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We report on angle-resolved, exciton-polariton photoluminescence measurements from asymmetric terminals of a microsphere-coupled organic waveguide (MOW). The MOW architecture consisted of a SiO2 microsphere coupled with a diaminoanthroquinone mesowire, self-assembled on a glass substrate. The angle-resolved emission measurements were performed using spatially filtered Fourier-plane optical imaging method. The light emanating from the sphere-terminus had two regions of angular emission in the Fourier-plane, of which one had azimuthal angular spread as small as 10°. The emission from wire terminus was uni-directional in nature, with some light emitted beyond the critical angle of glass-air interface. Our results highlight unique directional emission characteristics of a hybrid organic waveguide geometry and may have implications on single-element, exciton-polariton based light-emitting devices and lasers.

In this letter, we show how organic molecular waveguides of 1,5-diaminoanthraquinone molecules can be grown on a silica microsphere to obtain microsphere-coupled organic waveguides (MOWs). Using such MOWs, we remotely excite and detect whispering gallery modes (WGMs) of the attached microsphere. Interestingly, these WGMs showed mode-splitting and mode-mixing due to broken azimuthal symmetry of the microsphere. Furthermore, the waveguiding characteristics of MOWs showed a quadrupole intensity pattern as a function of input polarization. The presented geometry can be an excellent test-bed to study fundamental aspects of coupled resonant systems, and their properties can be harnessed in nano- and bio-photonics.

Herein, we report on the experimental observation of light propagation and localization capabilities of end-to-end connected silver nanowire (Ag NW) pairs. By exciting the surface plasmon polaritons at one end of Ag NW pair, we observed relatively intense light emission at the junction and weak light emission at the distal end of the pair. To probe the localization of light at nanowire junction, we captured far-field Raman image of an isolated Ag NW pair adsorbed with rhodamine 6 G and observed enhanced Raman scattering at the nanowire junction. Such nanophotonic modules with light propagation and localization capabilities can be harnessed for multiplexed on-chip plasmonics.