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The migration of arc magmatism that is a fundamental aspect of plate tectonics may reflect the complex interaction between subduction zone processes and regional tectonics. Here we report new observations on volcanic migration from northwestern Sumatra, in the westernmost Sunda arc, characterized by an oblique convergent boundary between the Indo-Australian and Eurasian plates. Our study indicates that in northwestern Sumatra, volcanism ceased at 15–10 Ma on the southern coast and reignited to form a suite of active volcanoes that erupt exclusively to the north of the trench-parallel Sumatran fault. Younger volcanic rocks from the north are markedly more enriched in K2O and other highly incompatible elements, delineating a geochemical variation over space and time similar to that in Java and reflecting an increase in the Benioff zone depth. We relate this mid-Miocene volcanic migration in northwestern Sumatra to the far-field effect of propagating extrusion tectonics driven by the India-Eurasia collision. The extrusion caused regional deformation southward through Myanmar to northwestern Sumatra and thus transformed the oblique subduction into a dextral motion–governed plate boundary. This tectonic transformation, associated with opening of the Andaman Sea, is suggested to be responsible for the volcanic migration in northwestern Sumatra.

Cenozoic magmatism occurs throughout West Sulawesi, Indonesia, yet its detailed evolution remains enigmatic due mainly to the scarcity of precise dating. Here, we report new whole-rock geochemical and zircon U-Pb-Hf isotopic data of plutonic/volcanic rocks and river sediments from West Sulawesi to constrain the petrogenesis and magmatic tempo. The magmatic rocks are intermediate to felsic (SiO2 = 58.1–68.0 wt%), high-K calc-alkaline to shoshonitic (K2O = 2.2–6.0 wt%), metaluminous to weakly peraluminous, and I-type in composition. Trace element concentrations and ratios (e.g., Nb/U = 1.7–4.3 and Ti/Zr < 28), along with negative zircon εHf(t) values (–17.0 to –0.4) and old crustal model ages (TDMC = 2.1–1.1 Ga), indicate a dominant magma source region from the underlying continental crystalline basement. U-Pb dating on zircons from ten magmatic rocks yielded weighted mean 206Pb/238U ages of 7.2–6.1 Ma, best representing the crystallization ages of host magmas, further consistent with the prominent age peaks (7.3–6.3 Ma) defined by detrital zircons from four sedimentary samples. Our new data, combined with available results, allow the identification of a noticeable climax of magmatism (flare-up) at ca. 7–6 Ma, forming a continuous magmatic belt throughout West Sulawesi. Given the absence of contemporaneous subduction and the coincidence of incipient opening of the South Banda Basin during ca. 7.15–6.5 Ma, the Late Miocene magmatic flare-up in West Sulawesi and coeval regional extension in eastern Indonesia are attributed to a resumed episode of Banda slab rollback.

The provenance of sediments in western Taiwan has been the subject of debate in recent years. Previous investigators, solely based on the U-Pb zircon geochronology for the detrital grains, all advocated the important roles, but with varying emphasis, of drainage systems in the South China Block. Influence of the Changjiang (Yangtze) River from the far-source Yangtze block versus nearby systems like Zhujiang, Minjiang and Jiulongjiang Rivers in the Cathaysia block has been the main issue. However, the fundamental question of whether the provenance is really the South China Block has never been evaluated. Here we report both the U-Pb zircon and Electron MicroProbe (EMP) monazite age data for seven sediment samples from two sides of the Taiwan Strait and synthesize the published data for all these rivers and sedimentary strata in western Taiwan to tackle this problem. The lack of, or insufficient, ~1.8 Ga monazites in the sediments of river mouths for all drainage systems in the South China Block makes them unlikely to be the source of Miocene sediments in western Taiwan where ~1.8 Ga monazite grains occupy 14.5–33.3% of the total age population. With reference to the tectonic evolution of the coastal southeast China-Taiwan region during Early Cretaceous to recent time, we propose a new explanation that invokes a now-concealed microcontinent along the Manila Trench. This microcontinent, probably related to a Paleoproterozoic orogen in Gondwana, eventually collided with the South China Block causing uplift of the easternmost structural element—the Pingtan-Dongshan Metamorphic Belt (PDMB) at ca. 130–120 Ma. It then drifted away sometime after 100 Ma and split into two parts with one becoming today's Palawan-Mindoro terrain of the Philippines. As indicated by the geophysical data near southern Taiwan, the remainder of this split microcontinent had subducted underneath the Philippine Sea plate along Manila Trench as a result of the opening of the South China Sea at ~33 Ma. Both the Peikang and Kuanyin basement highs in the offshore western Taiwan represent the unsubducted remnants of this microcontinent and also the major suppliers of Late Oligocene-Miocene sediments in western Taiwan. On the other hand, the Eocene-Early Oligocene strata of the Hsuehshan Range in central Taiwan show both zircon and monazite age patterns resembling the Eocene-Early Oligocene and recent sediments of the Zhujiang drainage system, indicating the southwestern origin of the protolith Taiwan. This scenario also matches the recent proposition that part of the Central Range belongs to the deep-level accretionary prism of a Miocene subduction system.

The origins of the Mesozoic low-δ18O A-type granites in eastern China are quite controversial. A new “low-δ18O” granite, the Taohuadao alkaline (A1-type) granite from the Zhoushan archipelago, offshore from Zhejiang, is reported in this study. Integrated in situ analyses of Hf-O-Li isotopes in zircon are used to provide insights on the petrogenesis and evolution of this granite, and low-δ18O granites in general. Three types of zircon have been recognized in Taohuadao samples: zircon with sector/oscillatary zoning (Type 1), disturbed zoning (Type 2) and extremely high-U (Type 3) grains. Data are carefully screened for radiation damage and post-magmatic alteration and only Type 1 zircon represents a magmatic origin. In Type 1 zircons, Type 1a with normal mantle δ18Ozrn value of 5.23‰ has a positive δ7Li value (2.0 ± 3.3‰), while Type 1b has a δ18O value of ∼4.81‰ and highly variable negative δ7Li values (−31.9‰ to −0.3‰). In contrast to the O-Li isotopes, zircon is quite homogeneous in terms of Hf isotopes (eHf(t) = −3.5 ± 1.7), suggesting that the Taohuadao A1-type granites were derived from a simple source. Our results show that the magmatic zircon δ18Ozrn values are negatively correlated with Hf content but positively correlated with Zr/Hf ratio in zircon, which indicates that fractional crystallization plays an important role in producing the slightly low δ18O signature. The anhydrous nature of the A1-type granites suppressed the crystallization of biotite and hornblende, while low oxygen fugacity is responsible for insufficient precipitation of magnetite, both of which drive the later differentiates towards slight depletion in 18O. Therefore, we suggest a ferrogabbro-type fractional crystallization may have played a major role in producing the chemical and oxygen isotopic variations of the Taohuadao A1-type granite and accounts for ∼0.5‰ 18O-depletion. The extremely depleted δ7Li in Type 1b zircons is most likely a result of diffusion-driven fractionation. Mantle-like O-Li isotopes and very low Li abundance in zircon suggest a predominantly mantle origin with little, if any, involvement of continental crustal materials in the granite. Thus the Taohuadao A1-type granite was most likely produced by intensive fractionation of reduced, anhydrous basaltic melts, rather than by mixing of mantle- and crustally-derived melts as previously thought.

The initiation and duration of magmatism in the Tatun Volcano Group (TVG), likely resulting from extensional collapse of the northern Taiwan mountain belt, remains an important issue of debates in the Taiwan orogeny. Here we report a detailed study of U-Pb ages determined by SIMS and LA-ICPMS, together with Hf isotopic data, of zircon separates from a total of 22 extrusive rocks from the TVG lava flow and additional two andesites from Keelungyu (KLY), a volcanic islet off NE Taiwan. Magmatic zircons from the TVG are characterized by uniform and high Hf isotopic ratios, with eHf(T) mostly from +20 to +10. Their overall 206Pb/238U ages suggest that the TVG magmatism was initiated ∼3 Ma but more active ≤0.8 Ma with a flare up ≤0.35 Ma. Magmatic zircons from the two KLY samples reveal identical 206Pb/238U ages (0.41 Ma), coupled with Hf isotopes [eHf(T): +25 to +9] comparable to those of the TVG. Thus, KLY is proposed as part of the TVG. Consequently, we argue that the main body of the TVG formed ≤0.8 Ma by post-collisional volcanism, but the mechanism resulting in the magmatic episodes ≥1.0 Ma remains obscure due to the scarcity of rock exposures.

The origin and geodynamic evolution of peak Early Cretaceous magmatism in the southern Great Xing'an Range, North China, have long been controversial. Here we report new U-Pb zircon ages (141–129 Ma) of a suite of dioritic-granitic rocks from central Inner Mongolia, far from the sutures or plate boundaries of the Paleo-Pacific and Mongol-Okhotsk oceans, thus delineating an Early Cretaceous intracontinental magmatic province, which had a peak activity at 130–120 Ma. Dioritic suite including diorite, tonalite, and granodiorite shows variable zircon eHf(t) of +1.4 to + 11.8 and δ18O values of +5.7 to +6.9‰, while granitic suite consisting of monzogranite, syenogranite, and granite porphyry also records variable zircon eHf(t) of −0.9 to +15.0 and δ18O values of +6.3 to +8.1‰, suggesting crustal melting by preexisting crustal source with important recycled supracrustal components including fluids. Furthermore, these rocks show variable whole-rock δ7Li values (−0.6 to +12.1‰), indicating fluids played an important role in magma source. We propose a deep-sourced water-fluxed melting scenario by ancient hydrous slabs inherited from the Paleo-Asian Ocean that were trapped in the deep interior, thus releasing aqueous fluids to melt the lithospheric mantle and produce water-rich mafic magmas. These mafic magmas were underplated into crust where they promoted water-fluxed partial melting to generate the large-scale Early Cretaceous magmatism in the southern Great Xing'an Range. Such melting due to fluxing of aqueous fluids was probably operating as a widespread process responsible for the Early Cretaceous dramatically tectonomagmatic events and evolution of continental crust in NE Asia.

This paper reports the first systematic analysis of age and geochemical variations in volcanic rocks from the Coastal Range of Taiwan, the Northern Luzon Arc. The rocks, recovered from four main volcanoes, vary from low-K tholeiitic to medium-K calc-alkaline basalts to dacites. The rocks are typical of arc magmatic products, exhibiting enrichment in the large ion lithophile elements and depletion in the high field strength elements. Our new 40Ar/39Ar age data constrain the youngest eruption time in each of the four volcanoes, i.e., from north to south, at ~ 7.2 Ma (Yuemei), ~ 4.2 Ma (Chimei), ~ 6.2 Ma (Chengkuang'ao) and ~ 8.5 Ma (Tuluanshan), respectively. These data indicate that volcanism in the Northern Luzon Arc did not cease progressively from north to south, as previously alleged. The high and broadly uniform Nd isotope ratios [eNd = + 10.1 to + 8.8] and trace element characteristics of the rocks suggest a principal magma source from the depleted mantle wedge. Their overall geochemical variations are ascribed to magma chamber processes. The effects of magmatic differentiation and crustal contamination differ among each volcano, most likely owing to the discrepancy of residence time in individual magma chambers. Consequently, we propose a binary mixing model for the magma generation that involves arc magmas sourced from the depleted mantle wedge and up to ~ 5% crustal contamination with a continental fragment split off from the Eurasian margin.

To understand the behavior of Li in zircon, we have analyzed the abundance and isotopic composition of Li in three zircon standards (Plešovice, Qinghu and Temora) widely used for microbeam analysis of U-Pb ages and O-Hf isotopes. We have mapped Li concentration ([Li]) on large grains, using a Cameca 1280HR Secondary Ion Mass Spectrometer (SIMS). All zircons have a rim 5–20 μm wide in which [Li] is 5 to 20 times higher than in the core. Up to ~20‰ isotopic fractionation is observed on a small scale in the rims of a single zircon grain. The measured δ7Li values range from –14.3 to 3.7‰ for Plešovice, –22.8 to 1.4‰ for Qinghu and –4.7 to 16.1‰ for Temora zircon. The [Li] and δ7Li are highly variable at the rims, but relatively homogenous in the cores of the grains. From zircon rim to core, [Li] decreases rapidly, while δ7Li increases, suggesting that the large isotopic variation of Li in zircons could be caused by diffusion. Our data demonstrate that homogeneous δ7Li in the cores of zircon can retain the original isotopic signatures of the magmas, while the bulk analysis of Li isotopes in mineral separates and in bulk-rock samples may produce misleading data.