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We consider the generation of Schr\"odinger cat states using a quantum measurement-induced logical gate where entanglement between the input state of the target oscillator and the Fock state of the ancillary system produced by the quantum non-demolition entangling $C_Z$ operation is combined with the homodyne measurement. We utilize the semiclassical approach to construct both the input-output mapping of the field variables in the phase space and the wave function of the output state. This approach is found to predict that the state at the gate output is represented by a minimum disturbed cat-like state which is a superposition of two initial state copies symmetrically displaced by momentum variable. For the target oscillator prepared in the coherent state, we show that the fidelity between the exact solution for the gate output state and the "perfect" Schr\"odinger cat reconstructed from the semiclassical theory can reach high values exceeding 0.99., Comment: 14 pages, 12 figures

We develop the algebraic method based on the Lie algebra of quadratic combinations of left and right superoperators associated with matrices to study the Lindblad dynamics of multimode bosonic systems coupled a thermal bath and described by the Liouvillian superoperator that takes into account both dynamical (coherent) and environment mediated (incoherent) interactions between the modes. Our algebraic technique is applied to transform the Liouvillian into the diagonalized form by eliminating jump superoperators and solve the spectral problem. The temperature independent effective non-Hermitian Hamiltonian, $\hat{H}_{eff}$, is found to govern both the diagonalized Liouvillian and the spectral properties. It is shown that the Liouvillian exceptional points are represented by the points in the parameter space where the matrix, $H$, associated with $\hat{H}_{eff}$ is non-diagonalizable. We use our method to derive the low-temperature approximation for the superpropagator and to study the special case of a two mode system representing the photonic polarization modes. For this system, we describe the geometry of exceptional points in the space of frequency and relaxation vectors parameterizing the intermode couplings and, for a single-photon state, evaluate the time dependence of the speed of evolution as a function of the angles characterizing the couplings and the initial state., Comment: 19 pages, 3 figures, a continuation of arxiv:2207.01383

Spectral loopholes in the 1000-2100 nm range have been the focus of attention of quantum hacking research aimed at searching and elimination of vulnerabilities in quantum key distribution systems. In this work, we concentrate on shorter wavelengths ranged from 400 nm up to 800 nm and experimentally study spectra of insertion losses for a number of fiber optical components to assess potentials for their implementation as countermeasures. We show that efficiency of the elements commonly used as countermeasures against hacking attacks in the telecom range can be significantly impaired in the visible range. It is found that the vulnerabilities detected in this range play an increasingly important role for hacking strategies such as the induced-photorefraction attack whose efficiency improves when the wavelength decreases., Comment: 11 pages, 7 figures

The open water surface is known to be charged. Yet, the magnitude of the charge and the physical mechanism of the charging remain unclear, causing heated debates across the scientific community. Here we directly measure the charge Q of microdrops ejected from hydrophilic and hydrophobic capillaries and show that the water surface can take both positive or negative charge values depending on pH and the capillary type. Our experiments, theory, and simulations provide evidence that a junction of two aqueous interfaces with a different ion adsorption energy (e.g., liquid-solid and liquid-air interfaces) develops a pH-dependent contact potential difference {\Delta}{\phi} up to 52 mV. The longitudinal charge transfer between the interfaces stimulated by {\Delta}{\phi} determines the charge of the open water surface. The suggested static electrification mechanism provides far-reaching insights into the origin of electrical potentials in biological and electrochemical energy systems., Comment: 21 pages main text, 4 figures, supporting information, including the theory of the charge transfer between two dissimilar aqueous interfaces induced by the contact potential difference, details of molecular dynamics simulations, and additional graphs, photos, and diagrams, including Figures S1 to S18 and Table S1

We present a scheme of quantum repeater that uses entangled multimode coherent states which are obtained by electro-optic modulation of symmetric and antisymmetric Schr\"odinger cat states. In this method subcarrier modes of the phase modulated states generated by the remote parties are sent to a symmetric beam splitter at the central node. The entangled coherent states are heraldedly prepared by photon counting measurements at the output channels of the beam splitter. We study how the effects of decoherence in the quantum channel affect statistics of photocounts and corresponding fidelity. We show how the proposed scheme can be useful for extending range of quantum key distribution with sub carrier wave encoding by exploiting quantum teleportation with the generated entanglement., Comment: 18 pages, 10 figures

We introduce algebraic approach for superoperators that might be useful tool for investigation of quantum (bosonic) multi-mode systems and its dynamics. In order to demonstrate potential of proposed method we consider multi-mode Liouvillian superoperator that describes relaxation dynamics of a quantum system (including thermalization and intermode coupling). Considered algebraic structure of superoperators that form Liouvillian and their algebraic properties allows us to diagonilize multi-mode Liouvillian to find its spectrum. Also it allows to derive linear by mean number of thermal (environmental) photons approximation for time-evolution superoperator that keeps amount of considered dimensions in Fock space finite (assuming initial amount of dimensions finite) that might be helpful regarding entanglement dynamics problems. Conjugate Liouvillian is considered as well in order to perform analysis in Heisenberg picture, it can be implemented for multi-time correlation functions derivation.

In this paper, using the full security framework for continuous variable quantum key distribution (CV-QKD), we provide a composable security proof for the CV-QKD system in a realistic implementation. We take into account equipment losses and contributions from various components of excess noise and evaluate performance against collective and coherent attacks assuming trusted hardware noise. The calculation showed that the system remains operable at channel losses up to 10.2 dB in the presence of collective attacks and up to 7.5 dB in the presence of coherent ones., Comment: 28 pages, 5 figures

The renewable energy sector critically needs low-cost and environmentally neutral energy storage solutions throughout the entire device life cycle. However, the limited performance of standard water-based electrochemical systems prevents their use in specific applications. Meanwhile, recent fundamental studies revealed dielectric anomalies of water near solid-liquid interfaces of carbon-based nanomaterials. In contrast to the bulk water properties, these anomalies of water under nano-confinement and in the presence of electric fields have not yet been understood and used. Here, we experimentally study the ability of the interfacial water layer to engender and store charge in electrochemical double-layer capacitance. We demonstrate the prototype of a 'water only' membrane-electrode assembly. The prototype exhibits characteristics with a perspective of competing with existing batteries and supercapacitors without using electrolytes as ionic carriers. The results provide the impetus for developing high-energy-density electrochemical double-layer capacitors and open up other avenues for ecologically-neutral batteries, fuel cells, and nanofluidic devices., Comment: 21 pages, 3 figures. The supplementary information includes Samples preparation and treatment, Measurement methods, Figures S1 to S10, and Table S1

We study minimum-energy pathways (MEPs) between the branches of metastable helical structures in chiral nematic liquid crystals (CNLCs)subjected to the electric field applied across the cell. By performing stability analysis we have found that, for the branches with non-vanishing half-turn number, the threshold (critical) voltage of the Freedericksz transition is an increasing function of the free twisting wave number. The curves for the threshold voltage depend on the elastic anisotropy and determine the zero-field critical free twisting number where the director out-of-plane fluctuations destabilize the CNLC helix. For each MEP passing through a first order saddle point we have computed the energy barrier as the energy difference between the saddle-point and the initial structures at different values of the applied field. In our calculations, where the initial approximation for a MEP at the next step was determined by the MEP obtained at the previous step, the electric field dependence of the energy barrier is found to exhibit the hysteresis. This is the hysteresis of electrically driven transition of the saddle-point configuration between the planar and the tilted structures involving out-of-plane director deformations. It turned out that, by contrast to the second-order Freedericksz transition, this transition is first order and we have studied how it depends on the zenithal anchoring energy strength., Comment: revtex 4-2, 10 pages, 7 figures, a continuation of arXiv:1911.03987 [cond-mat.soft]

We examine different methods to implement coherent detection in the subcarrier wave quantum key distribution (SCW QKD) systems. For classical wavefields, we present the models describing homodyne-type and heterodyne-type coherent detection schemes needed to extract information from the quadrature phase-coded multimode signals used in SCW QKD. Practical feasibility of the proposed schemes is corroborated by the experiments., Comment: 14 pages, 10 figures

We apply the minimum energy paths (MEPs) approach to study the helix unwinding transition in chiral nematic liquid crystals. A mechanism of the transition is determined by a MEP passing through a first order saddle point on the free energy surface. The energy difference between the saddle point and the initial state gives the energy barrier of the transition. Two starting approximations for the paths are used to find the MEPs representing different transition scenarios: (a) the director slippage approximation with in-plane helical structures; and (b) the anchoring breaking approximation that involves the structures with profound out-of-plane director deviations. It is shown that, at sufficiently low voltages, the unwinding transition is solely governed by the director slippage mechanism with the planar saddle point structures. When the applied voltage exceeds its critical value below the threshold of the Freedericksz transition, the additional scenario through the anchoring breaking transitions is found to come into play. For these transitions, the saddle point structure is characterized by out-of-plane deformations localized near the bounding surface. The energy barriers for different paths of transitions are computed as a function of the voltage and the anchoring energy strengths., Comment: revtex4-1, 13 pages, 12 figures

We employ the transfer matrix approach combined with the Green's function method to theoretically study polarization resolved far-field angular distributions of photoluminescence from quantum nanorods (NRs) embedded in an anisotropic polymer film. The emission and excitation properties of NRs are described by the emission and excitation anisotropy tensors. These tensors and the solution of the emission problem expressed in terms of the evolution operators are used to derive the orientationally averaged coherency matrix of the emitted wavefield. For the case of in-plane alignment and unpolarized excitation, we estimate the emission anisotropy parameter and compute the angular profiles for the photoluminescence polarization parameter such as the degree of linear polarization, the Stokes parameter $s_1$, the ellipticity and the polarization azimuth. We show that the alignment order parameter has a profound effect on the angular profiles., Comment: revtex4-1, 25 pages, 13 figures, corrected version

We perform direct numerical simulations of the settling of an ice sphere in an ambient fluid accounting for heat and mass transfer with the aim of studying in a meteorological context the case of falling graupel in humid air. The study is motivated by the fact that falling graupels in clouds are heated by the latent heat released during the accretion of liquid water droplets. They may therefore be considerably warmer than their surrounding and evaporate water vapor, which mixes with the surrounding air in the wake of the graupel, thereby creating transient zones of supersaturation there. The problem of a falling graupel is modeled as that of a heated sphere falling in a quiescent ambient fluid under the action of gravity. The coupling between the temperature and velocity fields is accounted for by the Boussinesq approximation. This problem can be parameterized by four parameters: the particle/fluid density ratio, the Galileo number, the Prandtl number, and the Richardson number. A separate scalar transport equation accounts for the vapor transport. Typical cloud conditions involve small temperature differences between the sphere and the surrounding, yielding relatively small Richardson numbers for both heat and mass transport. We give a special emphasis to the Galileo numbers 150, 170, 200 and 300 in order to analyze the specificities of each settling regime. The questions addressed in this study are mainly methodological and concern the influence of the settling regime and the mobility of the sphere on the structure of the scalar fields, the possible influence of modest Richardson numbers on the structure of the wake, and the possible application of this simulation framework to the investigation of the saturation in the wake of a falling graupel.

We theoretically analyze the waveguide regime of light propagation in a cylindrical pore of a polymer matrix filled with liquid crystals assuming that the effective radial optical anisotropy is biaxial. From numerical analysis of the dispersion relations, the waveguide modes are found to be sensitive to the field-induced changes of the anisotropy. The electro-optic properties of the polymer porous polyethylene terephthalate (PET) films filled with the nematic liquid crystal 5CB are studied experimentally and the experimental results are compared with the results of the theoretical investigation., Comment: 15 pages, 10 figures, revtex4-1

In our investigation into the effects of the degree of polarization in modulation of partially polarized light we assume general settings of the interferometry of partially polarized lightwaves and perform theoretical analysis of the Uhlmann and the interferometric phases. We introduce the relative Uhlmann phase determined by the Uhlmann holonomies of interfering beams and show that the interferometric phase generalized to the case of nonunitary evolution can, similar to the Uhlmann phase, be cast into the holonomy defined form. By using the technique based on a two-arm Mach-Zehnder interferometer, two different dynamical regimes of light modulation are experimentally studied: (a) modulation of the input light by the rotating quarter-wave plate (QWP); and (b) modulation of the testing beam by a birefringent plate with electrically controlled anisotropy represented by the deformed-helix ferroelectric liquid crystal (DHFLC) cell. In the setup with the rotating QWP, the interferometric phase is found to be equal to the relative Uhlmann phase. Experimental and theoretical results being in excellent agreement both show that this phase is an oscillating function of the QWP angle and increases with the degree of polarization. For modulation by the DHFLC cell, the data derived from our electro-optic measurements are fitted using the theory of the orientational Kerr effect in FLCs. This theory in combination with the results of fitting is used to evaluate electric field dependencies of the interferometric and the Uhlmann phases., Comment: revtex 4.1, 19 pages, 12 figures (published version)

We study the electro-optic properties of subwavelength-pitch deformed-helix ferroelectric liquid crystals (DHFLC) illuminated with unpolarized light. In the experimental setup based on the Mach-Zehnder interferometer, it was observed that the reference and the sample beams being both unpolarized produce the interference pattern which is insensitive to rotation of in-plane optical axes of the DHFLC cell. We find that the field-induced shift of the interference fringes can be described in terms of the electrically dependent Pancharatnam relative phase determined by the averaged phase shift, whereas the visibility of the fringes is solely dictated by the phase retardation., Comment: 8 pages, 7 figures, revised version. arXiv admin note: text overlap with arXiv:1508.04964

We theoretically study electro-optic light modulation based on the quantum model where the linear electro-optic effect and the externally applied microwave field result in the interaction between optical cavity modes. The model assumes that the number of interacting modes is finite and effects of the mode overlapping coefficient on the strength of the intermode interaction can be taken into account through dependence of the coupling coefficient on the mode characteristics. We show that, under certain conditions, the model is exactly solvable and, in the semiclassical approximation where the microwave field is treated as a classical mode, can be analyzed using the technique of the Jordan mappings for the su(2) Lie algebra. Analytical results are applied to study effects of light modulation on the frequency dependence of the photon counting rate. We also establish the conditions of validity of the semiclassical approximation by applying the methods of polynomially deformed Lie algebras for analysis of the model with quantized microwave field., Comment: 13 pages; 7 figures, revised version

We use the T-matrix formalism in combination with the method of far-field matching to evaluate the optical force exerted by Laguerre-Gaussian (LG) light beams on a spherical (Mie) particle. For both non-vortex and optical vortex LG beams, the theoretical results are used to analyze the optical-force-induced dynamics of the scatterer near the trapping points represented by the equilibrium (zero-force) positions. The regimes of linearized dynamics are described in terms of the stiffness matrix spectrum and the damping constant of the ambient medium. For the purely azimuthal LG beams, the dynamics is found to be locally non-conservative and is characterized by the presence of conditionally stable equilibria (unstable zero-force points that can be stabilized by the ambient damping). The effects related to the Mie resonances that under certain conditions manifest themselves as the points changing the trapping properties of the particles are discussed., Comment: 29 pages, 17 figures. corrected and expanded version; a continuation of our study arXiv:1401.7585

We study both experimentally and theoretically modulation of light in a planar aligned deformed-helix ferroelectric liquid crystal (DHFLC) cell with subwavelength helix pitch, which is also known as a short-pitch DHFLC. In our experiments, azimuthal angle of the in-plane optical axis and electrically controlled parts of the principal in-plane refractive indices were measured as a function of voltage applied across the cell. Theoretical results giving the effective optical tensor of a short-pitch DHFLC expressed in terms of the smectic tilt angle and the refractive indices of FLC are used to fit the experimental data. Optical anisotropy of the FLC material is found to be weakly biaxial. For both the transmissive and reflective modes, the results of fitting are applied to model phase and amplitude modulation of light in the DHFLC cell. We demonstrate that, if the thickness of the DHFLC layer is about 50 $\mu$m, the detrimental effect of field-induced rotation of the in-plane optical axes on the characteristics of an axicon designed using the DHFLC spatial light modulator in the reflective mode is negligible., Comment: 14 pages, 11 figures