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With the proliferation of non-linear loads and distributed power resources that connect through power electronic equipment, decentralized harmonic pollution in three-phase symmetric power system becomes increasingly serious. Despite this, monitoring the current harmonic of all substation feeders regardless of cost is unrealistic. To this end, a multi-source data driven method is proposed in this paper, utilizing data from the power quality monitoring system, dispatching system, and market business system, to estimate the harmonic spectrum of substation feeder currents and estimate the harmonic current components of each feeder with monitoring data of bus voltage harmonics and line harmonic currents. The objective function of the harmonic spectrum estimation model is constructed based on the analysis of current harmonic phasor and power relationship on the feeders. An improved particle swarm optimization (PSO) algorithm is proposed to solve the proposed estimation model thereby obtaining the current harmonic content of each feeder and the phase angle difference between the current harmonics of the feeders. The performance of the proposed model and algorithm is validated by numerical simulation with a test system and an actual system.