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The Local Climate Zone (LCZ) classification scheme is a vital method of building a category dataset for high-resolution urban land. For the development of urban meteorology, air pollution and related disciplines, the high-resolution classification data of urban buildings are very important. This study aims to create LCZ datasets with detailed architectural characteristics for major cities and urban agglomerations in China, and obtain more accurate results. We constructed 120 m resolution land use datasets for 63 cities (mainly provincial capitals, municipalities directly under the Central Government, important prefecture-level cities and special administrative regions) and 4 urban agglomerations in China based on the local climate zone (LCZ) classification scheme using the World Urban Database and Access Portal Tools method (WUDAPT). Nearly 100,000 samples were used, of which 76,000 training samples were used to provide spectral signatures and 23,000 validation samples were used to ensure accuracy assessments. Compared with similar studies, the LCZ datasets in this paper were generally of good quality, with an overall accuracy of 71–93% (mean 82%), an accuracy for built classifications of 57–83% (mean 72%), and an accuracy for natural classifications of 70–99% (mean 90%). In addition, 35% of 63 Chinese cities have construction areas of more than 5%, and the plateaus northwest of Chengdu and Chongqing are covered with snow all year round. Therefore, based on the original LCZ classification system, the construction area (LZC H) and the snow cover (LCZ I) were newly added as the basic classifications of urban LCZ classification in China. Detailed architectural features of cities and urban agglomerations in China are provided by the LCZ datasets in this study. It can be applied to fine numerical models of the meteorological and atmospheric environment and improve the prediction accuracy. [ABSTRACT FROM AUTHOR]