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In this work we present a novel technique, based on a trust-region optimization algorithm and second-order trajectory sensitivities, to compute the extreme trajectories of power system dynamic simulations given a bounded set that represents parametric uncertainty. We show how this method, while remaining computationally efficient compared with sampling-based techniques, overcomes the limitations of previous sensitivity-based techniques to approximate the bounds of the trajectories when the local approximation loses validity because of the nonlinearity. We present several numerical experiments that showcase the accuracy and scalability of the technique, including a demonstration on the IEEE New England test system. [ABSTRACT FROM AUTHOR]