1. Applicability assessment of effective-medium approximation in predicting radiative characteristics of fractal aggregates with non-absorbing spherical particles.
- Author
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Zhang, Xiaoyue, Zhang, Jin, Zhang, Yuhan, and Fang, Le
- Subjects
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FRACTAL dimensions , *MULTIPLE scattering (Physics) , *LORENZ equations , *REFRACTIVE index , *T-matrix , *FORECASTING , *SMALL-angle neutron scattering , *MIE scattering - Abstract
• Impact of fractal dimension on aggregate scattering cross-section predicted by EMA was assessed. • Condition when EMA is more accurate than RDG-FA was proposed with reference to MSTM. • A critical aggregate size parameter value for which EMA is applicable was suggested. Particles within aggregates are commonly in a status of dependent scattering due to the near-field multiple scattering and far-field interferences from neighboring particles. The integral radiative characteristics of fractal aggregates are consequently not only influenced by the monomer size parameter x s , the refractive index n m , and the monomer number N s , but also tied to the fractal dimension D f. The effective-medium approximation (EMA) simplifies the calculation of aggregate radiative characteristics by treating an aggregate and its surrounding medium as a homogeneous sphere with an effective refractive index, and by applying the Lorenz-Mie theory to this equivalent sphere. The study aims to assess the applicability of EMA to predict the scattering cross-section of fractal aggregates consisting of non-absorbing monomers with x s , varying from 0.001 to 1.25, N s ranging from 10 to 500, under different fractal dimensions D f. The accurate results obtained using the multiple spheres T-matrix were used as a reference. In addition, the RDG-FA (Rayleigh-Deybe-Gans Fractal Aggregates) theory, which is widely used for aggregates with monomer size x s ≪ 1, was also evaluated for comparison. The finding reveals that both EMA and RDG-FA provide accurate predictions for aggregates satisfying the equivalent aggregate size parameter χ m less than D f , where the dependent scattering is limited. As the dependent scattering effect increases, the fractal dimension D f emerges as a critical factor influencing EMA's accuracy, with EMA excelling for aggregates with larger fractal dimensions close to 3. Furthermore, 2.1 is a critical value of D f above which EMA outperforms RDG-FA. [ABSTRACT FROM AUTHOR]
- Published
- 2024
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