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1. On the adsorption and reactivity of element 114, flerovium

Author

Yakushev, A., Lens, Lotte, Düllmann, Ch. E., Khuyagbaatar, J., Jäger, E., Krier, J., Runke, J., Albers, H. M., Asai, M., Block, M., Despotopulos, J., Di Nitto, Antonio, Eberhardt, K., Forsberg, U., Golubev, P., Götz, M., Götz, Stefan, Haba, H., Harkness-Brennan, L., Herzberg, R.-D., Heßberger, F., Hinde, D., Hübner, A., Judson, D., Kindler, B., Komori, Y., Konki, J., Kratz, J. V., Kurz, N., Laatiaoui, Mustapha, Lahiri, S., Lommel, B., Maiti, M., Mistry, A. K., Mokry, Ch., Moody, K. J., Nagame, Y., Omtvedt, J. P., Papadakis, P., Pershina, V., Rudolph, D., Samiento, L. G., Sato, T. K., Schädel, M., Scharrer, P., Schausten, B., Shaughnessy, D. A., Steiner, J., Thörle-Pospiech, P., Toyoshima, A., Trautmann, N., Tsukada, K., Uusitalo, J., Voss, K.-O., Ward, A., Wegrzecki, M., Wiehl, N., Williams, E., Yakusheva, V., Yakushev, A., Lens, L., Dullmann, C. E., Khuyagbaatar, J., Jager, E., Krier, J., Runke, J., Albers, H. M., Asai, M., Block, M., Despotopulos, J., Di Nitto, A., Eberhardt, K., Forsberg, U., Golubev, P., Gotz, M., Gotz, S., Haba, H., Harkness-Brennan, L., Herzberg, R. -D., Hessberger, F. P., Hinde, D., Hubner, A., Judson, D., Kindler, B., Komori, Y., Konki, J., Kratz, J. V., Kurz, N., Laatiaoui, M., Lahiri, S., Lommel, B., Maiti, M., Mistry, A. K., Mokry, C., Moody, K. J., Nagame, Y., Omtvedt, J. P., Papadakis, P., Pershina, V., Rudolph, D., Samiento, L. G., Sato, T. K., Schadel, M., Scharrer, P., Schausten, B., Shaughnessy, D. A., Steiner, J., Thorle-Pospiech, P., Toyoshima, A., Trautmann, N., Tsukada, K., Uusitalo, J., Voss, K. -O., Ward, A., Wegrzecki, M., Wiehl, N., Williams, E., and Yakusheva, V.

Subjects
superheavy elements, adsorption, ddc:540, General Chemistry, radiochemistry, nuclear chemistry, element 114, recoil separator
Abstract

Frontiers in Chemistry 10, 976635 (2022). doi:10.3389/fchem.2022.976635, Flerovium (Fl, element 114) is the heaviest element chemically studied so far. Todate, its interaction with gold was investigated in two gas-solid chromatographyexperiments, which reported two different types of interaction, however, eachbased on the level of a few registered atoms only. Whereas noble-gas-likeproperties were suggested from the first experiment, the second one pointed ata volatile-metal-like character. Here, we present further experimental data onadsorption studies of Fl on silicon oxide and gold surfaces, accounting for theinhomogeneous nature of the surface, as it was used in the experiment andanalyzed as part of the reported studies. We confirm that Fl is highly volatile andthe least reactive member of group 14. Our experimental observations suggestthat Fl exhibits lower reactivity towards Au than the volatile metal Hg, but higherreactivity than the noble gas Rn., Published by Frontiers Media, Lausanne

Published
2022
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2. Spectroscopy along Flerovium Decay Chains: Discovery of ^{280}Ds and an Excited State in ^{282}Cn

Author

Såmark-Roth, A., Cox, D. M., Rudolph, D., Sarmiento, L. G., Carlsson, B. G., Egido, J. L., Golubev, P., Heery, J., Yakushev, A., Åberg, S., Albers, H. M., Albertsson, M., Block, M., Brand, H., Calverley, T., Cantemir, R., Clark, R. M., Düllmann, Ch. E., Eberth, J., Fahlander, C., Forsberg, U., Gates, J. M., Giacoppo, F., Götz, M., Götz, S., Herzberg, R.-D., Hrabar, Y., Jäger, E., Judson, D., Khuyagbaatar, J., Kindler, B., Kojouharov, I., Kratz, J. V., Krier, J., Kurz, N., Lens, L., Ljungberg, J., Lommel, B., Louko, J., Meyer, C.-C., Mistry, A., Mokry, C., Papadakis, P., Parr, E., Pore, J. L., Ragnarsson, I., Runke, J., Schädel, M., Schaffner, H., Schausten, B., Shaughnessy, D. A., Thörle-Pospiech, P., Trautmann, N., and Uusitalo, J.

Subjects
General Physics, Engineering, Superheavy elements, Subatomic Physics, Island of stability, Physical Sciences, Mean field theory, Alpha decay, ddc:530, Mathematical Sciences, Nuclear spectroscopy
Abstract

Physical review letters 126(3), 032503 (2021). doi:10.1103/PhysRevLett.126.032503, Published by APS, College Park, Md.

Published
2021
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3. Low-lying states in Ra219 and Rn215: Sampling microsecond α-decaying nuclei

Author

Såmark-Roth, A, Sarmiento, LG, Rudolph, D, Ljungberg, J, Carlsson, BG, Fahlander, C, Forsberg, U, Golubev, P, Ragnarsson, I, Ackermann, D, Andersson, L-L, Block, M, Brand, H, Cox, DM, Di Nitto, A, Düllmann, Ch E, Eberhardt, K, Even, J, Gates, JM, Gerl, J, Gregorich, KE, Gross, CJ, Herzberg, R-D, Heßberger, FP, Jäger, E, Khuyagbaatar, J, Kindler, B, Kojouharov, I, Kratz, JV, Krier, J, Kurz, N, Lommel, B, Mistry, A, Mokry, C, Omtvedt, JP, Papadakis, P, Runke, J, Rykaczewski, K, Schädel, M, Schaffner, H, Schausten, B, Thörle-Pospiech, P, Trautmann, N, Torres, T, Türler, A, Ward, A, Wiehl, N, and Yakushev, A

Subjects
Particle and Plasma Physics, Molecular, Nuclear, Atomic, Nuclear & Particles Physics
Abstract

Short-lived α-decaying nuclei "northeast" of Pb208 in the chart of nuclides were studied using the reaction Ca48+Am243 with the decay station TASISpec at TASCA, GSI Darmstadt. Decay energies and times from pile-up events were extracted with a tailor-made pulse-shape analysis routine and specific α-decay chains were identified in a correlation analysis. Decay chains starting with the even-even Ra220 and its odd-A neighbors, Fr219, and Ra221,219, with a focus on the Ra219→Rn215 decay, were studied by means of α-γ spectroscopy. A revised α-decay scheme of Ra219 is proposed, including a new decay branch from a previously not considered isomeric state at 17 keV excitation energy. Conclusions on nuclear structure are drawn from the experimental data, aided by Geant4 simulations and a discussion on theoretical calculations.

Published
2018

4. Study of non-fusion products in the Ti50+Cf249 reaction

Author

Di Nitto, A, Khuyagbaatar, J, Ackermann, D, Andersson, LL, Badura, E, Block, M, Brand, H, Conrad, I, Cox, DM, Düllmann, CE, Dvorak, J, Eberhardt, K, Ellison, PA, Esker, NE, Even, J, Fahlander, C, Forsberg, U, Gates, JM, Golubev, P, Gothe, O, Gregorich, KE, Hartmann, W, Herzberg, RD, Heßberger, FP, Hoffmann, J, Hollinger, R, Hübner, A, Jäger, E, Kindler, B, Klein, S, Kojouharov, I, Kratz, JV, Krier, J, Kurz, N, Lahiri, S, Lommel, B, Maiti, M, Mändl, R, Merchán, E, Minami, S, Mistry, AK, Mokry, C, Nitsche, H, Omtvedt, JP, Pang, GK, Renisch, D, Rudolph, D, Runke, J, Sarmiento, LG, Schädel, M, Schaffner, H, Schausten, B, Semchenkov, A, Steiner, J, Thörle-Pospiech, P, Trautmann, N, Türler, A, Uusitalo, J, Ward, D, Wegrzecki, M, Wieczorek, P, Wiehl, N, Yakushev, A, Yakusheva, V, Di Nitto, A., Khuyagbaatar, J., Ackermann, D., Andersson, L. -L., Badura, E., Block, M., Brand, H., Conrad, I., Cox, D. M., Dullmann, C. E., Dvorak, J., Eberhardt, K., Ellison, P. A., Esker, N. E., Even, J., Fahlander, C., Forsberg, U., Gates, J. M., Golubev, P., Gothe, O., Gregorich, K. E., Hartmann, W., Herzberg, R. D., Hessberger, F. P., Hoffmann, J., Hollinger, R., Hubner, A., Jager, E., Kindler, B., Klein, S., Kojouharov, I., Kratz, J. V., Krier, J., Kurz, N., Lahiri, S., Lommel, B., Maiti, M., Mandl, R., Merchan, E., Minami, S., Mistry, A. K., Mokry, C., Nitsche, H., Omtvedt, J. P., Pang, G. K., Renisch, D., Rudolph, D., Runke, J., Sarmiento, L. G., Schadel, M., Schaffner, H., Schausten, B., Semchenkov, A., Steiner, J., Thorle-Pospiech, P., Trautmann, N., Turler, A., Uusitalo, J., Ward, D., Wegrzecki, M., Wieczorek, P., Wiehl, N., Yakushev, A., and Yakusheva, V.

Subjects
Multi-nucleon transfer reactions, alpha decay, Molecular, Production of radioactive nuclei, Atomic, Nuclear & Particles Physics, lcsh:QC1-999, Particle and Plasma Physics, Quasifission, Nuclear, Multi-nucleon transfer reaction, α decay, Nuclear Experiment, lcsh:Physics, Mathematical Physics, Astronomical and Space Sciences
Abstract

The isotopic distribution of nuclei produced in the 50Ti + 249Cf reaction has been studied at the gas-filled recoil separator TASCA at GSI Darmstadt, which separates ions according to differences in magnetic rigidity. The bombardment was performed at an energy around the Bass barrier and with the TASCA magnetic fields set for collecting fusion-evaporation reaction products. Fifty-three isotopes located “north-east” of 208Pb were identified as recoiling products formed in non-fusion channels of the reaction. These recoils were implanted with energies in two distinct ranges; besides one with higher energy, a significant low-energy contribution was identified. The latter observation was not expected to occur according to kinematics of the known types of reactions, namely quasi-elastic, multi-nucleon transfer, deep-inelastic collisions or quasifission. The present observations are discussed within the framework of two-body kinematics passing through the formation of a composite system. Keywords: Production of radioactive nuclei, α decay, Multi-nucleon transfer reactions, Quasifission

Published
2018
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5. Study of non-fusion products in the Ti 50 + Cf 249 reaction

Author

Di Nitto, A, Khuyagbaatar, J, Ackermann, D, Andersson, L-L, Badura, E, Block, M, Brand, H, Conrad, I, Cox, DM, Düllmann, Ch E, Dvorak, J, Eberhardt, K, Ellison, PA, Esker, NE, Even, J, Fahlander, C, Forsberg, U, Gates, JM, Golubev, P, Gothe, O, Gregorich, KE, Hartmann, W, Herzberg, RD, Heßberger, FP, Hoffmann, J, Hollinger, R, Hübner, A, Jäger, E, Kindler, B, Klein, S, Kojouharov, I, Kratz, JV, Krier, J, Kurz, N, Lahiri, S, Lommel, B, Maiti, M, Mändl, R, Merchán, E, Minami, S, Mistry, AK, Mokry, C, Nitsche, H, Omtvedt, JP, Pang, GK, Renisch, D, Rudolph, D, Runke, J, Sarmiento, LG, Schädel, M, Schaffner, H, Schausten, B, Semchenkov, A, Steiner, J, Thörle-Pospiech, P, Trautmann, N, Türler, A, Uusitalo, J, Ward, D, Wegrzecki, M, Wieczorek, P, Wiehl, N, Yakushev, A, and Yakusheva, V

Subjects
Multi-nucleon transfer reactions, Particle and Plasma Physics, alpha decay, Quasifission, Molecular, Nuclear, Production of radioactive nuclei, Atomic, Nuclear & Particles Physics, Mathematical Physics, Astronomical and Space Sciences
Abstract

The isotopic distribution of nuclei produced in the 50Ti + 249Cf reaction has been studied at the gas-filled recoil separator TASCA at GSI Darmstadt, which separates ions according to differences in magnetic rigidity. The bombardment was performed at an energy around the Bass barrier and with the TASCA magnetic fields set for collecting fusion-evaporation reaction products. Fifty-three isotopes located “north-east” of 208Pb were identified as recoiling products formed in non-fusion channels of the reaction. These recoils were implanted with energies in two distinct ranges; besides one with higher energy, a significant low-energy contribution was identified. The latter observation was not expected to occur according to kinematics of the known types of reactions, namely quasi-elastic, multi-nucleon transfer, deep-inelastic collisions or quasifission. The present observations are discussed within the framework of two-body kinematics passing through the formation of a composite system.

Published
2018

6. New Short-Lived Isotope ^{221}U and the Mass Surface Near N=126

Author

Khuyagbaatar, J., Yakushev, A., Düllmann, Ch. E., Ackermann, D., Andersson, L.-L., Block, M., Brand, H., Cox, D. M., Even, J., Forsberg, Ulrika, Golubev, Pavel, Hartmann, W., Herzberg, R.-D., Heßberger, F. P., Hoffmann, J., Hübner, A., Jäger, E., Jeppsson, J., Kindler, B., Kratz, J. V., Krier, J., Kurz, N., Lommel, B., Maiti, M., Minami, S., Mistry, A. K., Mrosek, Ch. M., Pysmenetska, I., Rudolph, Dirk, Sarmiento, Luis, Schaffner, H., Schädel, M., Schausten, B., Steiner, J., De Heidenreich, T. Torres, Uusitalo, J., Wegrzecki, M., Wiehl, N., and Yakusheva, V.

Subjects
Shell Structure, Heavy Elements Shell Structure Sampling Electronics, Heavy Elements, Sampling Electronics, Subatomic Physics
Abstract

Two short-lived isotopes ^{221}U and ^{222}U were produced as evaporation residues in the fusion reaction ^{50}Ti+^{176}Yb at the gas-filled recoil separator TASCA. An α decay with an energy of E_{α}=9.31(5) MeV and half-life T_{1/2}=4.7(7) μs was attributed to ^{222}U. The new isotope ^{221}U was identified in α-decay chains starting with E_{α}=9.71(5) MeV and T_{1/2}=0.66(14) μs leading to known daughters. Synthesis and detection of these unstable heavy nuclei and their descendants were achieved thanks to a fast data readout system. The evolution of the N=126 shell closure and its influence on the stability of uranium isotopes are discussed within the framework of α-decay reduced width.

Published
2015

7. Experimental study of the U238(S36,3-5n)Hs269-271 reaction leading to the observation of Hs270

Author

Graeger, R, Ackermann, D, Chelnokov, M, Chepigin, V, Düllmann, CE, Dvorak, J, Even, J, Gorshkov, A, Heßberger, FP, Hild, D, Hübner, A, Jäger, E, Khuyagbaatar, J, Kindler, B, Kratz, JV, Krier, J, Kuznetsov, A, Lommel, B, Nishio, K, Nitsche, H, Omtvedt, JP, Petrushkin, O, Rudolph, D, Runke, J, Samadani, F, Schädel, M, Schausten, B, Türler, A, Yakushev, A, and Zhi, Q

Subjects
Particle and Plasma Physics, Molecular, Nuclear, Nuclear & Particles Physics, Atomic
Abstract

The deformed doubly magic nucleus Hs270 has so far only been observed as the four-neutron (4n) evaporation residue of the reaction Mg26+Cm248, where a maximum cross section of 3 pb was measured. Theoretical studies on the formation of Hs270 in the 4n evaporation channel of fusion reactions with different entrance channel asymmetry in the framework of a two-parameter Smoluchowski equation predict that the reactions Ca48+Ra226 and S36+U238 result in higher cross sections due to lower reaction Q values, in contrast to simple arguments based on the reaction asymmetry, which predict opposite trends. Calculations using hivap predict cross sections for the reaction S36+U238 that are similar to those of the Mg26+Cm248 reaction. Here, we report on the first measurement of evaporation residues formed in the complete nuclear fusion reaction S36+U238 and the observation of Hs270, which is produced in the 4n evaporation channel, with a measured cross section of 0.8-0.7+2.6 pb at 51-MeV excitation energy. The one-event cross-section limits (68% confidence level) for the 3n, 4n, and 5n evaporation channels at 39-MeV excitation energy are 2.9 pb, while the cross-section limits of the 3n and 5n channel at 51 MeV are 1.5 pb. This is significantly lower than the 5n cross section of the Mg26+Cm248 reaction at similar excitation energy. © 2010 The American Physical Society.

Published
2010
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20. Aqueous Chemistry of Seaborgium (Z = 106)

Author

Schädel, M., Brüchle, W., Jäger, E., Schausten, B., Wirth, G., Paulus, W., Günther, R., Eberhardt, K., Kratz, J. V., Seibert, A., Strub, E., Thörle, P., Trautmann, N., Waldek, A., Zauner, S., Schumann, D., Kirbach, U., Kubica, B., Ryszard Misiak, Nagame, Y., and Gregorich, K. E.

24. Efficient in vivo priming by vaccination with recombinant NY-ESO-1 protein and CpG in antigen naive prostate cancer patients

Author

Kathrin Brand, Elke Jäger, Lotta von Boehmer, Armin Bender, Antje Neumann, Lloyd J. Old, Alexander Knuth, Claudia Wahle, Gerd Ritter, Akin Atmaca, Julia Karbach, University of Zurich, and Jäger, E

Subjects
CD4-Positive T-Lymphocytes, Male, Cancer Research, Injections, Intradermal, medicine.medical_treatment, 610 Medicine & health, Adaptive Immunity, CD8-Positive T-Lymphocytes, Cancer Vaccines, Prostate cancer, Antigen, Adjuvants, Immunologic, Antigens, Neoplasm, Medicine, Humans, 1306 Cancer Research, biology, business.industry, Antibody titer, Membrane Proteins, Prostatic Neoplasms, medicine.disease, Vaccination, Treatment Outcome, Oncology, CpG site, Oligodeoxyribonucleotides, Chemotherapy, Adjuvant, Immunology, 10032 Clinic for Oncology and Hematology, biology.protein, 2730 Oncology, Recombinant NY-ESO-1 Protein, Antibody, business, Adjuvant
Abstract

Purpose: NY-ESO-1, one of the most immunogenic tumor antigens, is expressed in 15% to 25% of metastatic prostate cancers. The immunological and clinical effects of vaccination with recombinant NY-ESO-1 protein combined with CpG as adjuvant were evaluated. Experimental Design: In a phase I clinical study, patients with advanced prostate cancer were vaccinated with recombinant NY-ESO-1 protein (100 μg) mixed with CpG 7909 (2.5 mg) every 3 weeks intradermally for 4 doses. Objectives of the study were the safety of the vaccine and changes of specific humoral and cellular immunological responses to NY-ESO-1 in relation to detectable NY-ESO-1 expression in the individual tumor. Results: All 12 baseline sero-negative patients developed high-titer NY-ESO-1 antibody responses. B-cell epitope mapping identified NY-ESO-1 p91–110 to be recognized most frequently by vaccine-induced antibodies. Two patients developed significant antibody titers against the adjuvant CpG. NY-ESO-1-specific CD4+ and/or CD8+ T-cell responses were induced in 9 patients (69%). Five of these 9 patients did not express NY-ESO-1 in the autologous tumor. Postvaccine CD8+ T-cell clones recognized and lyzed HLA-matched tumor cell lines in an antigen-specific manner. Conclusion: Our data provide clear evidence for the capacity of NY-ESO-1 protein/CpG vaccine to induce integrated antigen-specific immune responses in vivo and to efficiently prime CD8+ T-cell responses in NY-ESO-1 antigen-negative patients. Our results may also support further clinical vaccination protocols with NY-ESO-1 protein not only focused on the treatment of existing cancer, but also to prevent further development of NY-ESO-1 positive cancers in vivo. Clin Cancer Res; 17(4); 1–10. ©2010 AACR.

Published
2010

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