1. Strong peak in Tc of Sr2RuO4 under uniaxial pressure
- Author
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Alexander Steppke, Lishan Zhao, Andrew P. Mackenzie, Yoshiteru Maeno, Fabian Jerzembeck, Mark Edward Barber, Alexandra S. Gibbs, Thomas Scaffidi, Helge Rosner, Steven H. Simon, Clifford W. Hicks, EPSRC, University of St Andrews. School of Physics and Astronomy, and University of St Andrews. Condensed Matter Physics
- Subjects
TP ,Hydrostatic pressure ,FOS: Physical sciences ,02 engineering and technology ,Electron ,Electronic structure ,01 natural sciences ,TP Chemical technology ,Superconductivity (cond-mat.supr-con) ,Condensed Matter::Superconductivity ,0103 physical sciences ,010306 general physics ,Critical field ,R2C ,QC ,Physics ,Superconductivity ,Multidisciplinary ,Condensed matter physics ,Condensed Matter - Superconductivity ,Fermi surface ,DAS ,021001 nanoscience & nanotechnology ,QC Physics ,Charge carrier ,0210 nano-technology ,Ground state ,BDC - Abstract
INTRODUCTION A central challenge of modern condensed matter physics is to understand the range of possible collective states formed by assemblies of strongly interacting electrons. Most real materials contain high levels of disorder, which can disrupt possible ordered states and so substantially hinder the path to understanding. There is a premium, therefore, on working with extremely clean materials and identifying clean ways to tune their physical properties. Here, we show that uniaxial pressure can induce profound changes in the superconductivity of one of the model materials in the field, Sr 2 RuO 4 , and demonstrate using explicit calculations how our findings provide strong constraints on theory. RATIONALE Superconductivity remains arguably the most intriguing collective electron state. All superconductors form from the condensation of pairs of electrons into a single ground state, but in “unconventional” superconductors, a rich variety of qualitatively different ground states is possible. One of the most celebrated examples, and the one with the lowest known levels of disorder, is Sr 2 RuO 4 . Previous experimental results suggest that its superconducting condensate has odd parity, that is, its phase is reversed upon inversion of spatial coordinates. A relatively unexplored route to test this possibility is to perturb the assembly of conduction electrons through lattice distortion, which introduces no additional disorder. Electronic structure calculations suggest that if sufficient uniaxial pressure could be applied to compress the lattice along the pressure axis by about 0.8%, the largest Fermi surface of Sr 2 RuO 4 would undergo a topological transition. One of the consequences of tuning to this transition would be to substantially lower the velocity of some of charge carriers, and because slow carriers are generally favorable for superconductivity, the superconductivity might be profoundly affected. Although this topological transition has been achieved with other experimental techniques, too much disorder was introduced for the superconductivity to survive. RESULTS Our central experimental result is summarized in the figure. We prepare the sample as a beam and use piezoelectric stacks to compress it along its length. Compressing the a axis of the Sr 2 RuO 4 lattice drives the superconducting transition temperature ( T c ) through a pronounced maximum, at a compression of ≈0.6%, that is a factor of 2.3 higher than T c of the unstrained material. At the maximum T c , the superconducting transition is very sharp, allowing precise determination of the superconducting upper critical magnetic fields for fields along both the a and c directions. The c -axis upper critical field is found to be enhanced by more than a factor of 20. We perform calculations using a weak-coupling theory to compare the T c ’s and upper critical fields of possible superconducting order parameters. The combination of our experimental and theoretical work suggests that the maximum T c is likely associated with the predicted Fermi surface topological transition and that at this maximum T c , Sr 2 RuO 4 might have an even-parity rather than an odd-parity superconducting order parameter. The anisotropic distortion is key to these results: Hydrostatic pressure is known experimentally to decrease T c of Sr 2 RuO 4 . CONCLUSION Our data raise the possibility of an odd-parity to even-parity transition of the superconducting state of Sr 2 RuO 4 as a function of lattice strain and fuel an ongoing debate about the symmetry of the superconducting state even in the unstrained material. We anticipate considerable theoretical activity to address these issues, and believe that the technique developed for these experiments will also have a broader significance to future study of quantum magnets, topological systems, and electronic liquid crystals as well as superconductors.
- Published
- 2017
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