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Understanding how the structured incident light interacts with the inherent properties of the manipulated particle and governs the optical force/torque exerted is a cornerstone in the design of optical manipulation techniques, apart from its theoretical significance. Based on the Cartesian multipole expansion theory, we establish a framework for optical force/torque exerted on an arbitrary sized bi-isotropic (chiral) spherical particle immersed in generic monochromatic optical fields. Rigorous expressions are thus derived which explicitly bridges such mechanical effects of light with particle-property-dependent coefficients and "force/torque source" quantities that characterize the incident light structures. Such quantities, totalled only 12, are quadratic in terms of electric and magnetic field vectors, among which are linear and angular momenta, gradient of energy density, spin density, and helicity. They are further organized into four categories based on their parity (P) and duality (D) symmetries and shown to couple with a particle with different P and D symmetries to induce optical force/torque. This classification specifies the symmetry-breaking criteria required to induce optical force/torque, offering a promising roadmap for engineering the optical manipulation.

Owing to the ubiquity and easy-to-shape property of optical intensity, the intensity gradient force of light has been most spectacularly exploited in optical manipulation of small particles. Manifesting the intensity gradient as an optical torque to spin particles is of great fascination on both fundamental and practical sides but remains elusive. Here, we uncover the existence of the optical intensity-gradient torque in the interaction of light with chiral particles. Such a new type of torque derives from the interplay between chirality induced multipoles, which switches its direction for particles with opposite chirality. We show that this torque can be directly detected by a simple standing wave field, created with the interference of two counterpropagating plane-like waves. Our work offers a unique route to achieve rotational control of matter by tailoring the field intensity of Maxwell waves. It also establishes a framework that maps a remarkable connection among the optical forces and torques, across chiral to nonchiral.

The exploration of the rich dynamics of electrons is a frontier in fundamental nano-physics. The dynamical behavior of electrons is dominated by random and chaotic thermal motion with ultrafast ($\approx$ ps) and nanoscale scatterings. This generates fluctuating electromagnetic fields in close vicinity of the moving electrons. W studied this fluctuation in small structures and found that its spatial distribution is not uniform, the magnitude of the fluctuation depends on external parameters such as the size ( ~1 $\mu m$) and the shape of the structure and changes can occur by an order of magnitude. Our work opens the possibility of improving the signal to noise ratio in small devices and in manipulating microscopic electron kinematics through nano-optical techniques and to applications in thermal detectors and photothermal photovoltaics.

We study the response of a conical metallic surface to an external electromagnetic (EM) field by representing the fields in basis functions containing integrable singularities at the tip of the cone. A fast analytical solution is obtained by the conformal mapping between the cone and a round disk. We apply our calculation to the scattering- based scanning near-field optical microscope (s-SNOM) and successfully quantify the elastic light scattering from a vibrating metallic tip over a uniform sample. We find that the field-induced charge distribution consists of localized terms at the tip and the base and an extended bulk term along the body of the cone far away from the tip. In recent s-SNOM experiments at the visible-IR range (600nm - 1$\mu m$) the fundamental is found to be much larger than the higher harmonics whereas at THz range ($100 \mu m-3mm$) the fundamental becomes comparable to the higher harmonics. We find that the localized tip charge dominates the contribution to the higher harmonics and becomes bigger for the THz experiments, thus providing an intuitive understanding of the origin of the near-field signals. We demonstrate the application of our method by extracting a two-dimensional effective dielectric constant map from the s-SNOM image of a finite metallic disk, where the variation comes from the charge density induced by the EM field.

It was theoretically proposed and experimentally demonstrated that anti-reflection coating allows one to trap a high dielectric sphere, at the same time enhancing the transverse optical force. Here, by explicitly calculating the gradient force and the scattering force, we rigorously show that these were mainly consequences of the reduction in scattering force due to the suppression of backward scattering, and enhancement in gradient force due to the increased in overall particle size. The reduction of scattering force can be understood within a ray optics theory and also the Mie theory. The coating approach only works for a spherical particle trapped by an aplanatic beam, and it does not work in general., Comment: 10 pages, 5 figures

We present a multipole expansion theory for optical force exerting on a particle immersed in generic monochromatic free-space optical field. Based on the theory, we have, for the first time, successfully decomposed the optical force on a spherical particle of arbitrary size into a conservative and a nonconservative parts, which are, respectively, written as a gradient of a scalar function and curl of a vector function in an explicit and analytical form. As a result, a scalar potential and a vector potential can be defined, up to gauge freedoms, for the optical force. The decomposition shed light on the understanding of the optical force and pave a new way to engineer optical force for various purposes such as equilibrium statistical mechanics as well as optical micromanipulation.

Like many other physical quantities, the optical force can be expanded using multipole expansion, which has been done in [Nat. Photon. 5, 531], up to electric octupole order. However, in that study, the existence of radiation multipoles were pre-assumed, and the role of the fundamental building units, charges, are not evident. Here, we derive the same multipolar expression of optical force by treating the particles as a collection of point charges or point dipoles, which results in more transparent physics and mathematics.

We establish universal relationships between optical force/torque on a general particle and different parts of linear and angular momentum (AM) of generic monochromatic optical field. It is rigorously proved that the optical force comes about by the transfer of orbital (canonical) optical momentum from light to matter, while the other part of optical momentum, known as spin momentum, does not generate optical force on matter but, instead, stays conserved even when the translational invariance is broken by putting particles into the optical fields. On the other hand, based on a generic multipole theory of optical torque, we demonstrate that the optical torque stems from the transfer of the total optical AM, including both orbital and spin AM, clarifying in generic case the long-standing confusion about whether the orbital AM can induce a spinning torque on a general particle in generic optical fields., Comment: 24 pages

We study the optical forces acting on toroidal nanostructures. A great enhancement of optical force is unambiguously identified as originating from the toroidal dipole resonance based on the source-representation, where the distribution of the induced charges and currents is characterized by the three families of electric, magnetic, and toroidal multipoles. On the other hand, the resonant optical force can also be completely attributed to an electric dipole resonance in the alternative field-representation, where the electromagnetic fields in the source-free region are expressed by two sets of electric and magnetic multipole fields based on symmetry. The confusion is resolved by conceptually introducing the irreducible electric dipole, toroidal dipole, and renormalized electric dipole. We demonstrate that the optical force is a powerful tool to identify toroidal response even when its scattering intensity is dwarfed by the conventional electric and magnetic multipoles., Comment: 25 pages, 7 figures

Optical forces have been fruitfully applied in a broad variety of areas that not only span the traditional scientific fields such as physics, chemistry, and biology, but also in more applied fields. It is customary and useful to split the optical force into the (conservative) gradient force and the (non-conservative) scattering and absorption force. These forces are different in attributes. The ability to tailor them will open great potential in fundamental optics and practical applications. Here, we present an analytical and a numerical approach to calculate these forces, and, with these tools, we create a fairly general class of 2D conservative optical force field. In general, particles immersed in an optical force do not obey equilibrium statistical mechanics, making the analysis complicated. With conservative forces, these issues are resolved., Comment: 16 pages, 4 figures