1. Quasicrystal Nanosheet/α-Fe2O3Heterostructure-Based Low Power NO2Sensors: Experimental and DFT Studies
- Author
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Kumar, Sumit, Hojamberdiev, Mirabbos, Chakraborty, Anyesha, Mitra, Rahul, Chaurasiya, Rajneesh, Kwoka, Monika, Tiwary, Chandra Sekhar, Biswas, Krishanu, and Kumar, Mahesh
- Abstract
Industrial emissions, environmental monitoring, and medical fields have put forward huge demands for high-performance and low power consumption sensors. Two-dimensional quasicrystal (2D QC) nanosheets of metallic multicomponent Al70Co10Fe5Ni10Cu5have emerged as a promising material for gas sensors due to their excellent catalytic and electronic properties. Herein, we demonstrate highly sensitive and selective NO2sensors developed by low-cost and scalable fabrication techniques using 2D QC nanosheets and α-Fe2O3nanoparticles. The sensitivity (ΔR/R%) of the optimal amount of 2D QC nanosheet-loaded α-Fe2O3sensor was 32%, which is significantly larger about 3.5 times than bare α-Fe2O3sensors for 1 ppm of NO2at 150 °C operating temperature. The sensors exhibited p-type conduction, and resistance was reduced when exposed to NO2, an oxidizing gas. The enhanced sensing characteristics are a result of the formation of nanoheterojunctions between 2D QC and α-Fe2O3, which improved the charge transport and provided a large sensing signal. In addition, the heterojunction sensor demonstrated excellent NO2selectivity over other oxidizing and reducing gases. Furthermore, density functional theory calculation examines the adsorption energy and charge transfer between NO2molecules on the α-Fe2O3(110) and QC/α-Fe2O3(110) heterostructure surfaces, which coincides well with the experimental results.
- Published
- 2024
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