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The term "laser microexplosion" has been introduced to stress the violent character of the optical breakdown by laser radiation under conditions of tight focusing. Generally, the starting phase of the breakdown has been neglected by the assumption of absorption triggered by the presence of damage precursors. The application of the plasticity–elasticity theory in the analysis of the dynamics of this phenomenon has not been extensively examined to date. This paper formulates a phenomenological model attempting to explain the creation of nanovoids in a soft matter under irradiation by a flux of extreme ultraviolet (XUV)/soft x-ray photons. The combined action of plastic deformation and dissociation waves on soft matter is found to be responsible for the material modifications. It is suggested that localized (volume ≃ λ 3) abundance of energy, coming most likely from photon bunching, constitutes the real onset of the photo-ablative decomposition. It is shown that the coincidental presence of some small number of energy carriers (2–3 XUV photons in the considered case) in such a small volume triggers processes denoted from now on as a laser nanoexplosion. The effect is considered to be the first step in the optical breakdown followed by an intense material removal resembling, to some extent, a phase explosion. [ABSTRACT FROM AUTHOR]

We present results of applying a compact laboratory system based on a laser-plasma soft X-ray (SXR) source to the extended X-ray absorption fine structure (EXAFS) spectroscopy of titanium in the vicinity of the LIII absorption edge. The source, operating with a plasma produced as a result of irradiation a krypton/helium double-stream gas-puff target, was optimized for an intense emission in the spectral range between 200 and 700 eV. A broad SXR spectrum and high photon flux are indispensable in the EXAFS studies. The experimental setup assured the simultaneous acquisition of both the reference and the absorption spectra. A grazing-incidence flat-field spectrometer was used to record the spectra. The absorption spectra of a thin (200-nm thick) titanium sample revealed the features in the EXAFS region allowing for quite accurate determination of the radial distances between the atoms. Results are in good agreement with the output of numerical modeling based on photoelectron wave function scattering and with the data reported for using a synchrotron source. This confirms the suitability of the source for using it in the standard EXAFS method. [ABSTRACT FROM AUTHOR]

In this work, we demonstrate near-edge X-ray absorption fine structure spectroscopy of agarose with a compact laboratory laser-plasma soft X-ray source. The source is based on a double stream gas puff target irradiated by nanosecond laser pulses. The emission spectra of the source and the absorption spectra of the investigated sample were measured simultaneously using a flat-field spectrometer. Soft X-ray emission from a krypton/helium target in the range between 1.5 and 5 nm was applied as the source. The transmission measurements revealed the specific spectral features near the carbon K - α absorption edge corresponding well to the results obtained with synchrotron radiation. [ABSTRACT FROM AUTHOR]

It is well known that from the two fundamental thermodynamic parameters pressure p is much more efficient in transformation of the matter state than temperature T. Optical breakdown in a form of microexplosion proved to be a simple, cheap, and efficient source of transient extreme pressure and temperature. Our interest is focused on the breakdown performed with femstosecond laser pulses both on a surface and in the bulk of material. The paper delivers some examples of the transformation effects observed mostly in the transparent dielectrics under irradiation with femtosecond laser pulses. [ABSTRACT FROM AUTHOR]

Portion of energy employed by a single, tightly focused laser pulse in various transparent dielectrics was demonstrated versus the incident energy fluence or alternatively, intensity. The measurements were conducted for both the femtosecond and nanosecond laser pulses. Moreover, the energy scattered during the long-lived breakdown process was estimated within the integrating sphere. It appeared that the recorded strongly non-linear dependence of absorptance on the energy fluence (intensity) can be well approximated by the sigmoidal Hill function. The stationary points of the absorptance curve were used to determine threshold-like values characterizing breakdown development. In this way, we defined threshold for the non-linear absorption which can be considered as an empirical laser-induced breakdown threshold (LIBT). Additionally, the fitting parameters of the experimental data substantiated the absorption character for short and long laser pulses. [ABSTRACT FROM AUTHOR]

Ultrafast time-resolved x-ray absorption near edge spectroscopy (XANES) experiment was performed on a magnetite (Fe 3 O 4 ) film using a femtosecond laser plasma x-ray source delivering Bremsstrahlung radiation. Ultrafast temporal evolution of the XANES of Fe 3 O 4 following an excitation by an infra-red (IR) laser pulse was observed in a pump-probe scheme. The Fe K x-ray absorption edge shifts towards low energy upon IR excitation as much as 12 eV, which is mainly attributed to the charge transfer between the Fe ions. The shift in the absorption edge occurred within about 150 fs, typical time of non-thermal electronic redistribution. The charge transfer also causes an ultrafast increase in the IR transmission in the similar time scale.

Dynamics of laser-induced optical breakdown in the bulk of fused-silica glass irradiated by a sub-nanosecond laser pulse at a wavelength of 790 nm with a fluence of 522 J/cm 2 was studied by the femtosecond time-resolved complex interferometry in Nomarski arrangement utilising a Fresnel bi-prism. Evolution of the plasma channel and the development of the free electron density were in focus of the investigation. The measured ultimate length of the plasma channel was equal to 30 μm and almost doubled the length estimated within the moving breakdown model. The history of the transient electron density distribution in the plasma was reconstructed from the phase shift maps using the inverse Abel transform and it revealed further deviation from this model. The core of the plasma channel exhibited at the last stages of the development a considerable level of the electron density up to 2.4×10 20 cm -3 . The signature of the pre-breakdown phase has been identified as radiation caused by ionization-released electrons interacting with ions and has been demonstrated in solids for the first time in this way. Origin of the discrepancy between the theoretical prediction of the moving breakdown model and the measured values of the channel length is discussed as well.

It is shown that the statistics of the intensity distribution in the output beam of a collisional X-ray laser, analysed in terms of the degree of freedom or equivalently the number of the coherence modes in the beam cross-section, has non-Gaussian character. The non-Gaussian character seems to be caused by the small-scale plasma/medium fluctuations. It was assumed that these overlap the modal structure imposed by the geometry of the medium and considered as equivalent to a large-scale inhomogeneity. Thus, the fluctuations decide about the character of the output beam transverse coherence. It is also shown that the relevant to this model compound statistics of the intensity fluctuations in the output beam is well described by the m-m-distribution, a specific form of the K-distribution. The deviation from the Gaussian statistics was confirmed by the field correlation function at the laser exit plane, retrieved from the experimental data.

Soft x-ray lasers pumped in the grazing incidence geometry show strongly reduced energetic needs but hardly changed conversion efficiency between the pump energy and the output short-wavelength radiation. Numerical analysis presented in the paper concerns with performance of a Ni-like Ag soft-x-ray laser pumped by a triple-pulse structure in the grazing incidence geometry as a function of the puming conditions. It was found that a weak precursor preceding the main preforming and heating pulses by a few nanoseconds is crucial for the energy deposition. Its presence enables in different arrangements a reasonable reduction in the pump energy and relaxation of the steep density gradients as well as a control over partition of the deposited energy. As a consequence, it was concluded that a well energetically balanced three- or multipulse composition seems to be a reasonable way to achieve performance improvement.

The operation of a Ni-like Mo x-ray laser at 18.9 nm with a repetition rate of 10 Hz has been demonstrated. The laser has been pumped applying the grazing incidence pump arrangement, where a short (picoseconds) pulse irradiates a Mo plasma column generated by a long (a few hundred picoseconds) pulse. The delayed short pulse is incident at a grazing angle on the plasma to heat it efficiently. We used a total energy of less than 450 mJ ( 150 mJ in the long and 250-300 mJ in the short pulse) in a line focus of 7 mm by 50 microm .