1. Colossal magnetoresistance from spin-polarized polarons in an Ising system
- Author
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Li, Ying-Fei, Been, Emily M., Balguri, Sudhaman, Jia, Chun-Jing, Mahenderu, Mira B., Wang, Zhi-Cheng, Cui, Yi, Chen, Su-Di, Hashimoto, Makoto, Lu, Dong-Hui, Moritz, Brian, Zaanen, Jan, Tafti, Fazel, Devereaux, Thomas P., and Shen, Zhi-Xun
- Subjects
Condensed Matter - Strongly Correlated Electrons - Abstract
Recent experiments suggest a new paradigm towards novel colossal magnetoresistance (CMR) in a family of materials EuM$_2$X$_2$(M=Cd, In, Zn; X=P, As), distinct from the traditional avenues involving Kondo-RKKY crossovers, magnetic phase transitions with structural distortions, or topological phase transitions. Here, we use angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations to explore their origin, particularly focusing on EuCd$_2$P$_2$. While the low-energy spectral weight royally tracks that of the resistivity anomaly near the temperature with maximum magnetoresistance (T$_{MR}$) as expected from transport-spectroscopy correspondence, the spectra are completely incoherent and strongly suppressed with no hint of a Landau quasiparticle. Using systematic material and temperature dependence investigation complemented by theory, we attribute this non-quasiparticle caricature to the strong presence of entangled magnetic and lattice interactions, a characteristic enabled by the $p$-$f$ mixing. Given the known presence of ferromagnetic clusters, this naturally points to the origin of CMR being the scattering of spin-polarized polarons at the boundaries of ferromagnetic clusters. These results are not only illuminating to investigate the strong correlations and topology in EuCd$_2$X$_2$ family, but, in a broader view, exemplify how multiple cooperative interactions can give rise to extraordinary behaviors in condensed matter systems.
- Published
- 2024