1. Symmetric/asymmetric p- and n-induced fission of Th, Pa, U and Np.
- Author
-
Maslov, Vladimir M.
- Subjects
PARTICLES (Nuclear physics) ,NUCLEAR reactions ,NUCLEAR fission ,NUCLEAR excitation ,ATOMS - Abstract
The excitation energy and nucleon composition dependence of the transition from asymmetric to symmetric scission of fission observables of Th(Pa) and U(Np) nuclei is interpreted for nucleon-induced fission cross sections of
232 Th(p,F)(232 Th(n,F)) and238 U(p,F) (238 U(n,F)) reactions at En(p) = 1–200 MeV. Predominantly symmetric fission in232 Th(p,F) and roughly equal contributions of symmetric and asymmetric modes in238 U(n,F) at En(p) = 200 MeV as revealed by experimental branching ratios is reproduced. Steep transition from asymmetric to symmetric fission with increase of nucleon incident energy is due to fission of neutron-deficient Th(Pa) (A<229) nuclei, since about 20 neutron-deficient nuclides might contribute to the fission reaction at En(p) ∼200 MeV. A structure of the potential energy surface (a drop of symmetric and asymmetric fission barriers difference (ESYM f -EASYM f ) from ∼3.5 MeV to ∼1 MeV) of N-deficient Pa nuclides (A<226) and available phase space at outer fission saddles, are shown to be responsible for the sharp increase with Bn(p) of the symmetric fission component contribution for Th(p,F) and232 Th(n,F) reactions. That is a strong evidence of emissive fission nature of higly excited actinides, reliably quantified only up to En(p ∼20(30) MeV. In case of U nucleon-induced fission the much lower yield of the symmetric fission mode at En(p) <=200 MeV is due to much lower contribution of neutron-deficient U(Np)nuclides, which may split symmetrically. [ABSTRACT FROM AUTHOR]- Published
- 2009
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