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This paper describes a neural network cloud masking scheme from PARASOL (Polarization and Anisotropy of Reflectances for Atmospheric Science coupled with Observations from a Lidar) multi-angle polarimetric measurements. The algorithm has been trained on synthetic measurements and has been applied to the processing of 1 year of PARASOL data. Comparisons of the retrieved cloud fraction with MODIS (Moderate Resolution Imaging Spectroradiometer) products show overall agreement in spatial and temporal patterns, but the PARASOL neural network (PARASOL-NN) retrieves lower cloud fractions. Comparisons with a goodness-of-fit mask from aerosol retrievals suggest that the NN cloud mask flags fewer clear pixels as cloudy than MODIS (∼ 3 % of the clear pixels versus ∼ 15 % by MODIS). On the other hand the NN classifies more pixels incorrectly as clear than MODIS (∼ 20 % by NN, versus ∼ 15 % by MODIS). Additionally, the NN and MODIS cloud mask have been applied to the aerosol retrievals from PARASOL using the Remote Sensing of Trace Gas and Aerosol Products (RemoTAP) algorithm. Validation with AERONET shows that the NN cloud mask performs comparably with MODIS in screening residual cloud contamination in retrieved aerosol properties. Our study demonstrates that cloud masking from multi-angle polarimeter (MAP) aerosol retrievals can be performed based on the MAP measurements themselves, making the retrievals independent of the availability of a cloud imager. [ABSTRACT FROM AUTHOR]

From a passive satellite remote sensing point of view, the richest set of information on aerosol properties can be obtained from instruments that measure both intensity and polarization of backscattered sunlight at multiple wavelengths and multiple viewing angles for one ground pixel. However, it is challenging to exploit this information at a global scale because complex algorithms are needed with many fit parameters (aerosol and land/ocean reflection), based on online radiative transfer models. So far, two such algorithms have demonstrated this capability at a global scale: the Generalized Retrieval of Atmosphere and Surface Properties (GRASP) algorithm and the Remote sensing of Trace gas and Aerosol Products (RemoTAP) algorithm. In this paper, we present a detailed comparison of the most recent versions of RemoTAP and GRASP. We evaluate both algorithms for synthetic observations, for real PARASOL (Polarization and Anisotropy of Reflectances for Atmospheric Science coupled with Observations from a Lidar) observations against AERONET (Aerosol Robotic Network) for common pixels, and for global PARASOL retrievals for the year 2008. For the aerosol optical depth (AOD) over land, both algorithms show a root mean square error (RMSE) of 0.10 (at 550 nm). For single scattering albedo (SSA), both algorithms show a good performance in terms of RMSE (0.04), but RemoTAP has a smaller bias (0.002) compared to GRASP (0.021). For the Ångström exponent (AE), GRASP has a smaller RMSE (0.367) than RemoTAP (0.387), mainly caused by a small overestimate of AE at low values (large particles). Over ocean both algorithms perform very well. For AOD, RemoTAP has an RMSE of 0.057 and GRASP an even smaller RMSE of 0.047. For AE, the RMSEs of RemoTAP and GRASP are 0.285 and 0.224, respectively. Based on the AERONET comparison, we conclude that both algorithms show very similar overall performance, where both algorithms have stronger and weaker points. For the global data products, we find a root mean square difference (RMSD) between RemoTAP and GRASP AOD of 0.12 and 0.038 over land and ocean, respectively. The largest differences occur over the biomass burning region in equatorial Africa. The global mean values are virtually unbiased with respect to each other. For AE the RMSD between RemoTAP and GRASP is 0.33 over land and 0.23 over ocean. For SSA, we find much better agreement over land (bias = - 0.01, RMSD = 0.043 for retrievals with AOD > 0.2) than over ocean (bias = 0.053, RMSD = 0.074). As expected, the differences increase towards low AOD, over both land and ocean. We also compared the GRASP and RemoTAP AOD and AE products against MODIS. For AOD over land, the agreement of either GRASP or RemoTAP with MODIS is worse than the agreement between the two PARASOL algorithms themselves. Over ocean, the agreement is very similar among the three products for AOD. For AE, the agreement between GRASP and RemoTAP is much better than the agreement of both products with MODIS. The agreement of the latest product versions with each other and with AERONET improved significantly compared to the previous version of the global products of GRASP and RemoTAP. The results demonstrate that the dedicated effort in algorithm development for multi-angle polarimetric (MAP) aerosol retrievals still leads to substantial improvement of the resulting aerosol products, and this is still an ongoing process. [ABSTRACT FROM AUTHOR]

Uncrewed aerial vehicles (UAVs) have become widely used in a range of atmospheric science research applications. Because of their small size, flexible range of motion, adaptability, and low cost, multirotor UAVs are especially well-suited for probing the lower atmosphere. However, their use so far has been limited to conditions outside of clouds, first because of the difficulty of flying beyond visual line of sight and second because of the challenge of flying in icing conditions in supercooled clouds. Here, we present two UAVs for cloud microphysical research: one UAV (the measurement UAV) equipped with a Portable Optical Particle Spectrometer (POPS) and meteorological sensors to probe the aerosol and meteorological properties in the boundary layer and one UAV (the seeding UAV) equipped with seeding flares to produce a plume of particles that can nucleate ice in supercooled clouds. A propeller heating mechanism on both UAVs allows for operating in supercooled clouds with icing conditions. These UAVs are an integral part of the CLOUDLAB project in which glaciogenic cloud seeding of supercooled low stratus clouds is utilized for studying aerosol–cloud interactions and ice crystal formation and growth. In this paper, we first show validations of the POPS on board the measurement UAV, demonstrating that the rotor turbulence has a small effect on measured particle number concentrations. We then exemplify the applicability for profiling the planetary boundary layer, as well as for sampling and characterizing aerosol plumes, in this case, the seeding plume. We also present a new method for filtering out high-concentration data to ensure good data quality of POPS. We explain the different flight patterns that are possible for both UAVs, namely horizontal or vertical leg patterns or hovering, with an extensive and flexible parameter space for designing the flight patterns according to our scientific goals. Finally, we show two examples of seeding experiments: first characterizing an out-of-cloud seeding plume with the measurement UAV flying horizontal transects through the plume and, second, characterizing an in-cloud seeding plume with downstream measurements from a POPS and a holographic imager mounted on a tethered balloon. Particle number concentrations and particle number size distributions of the seeding plume from the experiments reveal that we can successfully produce and measure the seeding plume, both in-cloud (with accompanying elevated ice crystal number concentrations) and out-of-cloud. The methods presented here will be useful for probing the lower atmosphere, for characterizing aerosol plumes, and for deepening our cloud microphysical understanding through cloud seeding experiments, all of which have the potential to benefit the atmospheric science community. [ABSTRACT FROM AUTHOR]

To tackle the current pressing atmospheric science issues, as well as those in the future, a robust scientific community is necessary in all regions across the globe. Unfortunately, this does not yet exist. There are many geographical areas that are still underrepresented in the atmospheric science community, many of which are in the Global South. There are also larger gaps in the understanding of atmospheric composition, processes, and impacts in these regions. In this opinion, we focus on two geographical areas in the Global South to discuss some common challenges and constraints, with a focus on our strengths in atmospheric science research. It is these strengths, we believe, that highlight the critical role of Global South researchers in the future of atmospheric science research. [ABSTRACT FROM AUTHOR]

Warm-sector heavy rainfall along the south China coast poses significant forecasting challenges due to its localized nature and prolonged duration. To improve the prediction of such high-impact weather events, high-resolution numerical weather prediction (NWP) models are increasingly used to more accurately represent topographic effects. However, as these models' grid spacing approaches the scale of convective processes, they enter a "gray zone", where the models struggle to fully resolve the turbulent eddies within the atmospheric boundary layer, necessitating partial parameterization. The appropriateness of applying convection parameterization (CP) schemes within this gray zone remains controversial. To address this, scale-aware CP schemes have been developed to improve the representation of convective transport. Among these, the multi-scale Kain–Fritsch (MSKF) scheme enhances the traditional Kain–Fritsch (KF) scheme, incorporating modifications that facilitate its effective application at spatial resolutions as high as 2 km. In recent years, there has been an increase in the application of machine learning (ML) models across various domains of atmospheric sciences, including efforts to replace conventional physical parameterizations with ML models. This work introduces a multi-output bidirectional long short-term memory (Bi-LSTM) model intended to replace the scale-aware MSKF CP scheme. This multi-output Bi-LSTM model is capable of simultaneously predicting the convection trigger while also modeling the associated convective tendencies and precipitation rates with a high performance. Data for training and testing the model are generated using the Weather Research and Forecast (WRF) model over south China at a horizontal resolution of 5 km. Furthermore, this work evaluates the performance of the WRF model coupled with the ML-based CP scheme against simulations with the traditional MSKF scheme. The results demonstrate that the Bi-LSTM model can achieve high accuracy, indicating the promising potential of ML models to substitute the MSKF scheme in the gray zone. [ABSTRACT FROM AUTHOR]

The acquisition and dissemination of essential information for understanding global biogeochemical interactions between the atmosphere and ecosystems and how climate–ecosystem feedback loops may change atmospheric composition in the future comprise a fundamental prerequisite for societal resilience in the face of climate change. In particular, the detection of trends and seasonality in the abundance of greenhouse gases and short-lived climate-active atmospheric constituents is an important aspect of climate science. Therefore, easy and fast access to reliable, long-term, and high-quality observational environmental data is recognised as fundamental to research and the development of environmental forecasting and assessment services. In our opinion article, we discuss the potential role that environmental research infrastructures in Europe (ENVRI RIs) can play in the context of an integrated global observation system. In particular, we focus on the role of the atmosphere-centred research infrastructures ACTRIS (Aerosol, Clouds and Trace Gases Research Infrastructure), IAGOS (In-service Aircraft for a Global Observing System), and ICOS (Integrated Carbon Observation System), also referred to as ATMO-RIs, with their capabilities for standardised collection and provision of long-term and high-quality observational data, complemented by rich metadata. The ATMO-RIs provide data through open access and offer data interoperability across different research fields including all fields of environmental sciences and beyond. As a result of these capabilities in data collection and provision, we elaborate on the novel research opportunities in atmospheric sciences which arise from the combination of open-access and interoperable observational data, tools, and technologies offered by data-intensive science and the emerging collaboration platform ENVRI-Hub, hosted by the European Open Science Cloud (EOSC). [ABSTRACT FROM AUTHOR]

The use of remote sensing methods to accurately measure cloud properties and their spatiotemporal changes has been widely welcomed in many fields of atmospheric research. The Nanjing Joint Institute for Atmospheric Sciences (NJIAS) Himawari-8/9 Cloud Feature Dataset (HCFD) provides a comprehensive description of cloud features over the East Asia and west North Pacific regions for the 7-year period from April 2016 to December 2022. Multiple cloud variables, such as cloud mask, phase/type, top height, optical thickness, and particle effective radius, as well as snow, dust, and haze masks, were generated from the visible and infrared measurements of the Advanced Himawari Imager (AHI) on board the Japanese geostationary satellites Himawari-8 and Himawari-9 using a series of recently developed cloud retrieval algorithms. Verifications with the Cloud–Aerosol Lidar with Orthogonal Polarization (CALIOP) 1 km cloud layer product and the Moderate Resolution Imaging Spectroradiometer (MODIS) Level-2 cloud product (MYD06) demonstrate that the NJIAS HCFD gives higher skill scores than the Japanese Himawari-8/9 operational cloud product for all cloud variables except for cloud particle effective radius. The NJIAS HCFD even outperforms the MYD06 in nighttime cloud detection; cloud-top height, pressure, and temperature estimation; and infrared-only cloud-top phase determination. All evaluations are performed at the nominal 2 km scale, not including the effects of sub-pixel cloudiness or very thin cirrus. Two examples are presented to demonstrate applications of the NJIAS HCFD for climate and typhoon research. The NJIAS HCFD has been published in the Science Data Bank (https://doi.org/10.57760/sciencedb.09950 , Zhuge 2023a; https://doi.org/10.57760/sciencedb.09953 , Zhuge 2023b; https://doi.org/10.57760/sciencedb.09954 , Zhuge 2023c; https://doi.org/10.57760/sciencedb.10158 , Zhuge 2023d; https://doi.org/10.57760/sciencedb.09945 , Zhuge 2023e). [ABSTRACT FROM AUTHOR]

Instruments measuring aerosol light absorption, such as the Aethalometer and the Multi-Wavelength Absorbance Analyzer (MWAA), have been extensively used to characterize optical absorption of atmospheric particulate matter. Data retrieved with such instruments can be analysed with mathematical models to apportion different aerosol sources (Aethalometer model) and components (MWAA model). In this work we present an upgrade to the MWAA optical apportionment model. In addition to the apportionment of the absorption coefficient babs in its components (black carbon and brown carbon) and sources (fossil fuels and wood burning), the extended model allows for the retrieval of the absorption Ångström exponent of each component and source, thereby avoiding initial assumptions regarding these parameters. We also present a new open-source software toolkit, the MWAA model toolkit (MWAA_MT), written in both Python and R, that performs the entire apportionment procedure. [ABSTRACT FROM AUTHOR]