1. Inelastic scattering of photoelectrons from He nanodroplets
- Author
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Thomas Pfeifer, Marcel Mudrich, Aaron LaForge, M. Shcherbinin, Sivarama Krishnan, Muhammad Hanif, F. Vad Westergaard, and Robert Richter
- Subjects
Physics ,010304 chemical physics ,FOS: Physical sciences ,General Physics and Astronomy ,Electron ,Photoionization ,Inelastic scattering ,Photoelectric effect ,010402 general chemistry ,01 natural sciences ,0104 chemical sciences ,Ion ,Extreme ultraviolet ,Ionization ,0103 physical sciences ,Physics::Atomic and Molecular Clusters ,Physics - Atomic and Molecular Clusters ,Physics::Atomic Physics ,Physical and Theoretical Chemistry ,Atomic physics ,Atomic and Molecular Clusters (physics.atm-clus) ,Electron ionization - Abstract
We present a detailed study of inelastic energy-loss collisions of photoelectrons emitted from He nanodroplets by tunable extreme ultraviolet (XUV) radiation. Using coincidence imaging detection of electrons and ions, we probe the lowest He droplet excited states up to the electron impact ionization threshold. We find significant signal contributions from photoelectrons emitted from free He atoms accompanying the He nanodroplet beam. Furthermore, signal contributions from photoionization and electron impact excitation/ionization occurring in pairs of nearest-neighbor atoms in the He droplets are detected. This work highlights the importance of inelastic electron scattering in the interaction of nanoparticles with XUV radiation.
- Published
- 2019