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In recent years, global attention to carbon emissions has increased, becoming one of the main drivers of global climate change. Accurate prediction of carbon emission trends in small and medium-sized countries and scientific regulation of carbon emissions can provide theoretical support and policy references for the effective and rational use of energy and the promotion of the coordinated development of energy, environment, and economy. This paper establishes a grey prediction model using the classical Logistic mathematical model in a determined environment to investigate the carbon emission system. At the same time, we use the basic principle of fractional-order accumulation to establish a grey prediction model with fractional-order Logistic and obtain the parameter estimation and time-response equation of the new model by solving the model through the theory related to fractional-order operators. The particle swarm optimization algorithm is used to complete the optimization process of the order of the fractional order grey prediction model and obtain the optimal model order. Then, the new model is applied to predict carbon emissions in five medium-emission countries: Ethiopia, Djibouti, Ghana, Belgium, and Austria. The new model shows better advantages in the validity analysis process, and the simulation results indicate that the new model proposed in this paper has stronger stability and better simulation and prediction accuracy than other comparative models, proving the model's validity. Finally, the model is used to forecast the carbon emissions of these five countries for the five years of 2021–2025, and the results are analyzed, and relevant policy recommendations are made. [ABSTRACT FROM AUTHOR]