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The electron-beam-pumped ArF laser is a laser technology capable of providing very high lasing energies at the shortest wavelength (λ = 193 nm) among the rare gas halide lasers and therefore has the potential to be a superior driver for inertial fusion. The electron kinetics are rigorously treated by numerically solving the steady-state, spatially averaged electron Boltzmann equation in Ar-F2 gas. The e-beam energy deposition and collisional reaction rates with electrons are calculated from the electron energy distribution function for a wide range of e-beam deposition powers (Pbeam =10 kW/cm3 –3 MW/cm3) and fluorine concentrations (xF2 = 0.01 – 10%). The rates are reduced to a set of coefficients that are fitted with analytical formulas as a function of two universal parameters: Pbeam/p and xF2 , where p is the gas pressure. It is found that in the regime of high e-beam power deposition, the fluorine molecules are rapidly destroyed through dissociative attachment and neutral dissociation. The loss of F2 over the duration of the beam is proportional to the e-beam energy deposition per unit volume, ebeam, and follows ΔnF2 (cm-3) ≅ 4 x 1017 દbeam(J /cm3, in agreement with experimental data. The fluorine molecule conversion to other fluorine species, including atomic fluorine, is shown to have a very small effect on the index of refraction even at percent level concentrations. [ABSTRACT FROM AUTHOR]

Carbon dioxide is the most important greenhouse gas contributing to global warming. To help mitigate increasing CO2 concentrations, we investigate a method of carbon dioxide reduction using high-power electron beams, which can be used on an industrial scale. A series of experiments are conducted in which the reduction of CO2 is measured for different gas compositions and power deposition rates. An electron beam deposition model is applied to compute reduction rates of CO2 and energy cost for breaking a CO2 molecule in flue gas and pure carbon dioxide at atmospheric pressure. For flue gas consisting of 82% N2, 6% O2, and 12% CO2, the calculated energy cost is 85 eV per molecule. In order to dissociate 50% of the CO2 molecules, beam energy density deposition on the order of 20 J/cm³ is required. Electron beam irradiation of 12.6 liter gas volume containing 90% CO2 and 10% CH4 at beam energy density deposition of 4.2 J/cm³, accumulated over 43 shots in a 20 min interval, reduced the CO2 concentration to 78%. Analogous experiments with a gas mixture containing 11.5% CO2, 11.5% CH4, and balance of Ar, reduced the CO2 concentration to below 11% with energy deposition 0.71 J/cm³, accumulated over 10 shots in a 5 min interval. The experimental data and the theoretical predictions of CO2 reduction using pulsed electron beams are in agreement within the experimental error. Other techniques to enhance the removal of CO2 with pulsed electron beams are also explored, yielding new possible avenues of research. [ABSTRACT FROM AUTHOR]

A theoretical study complemented with published experimental data of proton acceleration from sub-micron (thickness < 1 µm) foils irradiated by ultra-high contrast (>1010) short pulse lasers is presented. The underlying physics issues pertinent to proton acceleration are addressed using two-dimensional particle-in-cell simulations. For laser energy ε ≤ 4 J (intensity I ≤ 5 x 1020 W/cm²), simulation predictions agree with experimental data, both exhibiting scaling superior to Target Normal Sheath Acceleration's model. Anomalous behavior was observed for ε > 4 J (I > 5 x 1020 W/cm²), for which the measured maximum proton energies were much lower than predicted by scaling and these simulations. This unexpected behavior could not be explained within the frame of the model, and we conjecture that pre-pulses preceding the main pulse by picoseconds may be responsible. If technological issues can be resolved, energetic proton beams could be generated for a wide range of applications such as nuclear physics, radiography, and medical science. [ABSTRACT FROM AUTHOR]

We present a broad study of linear, clustered, noble gas puffs irradiated with the frequency doubled (527 nm) Titan laser at Lawrence Livermore National Laboratory. Pure Ar, Kr, and Xe clustered gas puffs, as well as two mixed-gas puffs consisting of KrAr and XeKrAr gases, make up the targets. Characterization experiments to determine gas-puff density show that varying the experimental parameter gas-delay timing (the delay between gas puff initialization and laser-gas-puff interaction) provides a simple control over the gas-puff density. X-ray emission (>1.4 keV) is studied as a function of gas composition, density, and delay timing. Xe gas puffs produce the strongest peak radiation in the several keV spectral region. The emitted radiation was found to be anisotropic, with smaller X-ray flux observed in the direction perpendicular to both laser beam propagation and polarization directions. The degree of anisotropy is independent of gas target type but increases with photon energy. X-ray spectroscopic measurements estimate plasma parameters and highlight their difference with previous studies. Electron beams with energy in excess of 72 keV are present in the noble gas-puff plasmas and results indicate that Ar plays a key role in their production. A drastic increase in harder X-ray emissions (X-ray flash effect) and multi-MeV electron-beam generation from Xe gas-puff plasma occurred when the laser beam was focused on the front edge of the linear gas puff. [ABSTRACT FROM AUTHOR]

Nitric oxide (NOx) emission is under restrictive federal regulations because of its negative impact on atmosphere, biosphere, and human health. Therefore, its removal has been a subject of extensive research to develop new efficient and cost effective techniques that can be applied on an industrial scale. In this work, we study both experimentally and theoretically an effective removal of NOx pollutants from a surrogate flue gas (SFG) using high power electron beam (e-beam) pulses. SFG is a simulant for exhaust from coal combustion power plants (82% N2, 6% O2, 12% CO2, and ~ 100ppm of NOx). The pulsed electron beam is generated using the United States Naval Research Laboratory Electra facility, which delivers e-beams with energies of ~500keV and a power pulse duration of Ѧ 140 ns. During the e-beam irradiation, the energetic electrons generate a non-equilibrium plasma containing chemically active species, which then react with NOx to form harmless substances. A non-equilibrium time-dependent model is developed to describe NOx remediation from SFG. The model combines e-beam deposition rates obtained by solving the electron Boltzmann equation and extensive plasma chemistry modeling, which follows the species on a time scale from sub-nanoseconds to a few seconds. NOx decomposition as a function of electron beam parameters is studied. It is demonstrated experimentally that short (ns) pulses are the most efficient for NOx removal. A sharp reduction of NOx was measured with e-beam power deposition increasing, following the trend predicted by the model, achieving a 20 fold reduction to ~5 ppm at energy deposition ~ 20J/l. [ABSTRACT FROM AUTHOR]

Using several-mJ energy pulses from a high-repetition rate (1/2 kHz), ultrashort (35 fs) pulsed laser interacting with a ~10 µm diameter stream of free-flowing heavy water (D2O), we demonstrate a 2.45MeV neutron flux of 105/s. Operating at high intensity (of order 1019W/cm²), laser pulse energy is efficiently absorbed in the pre-plasma, generating energetic deuterons. These collide with deuterium nuclei in both the bulk target and the large volume of low density D2O vapor surrounding the target to generate neutrons through d(d, n) ³He reactions. The neutron flux, as measured by a calibrated neutron bubble detector, increases as the laser pulse energy is increased from 6 mJ to 12 mJ. A quantitative comparison between the measured flux and the results derived from 2D-particle-in-cell simulations shows comparable neutron fluxes for laser characteristics similar to the experiment. The simulations reveal that there are two groups of deuterons. Forward moving deuterons generate deuterium--deuterium fusion reactions in the D2O stream and act as a point source of neutrons, while backward moving deuterons propagate through the low-density D2O vapor filled chamber and yield a volumetric source of neutrons. [ABSTRACT FROM AUTHOR]

The effect of nitrogen addition on the emission intensities of the brightest argon lines produced in a low pressure argon/nitrogen electron beam-generated plasmas is characterized using optical emission spectroscopy. In particular, a decrease in the intensities of the 811.5 nm and 763.5 nm lines is observed, while the intensity of the 750.4 nm line remains unchanged as nitrogen is added. To explain this phenomenon, a non-equilibrium collisional-radiative model is developed and used to compute the population of argon excited states and line intensities as a function of gas composition. The results show that the addition of nitrogen to argon modifies the electron energy distribution function, reduces the electron temperature, and depopulates Ar metastables in exchange reactions with electrons and N2 molecules, all of which lead to changes in argon excited states population and thus the emission originating from the Ar 4p levels. [ABSTRACT FROM AUTHOR]