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High-resolution (e.g., 5 km) emission data of nitrogen oxides (NO x = NO + NO 2 ) provide localized knowledge of pollution sources for targeted regulations, yet such data are lacking or inaccurate over most regions at present. Here we improve our PHLET-based inversion method to derive NO x emissions in China at a 5-km resolution in summer 2019, based on the TROPOMI-POMINO satellite product of nitrogen dioxide (NO 2 ) columns. With low computational costs, our inversion explicitly accounts for the effects of horizontal transport and nonlinear chemistry. We find numerous small-to-medium sources related to minor roads and small human settlements at relatively low affluence levels, in addition to clear emission signals along major transportation lines, consistent with road line density and Tencent location data. Many small-to-medium sources and transportation emissions are unclear or missing in the spatial distributions of four widely used emission inventories. Our emissions offer a unique reference for targeted emission control.

Atmospheric transport of fine particulate matter (PM 2.5 ), the leading environmental risk factor for public health, is estimated to exert substantial transboundary effects at present. During the past several decades, human-produced pollutant emissions have undergone drastic and regionally distinctive changes, yet it remains unclear about the resulting global transboundary health impacts. Here we show that between 1950 and 2014, global anthropogenic PM 2.5 has led to 185.7 million premature deaths cumulatively, including about 14% from transboundary pollution. Among four country groups at different affluence levels, on a basis of per capita contribution to transboundary mortality, a richer region tends to exert severer cumulative health externality, with the poorest bearing the worst net externality after contrasting import and export of pollution mortality. The temporal changes in transboundary mortality and cross-regional inequality are substantial. Effort to reduce PM 2.5 -related transboundary mortality should seek international collaborative strategies that account for historical responsibility and inequality., Competing Interests: Conflict of interest The authors declare that they have no conflict of interest., (Copyright © 2021 Science China Press. Published by Elsevier B.V. All rights reserved.)

Ambient near-surface ozone pollution threatens public health. Over the past decades, the world has seen complex ozone changes across the globe, with important implications for public health. Previous studies have estimated premature mortality attributable to ozone exposure in more recent years, yet a historical assessment of the health impacts of ozone is largely lacking. Contrary to controlling many other air pollutants endangering public health, reducing ozone pollution is complicated by its nonlinear chemistry and complex relationship with precursor emissions. A historical evaluation is crucial to understanding the long-term changes in surface ozone concentration, driving factors, and health implications. This study uses chemical transport model simulations, ground measurements, and pollution-health response models to estimate the ozone changes over the past few decades, their health impacts, and the effectiveness of precursor emission control. Our results will help improve the ozone mitigation strategies on the global scale. [ABSTRACT FROM AUTHOR]