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Asymmetric spin–orbit interaction (ASOI) breaks the limitations in conjugate symmetry of traditional geometric phase metasurfaces, bringing new opportunities for various applications such as spin-decoupled holography, imaging, and complex light field manipulation. Since anisotropy is a requirement for spin–orbit interactions, existing ASOI mainly relies on meta-atom with C1 and C2 symmetries, which usually suffer from an efficiency decrease caused by the propagation phase control through the structural size. Here, we demonstrate for the first time that ASOI can be realized in meta-atoms with rotational symmetry ≥3 by combining the generalized geometric phase with the propagation phase. Utilizing an all-metallic configuration, the average diffraction efficiency of the spin-decoupled beam deflector based on C3 meta-atoms reaches ∼84 % in the wavelength range of 9.3–10.6 μm, which is much higher than that of the commonly used C2 meta-atoms with the same period and height. This is because the anisotropy of the C3 metasurface originates from the lattice coupling effect, which is relatively insensitive to the propagation phase control through the meta-atom size. A spin-decoupled beam deflector and hologram meta-device were experimentally demonstrated and performed well over a broadband wavelength range. This work opens a new route for ASOI, which is significant for realizing high-efficiency and broadband spin-decoupled meta-devices. [ABSTRACT FROM AUTHOR]

Low symmetric two dimensional (2D) semiconductors are of great significance for their potential applications in polarization‐sensitive photodetection and quantum information devices. However, their real applications are limited by their photo‐detecting wavelength ranges, which are restricted by their fundamental optical bandgaps. Recently, intercalation has been demonstrated to be a powerful strategy to modulate the optical bandgaps of 2D semiconductors. Here, the authors report the self‐driven oxygen (O2) intercalation induced bandgap reduction from 1.75 to 1.19 eV in gallium telluride (GaTe) in air. This bandgap shrinkage provides the long‐wavelength detection threshold above ≈1100 nm for O2 intercalated GaTe (referred to as GaTeO2), well beyond the cut‐off wavelength at ≈708 nm for pristine GaTe. The GaTeO2 photodetectors have a high photoresponsivity, and highly anisotropic photodetection behavior to even sub‐waveband radiation. The dichroic ratio (Imax/Imin) of photocurrent is about 1.39 and 2.9 for 600 nm and 1100 nm, respectively. This findings demonstrates a broadband photodetector utilizing GaTe after breaking through its bandgap limitation by self‐driven O2 intercalation in air and further reveal its photoconductivity anisotropic nature. This provides design strategies of 2D materials‐based high‐performance broadband photodetectors for the exploration of polarized state information. [ABSTRACT FROM AUTHOR]