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For solving a block lower triangular Toeplitz linear system arising from the time-space fractional diffusion equations more effectively, a single-parameter two-step split iterative method (TSS) is introduced, its convergence theory is established and the corresponding preconditioner is also presented. Theoretical analysis shows that the original coefficient matrix after preconditioned can be expressed as the sum of the identity matrix, a low-rank matrix, and a small norm matrix. Numerical experiments show that the preconditioner improve the calculation efficiency of the Krylov subspace iteration method.