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Sizable hyperpolarisation, i.e. an imbalance of the occupation numbers of nuclear spins in a sample deviating from thermal equilibrium, is needed in various fields of science. For example, hyperpolarised tracers are utilised in magnetic resonance imaging in medicine (MRI) and polarised beams and targets are employed in nuclear physics to study the spin dependence of nuclear forces. Here we show that the quantum interference of transitions induced by radio-wave pumping with longitudinal and radial pulses are able to produce large polarisations at small magnetic fields. This method is easier than established methods, theoretically understood and experimentally proven for beams of metastable hydrogen atoms in the keV energy range. It should also work for a variety of samples at rest. Thus, this technique opens the door for a new generation of polarised tracers, possibly low-field MRI with better spatial resolution or the production of polarised fuel to increase the efficiency of fusion reactors by manipulating the involved cross sections., Comment: 22 pages, 9 figures, splitted into two parts: main paper and methods

The origin of quantum physics was the discovery of the base unit of electromagnetic action $h$ by Max Planck in 1900 when he analyzed the experimental results of the black body radiation. This permitted Albert Einstein a few years later to explain the photoelectric effect by the absorption of photons with an energy of $E = h \cdot f$. We exploit the Planck-Einstein relation in a new type of fundamental spectroscopic measurements of direct transitions between two states with energy differences of about 10 neV and induced frequencies of a few MHz. Employing a Lamb-shift polarimeter and a Sona transition unit, featuring a relatively simple magnetic field configuration of two opposing solenoidal coils, we were able to determine $f$ and measure $E$ independently. Only resonances corresponding to integer multiples of Planck's constant $h$ were observed in our setup, which can very well be explained quantitatively by the Schr\"odinger equation. This new method beautifully demonstrates the quantization in the micro-cosmos and allows one to measure the hyperfine splitting energies between the substates with $F=1$ and $m_F = -1, 0, +1$ of metastable hydrogen atoms as function of a magnetic field and, thus, to investigate the influence of QED corrections on the Breit-Rabi diagram.

Polarized atomic beam sources have been in operation since many years to produce either nuclear polarized atomic hydrogen or deuterium beams. In recent experiments such a source was used to polarize both isotopes independently at the same time. By recombination of the atoms, HD molecules with all possible nuclear spin combinations can be created. Those spin isomers are useful for further applications like precision spectroscopy, as polarized targets for laser-particle acceleration, polarized fuel for fusion reactors or as an option for future measurements of electric dipole moments., Comment: to be published in Physical Review Letters