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The change in raindrop spectrum characteristics is an important factor affecting the accuracy of estimations of precipitation. The in-depth study of raindrop spectrum characteristics is of great interest for understanding precipitation process and improving quantitative radar precipitation estimation. In this paper, the raindrop size distributions at Longli (57913), Puding (57808) and Luodian (57916) stations in Guizhou were analyzed from the perspective of precipitation microphysical characteristics. The results showed that the raindrop size distribution was different among different regions. The correlation coefficients of the mass-weighted average diameter for the rain intensities at these three stations were 46.89%, 49.51%, and 47.03%, respectively, which were slightly lower than the normal correlation coefficients of the average volume diameter for the rain intensities: 67.80%, 71.28%, and 71.46%, respectively. Based on the data from the Guiyang weather radar, raindrop spectrometer, and automatic rain gauge, the dynamic Z-I relationship method and the LSTM neural network method were used to estimate precipitation. The correlation coefficients of the dynamic Z-I relationship method and the LSTM neural network method at the three stations studied were 0.8432, 0.7763, and 0.8658 and 0.8745, 0.9125, and 0.8676, respectively. Regarding the process of stratiform cloud precipitation, the correlation coefficients of the dynamic Z-I relationship method and LSTM neural network method at the three stations were 0.6933, 0.0902, and 0.1409 and 0.7114, 0.4984, and 0.4902, respectively. In the estimation of cumulative precipitation for 45 days from 1 July to 16 August 2020, the relative errors of the neural network estimation at the three stations were −4.25%, −11.35%, and −8.68% and the relative errors of the dynamic Z-I relationship estimation were −2.68%, −7.41%, and −21.23%, respectively. The final relative error of the neural network was slightly worse than that of the dynamic Z-I relationship in the cumulative precipitation estimations of Longli station and Puding station, but the overall correlation coefficients of the LSTM neural network method were better than those of the dynamic Z-I relationship method. [ABSTRACT FROM AUTHOR]