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Coherent supercontinuum radiation in the extreme-ultraviolet (XUV) range is indispensable for synthesizing attosecond light pulses and for exploring transient atomic structures. Here, we report the striking observations of coherent XUV supercontinuum (XSC) extended from below to far above the ionization threshold, which exhibits completely different temporal and spatial properties comparing to the conventional rescattering induced high harmonic generation (HHG). We demonstrate that the strong-field created coherence among bound orbitals strongly distort the atomic transition energies during the pulse, leading to coherent emission spanning tens of electron-volts, in contrast to the line emission via free-induction decay occurring after the pulse. The supposed non-radiating bound dark states contribute as well by emitting dressed energy through dark-to-bright emission mechanism. All the processes modulated at sub-cycle time scale jointly form this new-type coherent XSC. This work achieves the strong-field attosecond control of the exotic atomic radiation dynamics and provides the means of simultaneous generation of separated attosecond sources, i.e., XSC and HHG, with potential advancing attosecond interferometry.

The coupled electronic-vibrational dynamics of nitrogen ions induced by strong-field ionization is investigated theoretically to corroborate the recent transient X-ray K-edge absorption experiment [PRL 129, 123002 (2022)], where the population distribution of three electronic states in air lasing of N2+ was determined for the first time. By extending the ionization-coupling model to include the transient absorption, we successfully reproduce the time-resolved X-ray absorption spectra of nitrogen ions observed in the experiment. By identifying the contributions from different electronic states, the study provides different interpretation revealing the significant role of excited state A arising from the strong coupling between vibrational states in strong laser fields. It indicates that the electronic population inversion occurs at least for certain alignment of nitrogen molecules. The theory helps uncovering new features of absorption from forbidden transitions during ionization and confirming that the vibration coherence at each electronic channel induces the modulation of absorbance after strong field ionization. A new scheme is proposed to determine the population transfer at different probing geometry to avoid the spectral overlap. This work offers valuable insights into the intricate interplay between electronic and vibrational dynamics and helps to resolve the debate on nitrogen air lasing.

We study the generation of terahertz radiation from atoms and molecules driven by an ultrashort fundamental laser and its second harmonic field by solving time-dependent Schr\"odinger equation (TDSE). The comparisons between one-, two-, and three- dimensional TDSE numerical simulations show that initial ionized wave-packet and its subsequent acceleration in the laser field and rescattering with long-range Coulomb potential play key roles. We also present the dependence of the optimum phase delay and yield of terahertz radiation on the laser intensity, wavelength, duration, and the ratio of two-color laser components. Terahertz wave generation from model hydrogen molecules are further investigated by comparing with high harmonic emission. It is found that the terahertz yield is following the alignment dependence of ionization rate, while the optimal two-color phase delays varies by a small amount when the alignment angle changes from 0 to 90 degrees, which reflects alignment dependence of attosecond electron dynamics. Finally we show that terahertz emission might be used to clarify the origin of interference in high harmonic generation from aligned molecules by coincidently measuring the angle-resolved THz yields.