiency of PbWO4-based active shield to suppress background from the internal contamination of PbWO4 crystals, as well as possible contribution from radioactivity of copper shield and phototubes were calculated. Using of lead tungstate crystal scintillators as high-efficiency 4 pi active shield could allow to build sensitive 2 beta experiment (T-1/2(0 nu 2 beta) similar to 10(26) yr) to search for 0 nu 2 beta decay of Cd-116 with (CdWO4)-Cd-116 crystal scintillators. (c) 2005 Elsevier B.V. All rights reserved.

Energy resolution, α / β ratio, and the pulse shape discrimination ability of the ZnWO 4 crystal scintillators were studied. The radioactive contamination of a ZnWO 4 crystal was investigated in the Solotvina Underground Laboratory. Possibilities to apply ZnWO 4 crystals for the dark matter and double beta decay searches are discussed. New improved half-life limits on double beta decay in zinc isotopes were established, in particular, for ɛ β + decay of 64 Zn as: T 1 / 2 2 ν ⩾ 8.9 × 10 18 years and T 1 / 2 0 ν ⩾ 3.6 × 10 18 years, both at 68% CL.

The LUMINEU project is a demonstrator experiment that will search for the neutrinoless double beta decay of the isotope \(^{100}\)Mo embedded in zinc molybdate (ZnMoO\(_4\)) scintillating bolometers. In this context, a zinc molybdate crystal boule enriched in \(^{100}\)Mo to 99.5 % with a mass of 171 g was grown for the first time by the low-thermal-gradient Czochralski technique. The production cycle provided a high yield (the crystal boule mass was 84 % of the initial charge) and an acceptable level—around 4 %—of irrecoverable losses of the costly enriched material. Two crystals of 59 and 63 g, obtained from the enriched boule, were tested above ground at millikelvin temperatures as scintillating bolometers. They showed a good detection performance, equivalent to that of previously developed natural ZnMoO\(_4\) detectors. These results pave the way to future sensitive searches based on the LUMINEU technology, capable of approaching and exploring the inverted hierarchy region of the neutrino mass pattern.

The LUMINEU program aims at performing a pilot experiment on neutrinoless double beta decay of 100Mo using radiopure ZnMoO4 crystals operated as scintillating bolometers. Growth of high quality radiopure crystals is a complex task, since there are no commercially available molybdenum compounds with the required levels of purity and radioactive contamination. This paper discusses approaches to purify molybdenum and synthesize compound for high quality radiopure ZnMoO4 crystal growth. A combination of a double sublimation (with addition of zinc molybdate) with subsequent recrystallization in aqueous solutions (using zinc molybdate as a collector) was used. Zinc molybdate crystals up to 1.5 kg were grown by the low-thermal-gradient Czochralski technique, their optical, luminescent, diamagnetic, thermal and bolometric properties were tested., Comment: Contribution to Proc. of Int. Workshop on Radiopure Scintillators RPSCINT 2013, 17-20 September 2013, Kyiv, Ukraine; to be published in EPJ Web of Conferences; expected to be online in January 2014; 6 pages, 6 figures, and 3 tables

Cadmium tungstate crystal scintillators enriched in 106Cd and 116Cd were developed. The produced scintillators exhibit good optical and scintillation properties, and a low level of radioactive contamination. Experiments to search for double beta decay of 106Cd and 116Cd are in progress at the Gran Sasso National Laboratories of the INFN (Italy). Prospects to further improve the radiopurity of the detectors by recrystallization are discussed., Comment: 9 pages, 1 figure (4 eps-figs), 1 table. Accepted for publication in Radiation Measurements as a Proceedings of the 8th International Conference on Luminescent Detectors and Transformers of Ionizing Radiation (LUMDETR 2012), September 09-14, 2012, Halle (Saale), Germany

The studies performed in the research of new materials and purification techniques allow us a wide choice among inorganic scintillators for a variety of use. In this paper crystal scintillators and their application and potentialities in low background measurements are discussed, with a particular attention to direct dark matter investigation.

Development of low radioactive technique allows to investigate many other rare nuclear and subnuclear processes: double [Formula: see text] decay, rare [Formula: see text] and [Formula: see text] decays, and to search for hypothetical particles and processes like axions, charge nonconserving decays, the nucleon, di-nucleon and tri-nucleon decays into invisible channels, to test the Pauli principle. Here, we present results of the rare processes searches and development of instrumentation for low counting experiments.

In the anisotropic scintillators the light output and the pulse shape for heavy particles (p, α, nuclear recoils) depend on the direction with respect to the crystal axes; the response to γ/β radiation is isotropic instead. This feature offers the possibility to study the directionality approach, which is applicable in the particular case of those Dark Matter candidate particles inducing just nuclear recoils. Among the anisotropic scintillators, the ZnWO4 has unique features, which make it an excellent candidate for this type of research, and there is still plenty of room for the improvement of its performances. Studies on the exploitation of further possibilities are also considered and will be shortly mentioned. In this paper the possibility of a low background pioneer experiment (named ADAMO: Anisotropic detectors for DArk Matter Observation) to exploit the directionality approach by using anisotropic ZnWO4 scintillators is discussed.

The Aurora experiment to investigate double beta decay of $^{116}$Cd with the help of 1.162 kg cadmium tungstate crystal scintillators enriched in $^{116}$Cd to 82\% is in progress at the Gran Sasso Underground Laboratory. The half-life of $^{116}$Cd relatively to the two neutrino double beta decay is measured with the highest up-to-date accuracy $T_{1/2}=(2.62\pm0.14)\times10^{19}$ yr. The sensitivity of the experiment to the neutrinoless double beta decay of $^{116}$Cd to the ground state of $^{116}$Sn is estimated as $T_{1/2} \geq 1.9\times10^{23}$ yr at 90\% CL, which corresponds to the effective Majorana neutrino mass limit $\langle m_{\nu}\rangle \leq (1.2-1.8)$ eV. New limits are obtained for the double beta decay of $^{116}$Cd to the excited levels of $^{116}$Sn, and for the neutrinoless double beta decay with emission of majorons., Comment: 5 pages, 3 figures, 1 table, submitted as proceedings of the TAUP 2015 conference

A search for double $\ensuremath{\beta}$ processes in ${}^{106}$Cd was carried out at the Gran Sasso National Laboratories of the INFN (Italy) with the help of a ${}^{106}$CdWO${}_{4}$ crystal scintillator (215 g) enriched in ${}^{106}$Cd up to 66$%$. After 6590 h of data taking, new improved half-life limits on the double $\ensuremath{\beta}$ decay processes in ${}^{106}$Cd were established at the level of ${10}^{19}$--${10}^{21}$ yr; in particular, ${T}_{1/2}^{2\ensuremath{\nu}\ensuremath{\varepsilon}{\ensuremath{\beta}}^{+}}\ensuremath{\geqslant}2.1\ifmmode\times\else\texttimes\fi{}{10}^{20}$ yr, ${T}_{1/2}^{2\ensuremath{\nu}2{\ensuremath{\beta}}^{+}}\ensuremath{\geqslant}4.3\ifmmode\times\else\texttimes\fi{}{10}^{20}$ yr, and ${T}_{1/2}^{0\ensuremath{\nu}2\ensuremath{\varepsilon}}\ensuremath{\geqslant}1.0\ifmmode\times\else\texttimes\fi{}{10}^{21}$ yr. The resonant neutrinoless double-electron captures to the 2718-, 2741-, and 2748-keV excited states of ${}^{106}$Pd are restricted to ${T}_{1/2}^{0\ensuremath{\nu}2K}\ensuremath{\geqslant}4.3\ifmmode\times\else\texttimes\fi{}{10}^{20}$ yr, ${T}_{1/2}^{0\ensuremath{\nu}K{L}_{1}}\ensuremath{\geqslant}9.5\ifmmode\times\else\texttimes\fi{}{10}^{20}$ yr, and ${T}_{1/2}^{0\ensuremath{\nu}K{L}_{3}}\ensuremath{\geqslant}4.3\ifmmode\times\else\texttimes\fi{}{10}^{20}$ yr, respectively (all limits at 90$%$ confidence level). A possible resonant enhancement of the $0\ensuremath{\nu}2\ensuremath{\varepsilon}$ processes is estimated in the framework of the quasiparticle random phase approximation (QRPA) approach. Radioactive contamination of the ${}^{106}$CdWO${}_{4}$ crystal scintillator is reported.

Several experiments were performed during last years at underground (3600 m w.e.) Laboratori Nazionali del Gran Sasso (LNGS) of the INFN (Italy) to search for resonant 2$\varepsilon0\nu$ captures in 96Ru, 106Cd, 136Ce, 156Dy, 158Dy, 180W, 184Os, 190Pt with the help of HP Ge semiconductor detectors, and ZnWO4 and 106CdWO4 crystal scintillators. No evidence for r-2$\varepsilon0\nu$ decays was found, and only T_{1/2} limits were established in the range of 10^{14}-10^{21} yr., Comment: Proceedings of TAUP 2011 Conference

In June‐August 2006 an expedition with the aim to look for low‐radioactive archaeological lead at the bottom of the Black Sea, near the Crimean peninsula (Ukraine) was organised by a Korean‐Ukrainian collaboration. The first samples with ∼0.2 tons of total mass were found at a depth of 28 m among the relics of an ancient Greek ship. Their age has been dated to the first century B.C. This lead was used as ballast in the keel of the ship. The element composition of the samples was measured by means of X‐ray fluorescence and ICP‐MS analyses. The first preliminary limits on the 210Pb contamination of the samples are less than a few hundreds mBq/kg. The measurements were performed using gamma spectroscopy with HPGe‐detectors and alpha spectroscopy with commercial α‐detectors. Measurements of 40K, Th/U in the lead samples were undertaken in Kiev and in the underground laboratories of the Laboratori Nazionali del Gran Sasso (LNGS, Italy). If it was found to be radio‐clean this lead could be used as high efficien...

Radioactive contaminations of CaWO4, ZnWO4, CdWO4, and Gd2SiO5:Ce crystal scintillators were measured in the Solotvina Underground Laboratory. The Monte Carlo simulation of contributing radioactive sources, the time‐amplitude and pulse‐shape analyses of the experimental data were applied. CaWO4 and GSO scintillators are considerably polluted by uranium and thorium, while the total α activity in ZnWO4 and CdWO4 scintillators does not exceed the level of a few mBq/kg. Particular radioactivity was observed in CaWO4 (α active 180W), CdWO4 (β active 113Cd, 2v2β decay of 116Cd, 180W), and GSO (α active 152Gd) detectors. The radioactive contamination of the studied scintillation crystals is compared with that of commonly used detectors.

Radiopure ZnWO 4 crystal scintillators with mass (0.1–0.7 kg) have been developed and put inmeasurement in the Gran Sasso National Laboratories of the INFN to search for rare processes. The radioactive contamination of the crystals have been estimated and the double beta decay of zinc and tungsten isotopes was searched for, reaching a sensitivity at the level of 10 18 −10 21 yr; in addition a new half-life limit on alpha transition of 183 W to the metastable excited level of 179 Hf has also been obtained. The achieved radiopurity of the ZnWO 4 crystals make them very promising detectors for ββ decay investigations while their anisotropic features make them very interesting detectors to investigate dark matter particles directionality.

Cadmium tungstate crystal scintillators enriched in $^{116}$Cd to 82% ($^{116}$CdWO$_4$, total mass of $\approx$1.2 kg) are used to search for 2$\beta$ decay of $^{116}$Cd deep underground at the Gran Sasso National Laboratory of the INFN (Italy). The radioactive contamination of the $^{116}$CdWO$_4$ crystals has been studied carefully to reconstruct the background of the detector. The measured half-life of $^{116}$Cd relatively to 2$\nu$2$\beta$ decay is $T^{2\nu2\beta}_{1/2}$ = [2.8 $\pm$ 0.05(stat.) $\pm$ 0.4(syst.)] $\times$ 10$^{19}$ yr, in agreement with the results of previous experiments. The obtained limit on the 0$\nu$2$\beta$ decay of $^{116}$Cd (considering the data of the last 8696 h run with an advanced background 0.12(2) counts/yr/kg/keV in the energy interval 2.7-2.9 MeV) is $T_{1/2} \ge 1.0 \times 10^{23}$ yr at 90% C.L. The sensitivity of the experiment to the $0\nu2\beta$ process is $\lim T_{1/2} = 3 \times 10^{23}$ yr at 90% C.L. over 5 years of the measurements and it can be advanced (by further reduction of the background by a factor 3-30) to the level of $\lim T_{1/2} = (0.5-1.5) \times 10^{24}$ yr for the same period of the data taking., Comment: Contribution to Proc. of Int. Workshop on Radiopure Scintillators RPSCINT 2013, 17-20.09.2013, Kyiv, Ukraine; to be published in EPJ Web of Conferences; 4 pages, 1 figure and 3 tables

A search for double ? processes in 106Cd was carried out at the Gran Sasso National Laboratories of the INFN, Italy; by using a CdWC4 crystal scintillator (mass of 215 g) enriched in 106Cd up to 66%. After 6590 h of data taking, half-life limits on double beta processes in 106Cd were set at level of 1019 ? 1021 yr. A possible resonant enhancement of the 0?2? processes has also been estimated in the framework of the QRPA approach.

AMoRE (Advanced Mo based Rare process Experiment) collaboration is going to use calcium molybdate crystals as cryogenic scintillation detector in a search for neutrinoless DBD of 100Mo isotope. Simultaneous detection of phonons and light will be used to reject internal background. A FWHM resolution of 0.2% in the phonon channel has been achieved with a 0.5 cm3 crystal. Several 40Ca100MoO4 crystals (≈ 0.5 kg) have been developed from enriched 100Mo and depleted 40Ca materials. The light yield of these crystals has been shown to be comparable with reference CaMoO4 scintillators for temperatures ranging down to 8 K. The content of dangerous radioisotopes in the crystals is under measurement. The projected sensitivity of the experiment for a 250 kg × years exposure is lim T1/2 ~ 3 × 1026 years, which corresponds to the effective Majorana neutrino mass mv ~ 0.02 – 0.06 eV.

Sample of 100MoO3 with molybdenum enriched in 100Mo to 99.5% and mass of 1199 g was measured deep underground (3600 m w.e.) in the Laboratori Nazionali del Gran Sasso of INFN, Italy; during 17249 h with a low-background set-up with 4 HP Ge detectors. After 2β2ν decay of 100Mo to the 0+1 excited level of 100Ru (Eexc = 1131 keV), two γ quanta of 540 keV and 591 keV should be emitted in deexcitation process. Both these γ's are observed in the accumulated data as in coincidence spectrum as well in 1-dimensional sum spectrum. Measured half life is T1/2 = (7.0+1.1−0.8) × 1020 yr, in agreement with positive results obtained in previous experiments.

EURECA (European Underground Rare Event Calorimeter Array) is an astro-particle physics facility aiming to directly detect galactic dark matter. The Laboratoire Souterrain de Modane has been selected as host laboratory. The EURECA collaboration unites CRESST, EDELWEISS and the Spanish-French experiment ROSEBUD, thus concentrating and focussing effort on cryogenic detector research in Europe into a single facility. EURECA will use a target mass of up to one ton, enough to explore WIMP - nucleon scalar scattering cross sections in the region of 10-9 - 10-10 picobarn. A major advantage of EURECA is the planned use of more than just one target material (multi target experiment for WIMP identification). © EAS, EDP Sciences 2009.