Search

We present a search for neutrinoless double-beta ($0\nu\beta\beta$) decay of $^{136}$Xe using the full KamLAND-Zen 800 dataset with 745 kg of enriched xenon, corresponding to an exposure of $2.097$ ton yr of $^{136}$Xe. This updated search benefits from a more than twofold increase in exposure, recovery of photo-sensor gain, and reduced background from muon-induced spallation of xenon. Combining with the search in the previous KamLAND-Zen phase, we obtain a lower limit for the $0\nu\beta\beta$ decay half-life of $T_{1/2}^{0\nu} > 3.8 \times 10^{26}$ yr at 90% C.L., a factor of 1.7 improvement over the previous limit. The corresponding upper limits on the effective Majorana neutrino mass are in the range 28-122 meV using phenomenological nuclear matrix element calculations., Comment: arXiv admin note: text overlap with arXiv:2203.02139

We conducted measurements of $K^- + {^3{\rm He}} \to \pi \!Y \!N + N'$ reactions using a $1~{\rm GeV}/c$ $K^-$-beam, with the objective of understanding the broad decay width of $\bar{K} \!N \!N$ (approximately twice as broad as that of $\Lambda(1405)$ considered to be the $\bar{K} \!N$ quasi-bound state). We successfully reproduced distributions of the $\pi \! Y \! N$ invariant mass and momentum transfer for $\pi \! Y \! N$ using model fitting functions for $\bar{K} \!N \!N$ formation and quasi-free $\bar{K}$ absorption (${\rm QF}_{\bar{K}-{\rm abs}}$) processes. The model can describe the experimental data quite well, and four $\bar{K} \! N \! N \to \pi \! Y \! N $ cross-sections were obtained. The results indicate that mesonic decay is the dominant decay branch of $\bar{K} \! N \! N$. The results also suggest that $\Gamma_{\pi \Lambda N} \sim \Gamma_{\pi \Sigma N}$, which indicates that the $I_{\bar{K} \! N}=1$ absorption channel, in addition to the $I_{\bar{K} \! N}=0$ absorption channel, substantially contribute to the $\bar{K} \! N \! N$ decay, making the $\bar{K} \! N \! N$ state approximately twice as unstable as $\Lambda$(1405).

The existence of cosmic dark matter and neutrino properties are long-standing problems in cosmology and particle physics. These problems have been investigated by using radiation detectors. We will discuss the application of inorganic crystal scintillators to studies on dark matter and neutrino properties. A large volume and high-purity inorganic crystal is a promising detector for investigating dark matter and neutrino.

Radiation measurement relies on pulse detection, which can be performed using various configurations of high-speed analog-to-digital converters (ADCs) and field-programmable gate arrays (FPGAs). For optimal power consumption, design simplicity, system flexibility, and the availability of DSP slices, we consider the Radio Frequency System-on-Chip (RFSoC) to be a more suitable option than traditional setups. To this end, we have developed custom RFSoC-based electronics and verified its feasibility. The ADCs on RFSoC exhibit a flat frequency response of 1-125 MHz. The root-mean-square (RMS) noise level is 2.1 ADC without any digital signal processing. The digital signal processing improves the RMS noise level to 0.8 ADC (input equivalent 40 Vrms). Baseline correction via digital signal processing can effectively prevent photomultiplier overshoot after a large pulse. Crosstalk between all channels is less than -55 dB. The measured data transfer speed can support up to 32 kHz trigger rates (corresponding to 750 Mbps). Overall, our RFSoC-based electronics are highly suitable for pulse detection, and after some modifications, they will be employed in the Kamioka Liquid Scintillator Anti-Neutrino Detector (KamLAND)., Comment: 14 pages, 13 figures

Particle dark matter could belong to a multiplet that includes an electrically charged state. WIMP dark matter ($\chi^{0}$) accompanied by a negatively charged excited state ($\chi^{-}$) with a small mass difference (e.g. $<$ 20 MeV) can form a bound-state with a nucleus such as xenon. This bound-state formation is rare and the released energy is $\mathcal{O}(1-10$) MeV depending on the nucleus, making large liquid scintillator detectors suitable for detection. We searched for bound-state formation events with xenon in two experimental phases of the KamLAND-Zen experiment, a xenon-doped liquid scintillator detector. No statistically significant events were observed. For a benchmark parameter set of WIMP mass $m_{\chi^{0}} = 1$ TeV and mass difference $\Delta m = 17$ MeV, we set the most stringent upper limits on the recombination cross section times velocity $\langle\sigma v\rangle$ and the decay-width of $\chi^{-}$ to $9.2 \times 10^{-30}$ ${\rm cm^3/s}$ and $8.7 \times 10^{-14}$ GeV, respectively at 90% confidence level.

The dark matter observation claim by the DAMA/LIBRA collaboration has been a long-standing puzzle within the particle physics community. Efforts of other research groups to verify the claim have been insufficient by significant radioactivity of present NaI(Tl) crystals. PICOLON (Pure Inorganic Crystal Observatory for LOw-energy Neut(ra)lino) experiment conducts independent search for Weakly Interacting Massive Particles (WIMPs) using NaI(Tl) crystals. Our NaI(Tl) crystal manufactured in 2020 (Ingot #85) reached the same purity level as DAMA/LIBRA crystals. In this report, we describe the radiopurity of the new Ingot #94 crystal produced using the same purification technique as Ingot #85. The $\alpha$-ray events were selected by pulse-shape discrimination method. The impurities in the Ingot #94, $^{232}$Th, $^{226}$Ra and $^{210}$Po radioactivity were $4.6\pm 1.2~\mathrm{\mu Bq/kg}$, $7.9\pm 4.4~\mathrm{\mu Bq/kg}$, and $19\pm 6~\mathrm{\mu Bq/kg}$, which are equivalent to those of the DAMA/LIBRA crystals. The background rate in the energy region of 2-6 keV , was 2-5 events/d/kg/keV without applying a veto trigger., Comment: 14pages, 16 figures

While supervised neural networks have become state of the art for identifying the rare strong gravitational lenses from large imaging data sets, their selection remains significantly affected by the large number and diversity of nonlens contaminants. This work evaluates and compares systematically the performance of neural networks in order to move towards a rapid selection of galaxy-scale strong lenses with minimal human input in the era of deep, wide-scale surveys. We used multiband images from PDR2 of the HSC Wide survey to build test sets mimicking an actual classification experiment, with 189 strong lenses previously found over the HSC footprint and 70,910 nonlens galaxies in COSMOS. Multiple networks were trained on different sets of realistic strong-lens simulations and nonlens galaxies, with various architectures and data pre-processing. The overall performances strongly depend on the construction of the ground-truth training data and they typically, but not systematically, improve using our baseline residual network architecture. Improvements are found when applying random shifts to the image centroids and square root stretches to the pixel values, adding z band, or using random viewpoints of the original images, but not when adding difference images to subtract emission from the central galaxy. The most significant gain is obtained with committees of networks trained on different data sets, and showing a moderate overlap between populations of false positives. Nearly-perfect invariance to image quality can be achieved by training networks either with large number of bands, or jointly with the PSF and science frames. Overall, we show the possibility to reach a TPR0 as high as 60% for the test sets under consideration, which opens promising perspectives for pure selection of strong lenses without human input using the Rubin Observatory and other forthcoming ground-based surveys., Comment: 21 pages, 10 figures, submitted to A&A, comments are welcome

We present a new measurement of the $^4_\Lambda$H hypernuclear lifetime using in-flight $K^-$ + $^4$He $\rightarrow$ $^4_\Lambda$H + $\pi^0$ reaction at the J-PARC hadron facility. We demonstrate, for the first time, the effective selection of the hypernuclear bound state using only the $\gamma$-ray energy decayed from $\pi^0$. This opens the possibility for a systematic study of isospin partner hypernuclei through comparison with data from ($K^-$, $\pi^-$) reaction. As the first application of this method, our result for the $^4_\Lambda$H lifetime, $\tau(^4_\Lambda \mathrm{H}) = 206 \pm 8 (\mathrm{stat.}) \pm 12 (\mathrm{syst.})\ \mathrm{ps}$, is one of the most precise measurements to date. We are also preparing to measure the lifetime of the hypertriton ($^3_\Lambda$H) using the same setup in the near future.

Cosmic-ray muons produce various radioisotopes when passing through material. These spallation products can be backgrounds for rare event searches such as in solar neutrino, double-beta decay, and dark matter search experiments. The KamLAND-Zen experiment searches for neutrinoless double-beta decay in 745kg of xenon dissolved in liquid scintillator. The experiment includes dead-time-free electronics with a high efficiency for detecting muon-induced neutrons. The production yields of different radioisotopes are measured with a combination of delayed coincidence techniques, newly developed muon reconstruction and xenon spallation identification methods. The observed xenon spallation products are consistent with results from the FLUKA and Geant4 simulation codes.

This White Paper, prepared for the Fundamental Symmetries, Neutrons, and Neutrinos Town Meeting related to the 2023 Nuclear Physics Long Range Plan, makes the case for double beta decay as a critical component of the future nuclear physics program. The major experimental collaborations and many theorists have endorsed this white paper., Comment: white paper submitted for the Fundamental Symmetries, Neutrons, and Neutrinos Town Meeting in support of the US Nuclear Physics Long Range Planning Process

We report a measurement of the strange axial coupling constant $g_A^s$ using atmospheric neutrino data at KamLAND. This constant is a component of the axial form factor of the neutral-current quasielastic (NCQE) interaction. The value of $g_A^s$ significantly changes the ratio of proton and neutron NCQE cross sections. KamLAND is suitable for measuring NCQE interactions as it can detect nucleon recoils with low-energy thresholds and measure neutron multiplicity with high efficiency. KamLAND data, including the information on neutron multiplicity associated with the NCQE interactions, makes it possible to measure $g_A^s$ with a suppressed dependence on the axial mass $M_A$, which has not yet been determined. For a comprehensive prediction of the neutron emission associated with neutrino interactions, we establish a simulation of particle emission via nuclear deexcitation of $^{12}$C, a process not considered in existing neutrino Monte Carlo event generators. Energy spectrum fitting for each neutron multiplicity gives $g_A^s =-0.14^{+0.25}_{-0.26}$, which is the most stringent limit obtained using NCQE interactions without $M_A$ constraints. The two-body current contribution considered in this analysis relies on a theoretically effective model and electron scattering experiments and requires future verification by direct measurements and future model improvement.

We measured a set of $\pi^\pm\Sigma^\mp$, $\pi^0\Sigma^0$, and $\pi^-\Sigma^0$ invariant mass spectra below and above the $\bar{K}N$ mass threshold in $K^-$-induced reactions on deuteron. We deduced the $S$-wave $\bar{K}N\rightarrow\pi\Sigma$ and $\bar{K}N\rightarrow\bar{K}N$ scattering amplitudes in the isospin 0 channel in the framework of a $\bar{K}N$ and $\pi\Sigma$ coupled channel. We find that a resonance pole corresponding to $\Lambda(1405)$ is located at 1417.7$^{+6.0}_{-7.4}$(fitting errors)$^{+1.1}_{-1.0}$(systematic errors) + $[-26.1^{+6.0}_{-7.9}$(fitting errors)$^{+1.7}_{-2.0}$(systematic errors)]$i$ MeV/$c^2$, closer to the $\bar{K}N$ mass threshold than the value determined by the Particle Data Group., Comment: 8 pages, 5 figures

The decay of the primordial isotopes $^{238}\mathrm{U}$, $^{235}\mathrm{U}$, $^{232}\mathrm{Th}$, and $^{40}\mathrm{K}$ have contributed to the terrestrial heat budget throughout the Earth's history. Hence the individual abundance of those isotopes are key parameters in reconstructing contemporary Earth model. The geoneutrinos produced by the radioactive decays of uranium and thorium have been observed with the Kamioka Liquid-Scintillator Antineutrino Detector (KamLAND). Those measurements have been improved with more than 18-year observation time, and improvements in detector background levels mainly by an 8-year almost rector-free period now permit spectroscopy with geoneutrinos. Our results yield the first constraint on both uranium and thorium heat contributions. Herein the KamLAND result is consistent with geochemical estimations based on elemental abundances of chondritic meteorites and mantle peridotites. The High-Q model is disfavored at 99.76% C.L. and a fully radiogenic model is excluded at 5.2$\sigma$ assuming a homogeneous heat producing element distribution in the mantle., Comment: 13 pages, 2 figures, accepted for publication in Geophysical Research Letters on Aug 4th, 2022

We present the results of a search for core-collapse supernova neutrinos, using long-term KamLAND data from 2002 March 9 to 2020 April 25. We focus on the electron antineutrinos emitted from supernovae in the energy range of 1.8--111 MeV. Supernovae will make a neutrino event cluster with the duration of $\sim$10 s in the KamLAND data. We find no neutrino clusters and give the upper limit on the supernova rate as to be 0.15 yr$^{-1}$ with a 90% confidence level. The detectable range, which corresponds to a >95% detection probability, is 40--59 kpc and 65--81 kpc for core-collapse supernovae and failed core-collapse supernovae, respectively. This paper proposes to convert the supernova rate obtained by the neutrino observation to the Galactic star formation rate. Assuming a modified Salpeter-type initial mass function, the upper limit on the Galactic star formation rate is <(17.5--22.7) $M_{\odot} \mathrm{yr}^{-1}$ with a 90% confidence level., Comment: 10 pages, 4 figures, accepted for publication in Astrophysical Journal

The effect of pressure ($P$) on magnetic susceptibility of CsCuCl$_3$ was examined in magnetic fields ($\rm \mu_0$$H$) of up to 51 T using a proximity detector oscillator (PDO), and the $H$-$P$ phase diagram of CsCuCl$_3$ was constructed over the saturation field ($H_{\rm sat}$). We found that, with increasing $P$, $H_{\rm sat}$ increases and the uud-phase that appeared at $P$ = 0.7 GPa widened. Based on comparison between the experimental and calculated $H$-$P$ phase diagrams, the Y-phase was predicted to appear above 1.7 GPa. The interchain antiferromagnetic exchange interaction in the $ab$-plane was evaluated and found to increase with increasing $P$, which is consistent with a previous study under high pressure [D. Yamamoto {\it et al.}, Nat. Commun. {\bf 12}, 4263 (2021).]. Moreover, an anomaly was observed below $P$ = 0.6 GPa just below $H_{\rm sat}$ and might be a new phase transition derived from nonlinear response caused by the PDO technique., Comment: 14 pages, 7 figures

The KamLAND-Zen experiment has provided stringent constraints on the neutrinoless double-beta ($0\nu\beta\beta$) decay half-life in $^{136}$Xe using a xenon-loaded liquid scintillator. We report an improved search using an upgraded detector with almost double the amount of xenon and an ultralow radioactivity container, corresponding to an exposure of 970 kg yr of $^{136}$Xe. These new data provide valuable insight into backgrounds, especially from cosmic muon spallation of xenon, and have required the use of novel background rejection techniques. We obtain a lower limit for the $0\nu\beta\beta$ decay half-life of $T_{1/2}^{0\nu} > 2.3 \times 10^{26}$ yr at 90% C.L., corresponding to upper limits on the effective Majorana neutrino mass of 36-156 meV using commonly adopted nuclear matrix element calculations., Comment: 7 pages, 3 figures

We report the results of a search for MeV-scale astrophysical neutrinos in KamLAND presented as an excess in the number of coincident neutrino interactions associated with the publicly available high-energy neutrino datasets from the IceCube Neutrino Observatory. We find no statistically significant excess in the number of observed low-energy electron antineutrinos in KamLAND, given a coincidence time window of $\pm$500s, $\pm$1,000s, $\pm$3,600s, and $\pm$10,000s around each of the IceCube neutrinos. We use this observation to present limits from 1.8 MeV to 100 MeV on the electron antineutrino fluence, assuming a mono-energetic flux. We then compare the results to several astrophysical measurements performed by IceCube and place a limit at the 90% confidence level on the electron antineutrino isotropic thermal luminosity from the TXS 0506+056 blazar., Comment: 12 pages, 5 figures

PICOLON (Pure Inorganic Crystal Observatory for LOw-energy Neutr(al)ino) aims to search for cosmic dark matter by high purity NaI(Tl) scintillator. We developed extremely pure NaI(Tl) crystal by hybrid purification method. The recent result of $^{210}$Pb in our NaI(Tl) is less than 5.7 $\mu$Bq/kg. We will report the test experiment in the low-background measurement at Kamioka Underground Laboratory. The sensitivity for annual modulating signals and finding dark matter particles will be discussed., Comment: To be published in the Proceedings of TAUP2021. (Journal of Physics: Conference Series (JPCS),)

We present the results of a time-coincident event search for low-energy electron antineutrinos in the KamLAND detector with gamma-ray bursts from the Gamma-ray Coordinates Network and Fermi Gamma-ray Burst Monitor. Using a variable coincidence time window of $\pm$500s plus the duration of each gamma-ray burst, no statistically significant excess above background is observed. We place the world's most stringent 90% confidence level upper limit on the electron antineutrino fluence below 17.5 MeV. Assuming a Fermi-Dirac neutrino energy spectrum from the gamma-ray burst source, we use the available redshift data to constrain the electron antineutrino luminosity and effective temperature., Comment: 9 pages, 3 figures

$\bar K$-nuclear bound systems, kaonic nuclei, have been widely discussed as products of the strongly attractive $\bar K N$ interaction in $I = 0$ channels. Recently, we demonstrated that kaonic nuclei can be produced via in-flight $(K^-,N)$ reactions using the low-momentum DC kaon beam at the J-PARC E15 experiment. We observed the simplest kaonic nuclei, $K^-pp$, having a much deeper binding energy than normal nuclei. For further studies, we have proposed a series of experimental programs for the systematic investigation of light kaonic nuclei, from $\bar K N$ ($\Lambda(1405)$) to $\bar K NNNN$. In the new experiment approved as J-PARC E80, we will measure the $\bar K NNN$ ($A=3$) system as a first step toward a comprehensive study., Comment: 10 pages, 5 figures, proceedings of the 8th Asia-Pacific Conference on Few-Body Problems in Physics (APFB2020), accepted for publication in Fwe-Body Systems

We report on a search for electron antineutrinos ($\bar{\nu}_e$) from astrophysical sources in the neutrino energy range 8.3 to 30.8 MeV with the KamLAND detector. In an exposure of 6.72 kton-year of the liquid scintillator, we observe 18 candidate events via the inverse beta decay reaction. Although there is a large background uncertainty from neutral current atmospheric neutrino interactions, we find no significant excess over background model predictions. Assuming several supernova relic neutrino spectra, we give upper flux limits of 60--110 cm$^{-2}$ s$^{-1}$ (90% CL) in the analysis range and present a model-independent flux. We also set limits on the annihilation rates for light dark matter pairs to neutrino pairs. These data improves on the upper probability limit of $^{8}$B solar neutrinos converting into $\bar{\nu}_e$'s, $P_{\nu_e \rightarrow \bar{\nu}_e} < 3.5\times10^{-5}$ (90% CL) assuming an undistorted $\bar{\nu}_e$ shape. This corresponds to a solar $\bar{\nu}_e$ flux of 60 cm$^{-2}$ s$^{-1}$ (90% CL) in the analysis energy range., Comment: 21 pages, 9 figures, 4 tables, accepted for publication in Astrophysical Journal

We have carried out a systematic search for galaxy-scale strong lenses in multiband imaging from the Hyper Suprime-Cam (HSC) survey. Our automated pipeline, based on realistic strong-lens simulations, deep neural network classification, and visual inspection, is aimed at efficiently selecting systems with wide image separations (Einstein radii ~1.0-3.0"), intermediate redshift lenses (z ~ 0.4-0.7), and bright arcs for galaxy evolution and cosmology. We classified gri images of all 62.5 million galaxies in HSC Wide with i-band Kron radius >0.8" to avoid strict pre-selections and to prepare for the upcoming era of deep, wide-scale imaging surveys with Euclid and Rubin Observatory. We obtained 206 newly-discovered candidates classified as definite or probable lenses with either spatially-resolved multiple images or extended, distorted arcs. In addition, we found 88 high-quality candidates that were assigned lower confidence in previous HSC searches, and we recovered 173 known systems in the literature. These results demonstrate that, aided by limited human input, deep learning pipelines with false positive rates as low as ~0.01% can be very powerful tools for identifying the rare strong lenses from large catalogs, and can also largely extend the samples found by traditional algorithms. We provide a ranked list of candidates for future spectroscopic confirmation., Comment: 5 pages and 4 figures (plus appendix), version published in A&A

A dark matter search project needs and extremely low background radiation detector since the expected event rate of dark matter is less than a few events in one year in one tonne of the detector mass. The authors developed a highly radiopure NaI(Tl) crystal to search for dark matter. The best combination of the purification methods was developed, resulting $^{\mathrm{nat}}$K and $^{210}$Pb were less than 20 ppb and 5.7 $\mu$Bq/kg, respectively. The authors will construct a large volume detector system with high-purity NaI(Tl) crystals. The design and the performance of the prototype detector module will be reported in this article., Comment: 12 pages, 7 figures, RADIATION DETECTORS AND THEIR USES Proceedings of the 35th Workshop on Radiation Detectors and Their Uses in KEK

We report the result of a search for neutrinos in coincidence with solar flares from the GOES flare database. The search was performed on a 10.8 kton-year exposure of KamLAND collected from 2002 to 2019. This large exposure allows us to explore previously unconstrained parameter space for solar flare neutrinos. We found no statistical excess of neutrinos and established 90% confidence level upper limits of $8.4 \times 10^7$ cm$^{-2}$ ($3.0 \times 10^{9}$ cm$^{-2}$) on electron anti-neutrino (electron neutrino) fluence at 20 MeV normalized to the X12 flare, assuming that the neutrino fluence is proportional to the X-ray intensity., Comment: 13 pages, 9 figures, accepted October 27, 2021

The KamLAND-Zen 800 experiment is searching for the neutrinoless double-beta decay of $^{136}$Xe by using $^{136}$Xe-loaded liquid scintillator. The liquid scintillator is enclosed inside a balloon made of thin, transparent, low-radioactivity film that we call Inner Balloon (IB). The IB, apart from guaranteeing the liquid containment, also allows to minimize the background from cosmogenic muon-spallation products and $^{8}$B solar neutrinos. Indeed these events could contribute to the total counts in the region of interest around the Q-value of the double-beta decay of $^{136}$Xe. In this paper, we present an overview of the IB and describe the various steps of its commissioning minimizing the radioactive contaminations, from the material selection, to the fabrication of the balloon and its installation inside the KamLAND detector. Finally, we show the impact of the IB on the KamLAND background as measured by the KamLAND detector itself., Comment: 23 pages, 16 figures, to be submitted to JINST

There are many theories where a dark matter particle is part of a multiplet with an electrically charged state. If WIMP dark matter ($\chi^{0}$) is accompanied by a charged excited state ($\chi^{-}$) separated by a small mass difference, it can form a stable bound state with a nucleus. In supersymmetric models, the $\chi^{0}$ and the $\chi^{-}$ could be the neutralino and a charged slepton, such as the neutralino-stau degenerate model. The formation binding process is expected to result in an energy deposition of {\it O}(1--10 MeV), making it suitable for detection in large liquid scintillator detectors. We describe new constraints on the bound state formation with a xenon nucleus using the KamLAND-Zen 400 Phase-II dataset. In order to enlarge the searchable parameter space, all xenon isotopes in the detector were used. For a benchmark parameter set of $m_{\chi^{0}} = 100$ GeV and $\Delta m = 10$ MeV, this study sets the most stringent upper limits on the recombination cross section $\langle\sigma v\rangle$ and the decay-width of $\chi^{-}$ of $2.0 \times 10^{-31}$ ${\rm cm^3/s}$ and $1.1 \times 10^{-18}$ GeV, respectively (90\% confidence level).

Core-collapse supernovae are among the most magnificent events in the observable universe. They produce many of the chemical elements necessary for life to exist and their remnants -- neutron stars and black holes -- are interesting astrophysical objects in their own right. However, despite millennia of observations and almost a century of astrophysical study, the explosion mechanism of core-collapse supernovae is not yet well understood. Hyper-Kamiokande is a next-generation neutrino detector that will be able to observe the neutrino flux from the next galactic core-collapse supernova in unprecedented detail. We focus on the first 500 ms of the neutrino burst, corresponding to the accretion phase, and use a newly-developed, high-precision supernova event generator to simulate Hyper-Kamiokande's response to five different supernova models. We show that Hyper-Kamiokande will be able to distinguish between these models with high accuracy for a supernova at a distance of up to 100 kpc. Once the next galactic supernova happens, this ability will be a powerful tool for guiding simulations towards a precise reproduction of the explosion mechanism observed in nature., Comment: 21 pages, 7 figures. Article based on thesis published as arXiv:2002.01649. v2: added references and some explanations in response to reviewer comments

The highly radiopure NaI(Tl) was developed to search for particle candidates of dark matter. The optimized methods were combined to reduce various radioactive impurities. The $^{40}$K was effectively reduced by the re-crystallization method. The progenies of the decay chains of uranium and thorium were reduced by appropriate resins. The concentration of natural potassium in NaI(Tl) crystal was reduced down to 20 ppb. Concentrations of alpha-ray emitters were successfully reduced by appropriate selection of resin. The present concentration of thorium series and 226Ra were $1.2 \pm1.4$ $\mu$Bq/kg and $13\pm4$ $\mu$Bq/kg, respectively. No significant excess in the concentration of $^{210}$Pb was obtained, and the upper limit was 5.7 $\mu$Bq/kg at 90% C. L. The achieved level of radiopurity of NaI(Tl) crystals makes construction of a dark matter detector possible., Comment: 11 pages, 6 figures, accepted to Progress of Theoretical and Experimental Physics

We present the results of a search for MeV-scale electron antineutrino events in KamLAND in coincident with the 60 gravitational wave events/candidates reported by the LIGO/Virgo collaboration during their second and third observing runs. We find no significant coincident signals within a $\pm$ 500 s timing window from each gravitational wave and present 90% C.L. upper limits on the electron antineutrino fluence between $10^{8}$-$10^{13}\,{\mathrm cm^2}$ for neutrino energies in the energy range of 1.8-111 MeV., Comment: 11 pages, 2 figures, 2 tables, Accepted for publication in ApJ

We have performed an exclusive measurement of the $K^{-}+\! ~^{3}{\rm He} \to \Lambda pn$ reaction at an incident kaon momentum of $1\ {\rm GeV}/c$.In the $\Lambda p$ invariant mass spectrum, a clear peak was observed below the mass threshold of $\bar{K}\!+\!N\!+\!N$, as a signal of the kaonic nuclear bound state, $\bar{K}NN$.The binding energy, decay width, and $S$-wave Gaussian reaction form-factor of this state were observed to be $B_{K} = 42\pm3({\rm stat.})^{+3}_{-4}({\rm syst.})\ {\rm MeV}$, $\Gamma_{K} = 100\pm7({\rm stat.})^{+19}_{-9}({\rm syst.})\ {\rm MeV}$, and $Q_{K} = 383\pm11({\rm stat.})^{+4}_{-1}({\rm syst.})\ {\rm MeV}/c$, respectively. The total production cross-section of $\bar{K}NN$, determined by its $\Lambda p$ decay mode, was $\sigma^{tot}_{K} \cdot BR_{\Lambda p} = 9.3\pm0.8({\rm stat.})^{+1.4}_{-1.0}({\rm syst.})\ \mu{\rm b}$.We estimated the branching ratio of the $\bar{K}NN$ state to the $\Lambda p$ and $\Sigma^{0}p$ decay modes as $BR_{\Lambda p}/BR_{\Sigma^{0}p} \sim 1.7$, by assuming that the physical processes leading to the $\Sigma N\!N$ final states are analogous to those of $\Lambda pn$., Comment: 13 pages, 12 figures