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A new mechanism of new particle formation (NPF) is investigated using comprehensive measurements of aerosol physicochemical quantities and meteorological variables made in three continents, including Beijing, China; the Southern Great Plains site in the USA; and SMEAR II Station in Hyytiälä, Finland. Despite the considerably different emissions of chemical species among the sites, a common relationship was found between the characteristics of NPF and the stability intensity. The stability parameter (ζ = Z/L, where Z is the height above ground and L is the Monin-Obukhov length) is found to play an important role; it drops significantly before NPF as the atmosphere becomes more unstable, which may serve as an indicator of nucleation bursts. As the atmosphere becomes unstable, the NPF duration is closely related to the tendency for turbulence development, which influences the evolution of the condensation sink. Presumably, the unstable atmosphere may dilute pre-existing particles, effectively reducing the condensation sink, especially at coarse mode to foster nucleation. This new mechanism is confirmed by model simulations using a molecular dynamic model that mimics the impact of turbulence development on nucleation by inducing and intensifying homogeneous nucleation events.

Urban trees are known for their ability to settle fine particulate matter (PM2.5), yet the effects of historical pollution exposure on their dust-retention capacity and stress memory remain underexplored. Therefore, we selected Euonymus japonicus Thunb. var. aurea-marginatus Hort. and Photinia × fraseri Dress, which are two common urban greening tree species in the Yangtze River Delta, a highly urbanized region in China facing severe air pollution challenges, characterized by dense urban forests, and we employed an aerosol generator to perform controlled experiments aiming to simulate PM2.5 pollution exposure in a sealed chamber. The experiments encompassed a first pollution treatment period P1 (15 days), a recovery period R (15 days), and a second pollution treatment period P2 (15 days). The study investigates the historical impacts of pollution exposure by simulating controlled environmental conditions and assessing the morphological and physiological changes in trees. The main results are as follows: Vd of Euonymus japonicus Thunb. var. aurea-marginatus Hort. significantly decreased on the 10th day during P2 compared with that on the same day during P1, whereas Vd of Photinia × fraseri Dress significantly decreased on the 15th day. Compared with those during P1, the specific leaf area of both plants significantly decreased, the specific leaf weight significantly increased, the wax layer significantly thickened, the stomata decreased, and the content of photosynthetic pigments remained stable during P2. Furthermore, the air pollution tolerance index (APTI) generally increased during both P1 and P2. This study contributes to international knowledge by examining stress memory in urban trees and underscores the role of stress memory in enhancing plant resistance to periodic particulate pollution, offering insights into the adaptive mechanisms that can be applied globally, not just regionally. [ABSTRACT FROM AUTHOR]

The rapid urbanization of urban areas in China has brought about great variation in the layout of cities and serious air pollution. Recently, the focus has been directed toward understanding the role of urban morphology in the generation and spread of atmospheric pollution, particularly in PM2.5 emissions. However, there have been limited investigations into the impact of three-dimensional (3D) features on changes in PM2.5 concentrations. By analyzing a wealth of data on building structures based on a mixed linear model and variance partition analysis in the Yangtze River Delta throughout 2018, this study sought to examine the associations between PM2.5 concentrations and urban building form, and further compared the contributions of two-dimensional (2D) and 3D building features. The findings revealed that both 2D and 3D building forms played an important role in PM2.5 concentrations. Notably, the greater contribution of 3D building forms on PM2.5 concentrations was observed, especially during the summer, where they accounted for 20% compared to 7% for 2D forms. In particular, the building height range emerged as a crucial local factor affecting PM2.5 concentrations, contributing up to 12%. Moreover, taller buildings with more variability in height were found to aid in the dispersion of pollution. These results underscore the substantial contribution of 3D building morphology to PM2.5 pollution, contrasting with previous studies. Furthermore, compact buildings were linked to lower pollution levels, and an urban landscape characterized by polycentric urban structures and lower fragmentation was deemed more favorable for sustainable urban development. This study is significant in investigating the contribution of 3D morphology to PM2.5 and its importance for pollution dispersion mechanisms. It suggests the adoption of a polycentric urban form with a broader range of building heights in urban planning for local governments in the Yangtze River Delta. [ABSTRACT FROM AUTHOR]