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Spatiotemporal patterns of column-averaged dry air mole fraction of CO2 (XCO2) have not been well characterized on a regional scale due to limitations in data availability and precision. This paper addresses these issues by examining such patterns in China using the long-term mapping XCO2 dataset (2009–2016) derived from the Greenhouse gases Observing SATellite (GOSAT). XCO2 simulations are also constructed using the high-resolution nested-grid GEOS-Chem model. The following results are found: Firstly, the correlation coefficient between the anthropogenic emissions and XCO2 spatial distribution is nearly zero in summer but up to 0.32 in autumn. Secondly, on average, XCO2 increases by 2.08 ppm every year from 2010 to 2015, with a sharp increase of 2.6 ppm in 2013. Lastly, in the analysis of three typical regions, the GOSAT XCO2 time series is in better agreement with the GEOS-Chem simulation of XCO2 in the Taklimakan Desert region (the least difference with bias 0.65±0.78 ppm), compared with the northern urban agglomeration region (−1.3±1.2 ppm) and the northeastern forest region (−1.4±1.4 ppm). The results are likely attributable to uncertainty in both the satellite-retrieved XCO2 data and the model simulation data. [ABSTRACT FROM AUTHOR]