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Cropland ammonia (NH3) emission is a critical driver triggering haze pollution. Many agricultural policies were enforced in past four decades to improve nitrogen (N) use efficiency while maintaining crop yield. Inadvertant reductions of NH3 emissions, which may be induced by such policies, are not well evaluated. Here, we quantify the China’s cropland-NH3 emission change from 1980 to 2050 and its response to policy interventions, using a data-driven model and a survey-based dataset of the fertilization scheme. Cropland-NH3 emission in China doubled from 1.93 to 4.02 Tg NH3-N in period 1980-1996, and then decreased to 3.50 Tg NH3-N in 2017. The prevalence of four agricultural policies may avoid ~3.0 Tg NH3-N in 2017, mainly located in highly-fertilized areas. Optimization of fertilizer management and food consumption could mitigate three quarters of NH3 emission in 2050 and lower NH3 emission intensity (emission divided by crop production) close to the European Union and the United States. Our findings provide an evidence on the decoupling of cropland-NH3 from crop production in China, and suggest the need to achieve cropland-NH3 mitigation while sustaining crop yields in other developing economies.

Reducing ammonia (NH3) volatilization from croplands while satisfying the food demand is strategically required to mitigate haze pollution. However, the global pattern of NH3 volatilization remains uncertain, primarily because of the episodic nature of NH3 volatilization rates and the high variation of fertilization practices. Here, we improve a global estimate of crop specific NH3 emissions at a high spatial resolution using an updated data-driven model with a survey-based dataset of the fertilization scheme. Our estimate of the globally averaged volatilization rate (12.6% ± 2.1%) is in line with previous data-driven studies (13.7 ± 3.1%) but results in one-quarter lower emissions than process-based models (16.5 ± 3.1%). The associated global emissions are estimated at 14.4 ± 2.3 Tg N, with more than 50% of the total stemming from three stable crops or 12.2% of global harvested areas. Nearly three-quarters of global cropland-NH3 emissions could be reduced by improving fertilization schemes (right rate, right type, and right placement). A small proportion (20%) of global harvested areas, primarily located in China, India, and Pakistan, accounts for 64% of abatement potentials. Our findings provide a critical reference guide for the future abatement strategy design when considering locations and crop types.

Reliable detection and attribution of changes in nitrogen (N) runoff from croplands are essential for designing efficient, sustainable N management strategies for future. Despite the recognition that excess N runoff poses a risk of aquatic eutrophication, large-scale, spatially detailed N runoff trends and their drivers remain poorly understood in China. Based on data comprising 535 site-years from 100 sites across China's croplands, we developed a data-driven upscaling model and a new simplified attribution approach to detect and attribute N runoff trends during the period of 1990–2012. Our results show that N runoff has increased by 46% for rice paddy fields and 31% for upland areas since 1990. However, we acknowledge that the upscaling model is subject to large uncertainties (20% and 40% as coefficient of variation of N runoff, respectively). At national scale, increased fertilizer application was identified as the most likely driver of the N runoff trend, while decreased irrigation levels offset to some extent the impact of fertilization increases. In southern China, the increasing trend of upland N runoff can be attributed to the growth in N runoff rates. Our results suggested that increased SOM led to the N runoff rate growth for uplands, but led to a decline for rice paddy fields. In combination, these results imply that improving management approaches for both N fertilizer use and irrigation is urgently required for mitigating agricultural N runoff in China.

Measurement and monitoring are important for correct and efficient operation of a network, since these activities provide reliable information and accurate analysis for characterizing and troubleshooting a network’s performance. The focus of network measurement is to measure the volume and types of traffic on a particular network and to record the raw measurement results. The focus of network monitoring is to initiate measurement tasks, collect raw measurement results, and report aggregated outcomes. Network systems are continuously evolving: besides incremental change to accommodate new devices, more drastic changes occur to accommodate new applications, such as overlay-based content delivery networks. As a consequence, a network can experience significant increases in size and significant levels of long-range, coordinated, distributed activity; furthermore, heterogeneous network technologies, services and applications coexist and interact. Reliance upon traditional, point-to-point, ad hoc measurements to manage such networks is becoming increasingly tenuous. In particular, correlated, simultaneous 1-way measurements are needed, as is the ability to access measurement information stored throughout the network of interest. To address these new challenges, this dissertation proposes OverMon, a new paradigm for edge-to-edge network monitoring systems through the application of overlay techniques. Of particular interest, the problem of significant network overheads caused by normal overlay network techniques has been addressed by constructing overlay networks with topology awareness - the network topology information is derived from interior gateway protocol (IGP) traffic, i.e. OSPF traffic, thus eliminating all overlay maintenance network overhead. Through a prototype that uses overlays to initiate measurement tasks and to retrieve measurement results, systematic evaluation has been conducted to demonstrate the feasibility and functionality of OverMon. The measurement

Measurement and monitoring are important for correct and efficient operation of a network, since these activities provide reliable information and accurate analysis for characterizing and troubleshooting a network’s performance. The focus of network measurement is to measure the volume and types of traffic on a particular network and to record the raw measurement results. The focus of network monitoring is to initiate measurement tasks, collect raw measurement results, and report aggregated outcomes. Network systems are continuously evolving: besides incremental change to accommodate new devices, more drastic changes occur to accommodate new applications, such as overlay-based content delivery networks. As a consequence, a network can experience significant increases in size and significant levels of long-range, coordinated, distributed activity; furthermore, heterogeneous network technologies, services and applications coexist and interact. Reliance upon traditional, point-to-point, ad hoc measurements to manage such networks is becoming increasingly tenuous. In particular, correlated, simultaneous 1-way measurements are needed, as is the ability to access measurement information stored throughout the network of interest. To address these new challenges, this dissertation proposes OverMon, a new paradigm for edge-to-edge network monitoring systems through the application of overlay techniques. Of particular interest, the problem of significant network overheads caused by normal overlay network techniques has been addressed by constructing overlay networks with topology awareness - the network topology information is derived from interior gateway protocol (IGP) traffic, i.e. OSPF traffic, thus eliminating all overlay maintenance network overhead. Through a prototype that uses overlays to initiate measurement tasks and to retrieve measurement results, systematic evaluation has been conducted to demonstrate the feasibility and functionality of OverMon. The measurement

Measurement and monitoring are important for correct and efficient operation of a network, since these activities provide reliable information and accurate analysis for characterizing and troubleshooting a network’s performance. The focus of network measurement is to measure the volume and types of traffic on a particular network and to record the raw measurement results. The focus of network monitoring is to initiate measurement tasks, collect raw measurement results, and report aggregated outcomes. Network systems are continuously evolving: besides incremental change to accommodate new devices, more drastic changes occur to accommodate new applications, such as overlay-based content delivery networks. As a consequence, a network can experience significant increases in size and significant levels of long-range, coordinated, distributed activity; furthermore, heterogeneous network technologies, services and applications coexist and interact. Reliance upon traditional, point-to-point, ad hoc measurements to manage such networks is becoming increasingly tenuous. In particular, correlated, simultaneous 1-way measurements are needed, as is the ability to access measurement information stored throughout the network of interest. To address these new challenges, this dissertation proposes OverMon, a new paradigm for edge-to-edge network monitoring systems through the application of overlay techniques. Of particular interest, the problem of significant network overheads caused by normal overlay network techniques has been addressed by constructing overlay networks with topology awareness - the network topology information is derived from interior gateway protocol (IGP) traffic, i.e. OSPF traffic, thus eliminating all overlay maintenance network overhead. Through a prototype that uses overlays to initiate measurement tasks and to retrieve measurement results, systematic evaluation has been conducted to demonstrate the feasibility and functionality of OverMon. The measurement

Measurement and monitoring are important for correct and efficient operation of a network, since these activities provide reliable information and accurate analysis for characterizing and troubleshooting a network’s performance. The focus of network measurement is to measure the volume and types of traffic on a particular network and to record the raw measurement results. The focus of network monitoring is to initiate measurement tasks, collect raw measurement results, and report aggregated outcomes. Network systems are continuously evolving: besides incremental change to accommodate new devices, more drastic changes occur to accommodate new applications, such as overlay-based content delivery networks. As a consequence, a network can experience significant increases in size and significant levels of long-range, coordinated, distributed activity; furthermore, heterogeneous network technologies, services and applications coexist and interact. Reliance upon traditional, point-to-point, ad hoc measurements to manage such networks is becoming increasingly tenuous. In particular, correlated, simultaneous 1-way measurements are needed, as is the ability to access measurement information stored throughout the network of interest. To address these new challenges, this dissertation proposes OverMon, a new paradigm for edge-to-edge network monitoring systems through the application of overlay techniques. Of particular interest, the problem of significant network overheads caused by normal overlay network techniques has been addressed by constructing overlay networks with topology awareness - the network topology information is derived from interior gateway protocol (IGP) traffic, i.e. OSPF traffic, thus eliminating all overlay maintenance network overhead. Through a prototype that uses overlays to initiate measurement tasks and to retrieve measurement results, systematic evaluation has been conducted to demonstrate the feasibility and functionality of OverMon. The measurement