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Numerical simulations of turbulent moist Rayleigh–Bénard convection driving CCN activation and droplet growth in the laboratory Pi chamber are discussed. Supersaturation fluctuations come from isobaric mixing of warm and humid air rising from the lower boundary with colder air featuring lower water vapor concentrations descending from the upper boundary. Lagrangian particle–based microphysics is used to represent the growth of haze CCN and cloud droplets with kinetic, solute, and surface tension effects included. Dry CCN spectra in the range between 2- and 200-nm radii from field observations are considered. Increasing the total CCN concentration from pristine to polluted conditions results in an increase in the droplet concentration and reduction in the mean droplet radius and spectral width. These are in agreement with Pi chamber observations and numerical simulations, as well as with numerous past studies of CCN cloud-base activation in natural clouds. The key result is that a relatively small fraction of the available CCN is activated in the Pi chamber fluctuating supersaturations, from about a half in the pristine case to only a 10th in the polluted case. The activation fraction as a function of the dry CCN radius is similar in all simulations, close to zero at the CCN small end, increasing to a maximum at CCN radius around 50 nm, and decreasing to close to zero at the large CCN end. This is explained as too small supersaturations to activate small CCN as in natural clouds and insufficient time to allow large CCN reaching the critical radius. Significance Statement: Impact of turbulence on the formation and growth of cloud droplets is an important cloud physics problem. Laboratory experiments in the Michigan Technological University cloud chamber provide key insights into this problem. Numerical simulations of cloud chamber processes discussed in this paper complement laboratory experiments by providing insights difficult or impossible to obtain in the laboratory. The study contrasts the formation and growth of cloud droplets in the laboratory cloud chamber with processes taking place in natural clouds. The differences documented in this paper pose questions concerning the impact of turbulence on the formation and growth of cloud droplets as a result of interactions of clouds with their environment. [ABSTRACT FROM AUTHOR]

Numerical weather prediction (NWP), when accessible, is a crucial input to short-term solar power forecasting. WRF-Solar, the first NWP model specifically designed for solar energy applications, has shown promising predictive capability. Nevertheless, few attempts have been made to investigate its performance under high aerosol loading, which attenuates incoming radiation significantly. The North China Plain is a polluted region due to industrialization, which constitutes a proper testbed for such investigation. In this paper, aerosol direct radiative effect (DRE) on three surface shortwave radiation components (i.e., global, beam, and diffuse) during five heavy pollution episodes is studied within the WRF-Solar framework. Results show that WRF-Solar overestimates instantaneous beam radiation up to 795.3 W m−2 when the aerosol DRE is not considered. Although such overestimation can be partially offset by an underestimation of the diffuse radiation of about 194.5 W m−2, the overestimation of the global radiation still reaches 160.2 W m−2. This undesirable bias can be reduced when WRF-Solar is powered by Copernicus Atmosphere Monitoring Service (CAMS) aerosol forecasts, which then translates to accuracy improvements in photovoltaic (PV) power forecasts. This work also compares the forecast performance of the CAMS-powered WRF-Solar with that of the European Centre for Medium-Range Weather Forecasts model. Under high aerosol loading conditions, the irradiance forecast accuracy generated by WRF-Solar increased by 53.2% and the PV power forecast accuracy increased by 6.8%. Significance Statement: Numerical weather prediction (NWP) is the "go-to" approach for achieving high-performance day-ahead solar power forecasting. Integrating time-varying aerosol forecasts into NWP models effectively captures aerosol direct radiation effects, thereby enhancing the accuracy of solar irradiance forecasts in heavily polluted regions. This work not only quantifies the aerosol effects on global, beam, and diffuse irradiance but also reveals the physical mechanisms of irradiance-to-power conversion by constructing a model chain. Using the North China Plain as a testbed, the performance of WRF-Solar on solar power forecasting on five severe pollution days is analyzed. This version of WRF-Solar can outperform the European Centre for Medium-Range Weather Forecasts model, confirming the need for generating high spatial–temporal NWP. [ABSTRACT FROM AUTHOR]

Atmospheric aerosols affect human health and influence atmospheric and biological processes. Dust can be transported long distances in the atmosphere, and the mechanisms that influence dust transport are not fully understood. To improve the database for numerical models that simulate dust transport, measurements are needed that cover both the vertical distribution of the dust and its size distribution. In addition to measurements with crewed aircraft, uncrewed aircraft systems (UASs) provide a particularly suitable platform for this purpose. In this paper, we present a payload for the small fixed-wing UAS of the type Multiple-Purpose Airborne Sensor Carrier 3 (MASC-3) for aerosol particle measurements that is based on the optical particle counter (OPC) OPC-N3 (Alphasense, United Kingdom), modified by the addition of a dryer and a passive aspiration system (OPC-Pod). Based on field tests with a reference instrument in Mannheim, Germany, wind tunnel tests, and a comparison measurement with the UAS-mounted aerosol particle measurement Universal Cloud and Aerosol Sounding System (UCASS) during a dust event over Cyprus, we show that the OPC-Pod can measure particle number concentrations in the range of 0.66–31 μm as well as particle size distributions. The agreement of the OPC-Pod with UCASS is good. Both instruments resolve a vertical profile of the Saharan dust event, with a prominent dust layer between 1500 and 2800 m MSL, with particle number concentrations up to 35 cm−3 for particles between 0.66 and 31 μm. [ABSTRACT FROM AUTHOR]

The climate system responds to changes in the amount of atmospheric greenhouse gases or aerosols through rapid processes, triggered within hours and days, and through slower processes, where the full response may only be seen after centuries. In this paper, we aim to elucidate the mechanisms operating on time scales of hours to years to better understand the response of key climate quantities such as energy fluxes, temperature, and precipitation after a sudden increase in either carbon dioxide (CO2), black carbon (BC), or sulfate (SO4) aerosols. The results are based on idealized simulations from six global climate models. We find that the effect of changing ocean temperatures kicks in after a couple of months. Rapid precipitation reductions start occurring instantly and are established after just a few days. For BC, they constitute most of the equilibrium response. For CO2 and SO4, the magnitude of the precipitation response gradually increases as surface warming/cooling evolves, and for CO2, the sign of the response changes from negative to positive after 2 years. Rapid cloud adjustments are typically established within the first 24 h, and while the magnitude of cloud feedbacks for CO2 and SO4 increases over time, the geographical pattern of the equilibrium cloud change is present already after the first year. While there are model differences, our work underscores the overall similarity of the major time-varying processes and responses simulated by current global models and hence the robustness of key features of simulated responses to historical and future anthropogenic forcing. Significance Statement: How does the climate system respond to a change in the amount of atmospheric greenhouse gases or aerosols? Some processes are rapid, responding within hours and days. Others are slow, and the full response to a forcing of the climate may only be seen after centuries. In this paper, we use six global climate models to investigate the time scales of climate responses to carbon dioxide, black carbon, and sulfate, focusing on key climate quantities, such as temperature, precipitation, and clouds. While there are ample model differences, our work underscores the overall similarity of the major time-varying processes and responses simulated by current global models and hence the robustness of key features of simulated responses to historical and future anthropogenic forcing. [ABSTRACT FROM AUTHOR]

Aerosol properties are fundamentally different near clouds than away from clouds. This paper reviews the current state of knowledge of aerosol properties in the near-low-cloud environment and quantitatively compares them with aerosols far from clouds, according to remote sensing observations. It interprets observations of aerosol properties from different sensors using satellite, aircraft, and ground-based observations. The correlation (and anticorrelation) between proximity to cloud and aerosol properties is discussed. Retrieval artifacts in the near-cloud environment are demonstrated and quantified for different sensor attributes and environmental conditions. Finally, the paper describes the possible corrections for near-cloud enhancement in remote sensing retrievals. This study is timely in view of science definition studies for NASA's Aerosol, Cloud, Convection and Precipitation (ACCP) mission, which will also seek to directly link aerosol properties to nearby clouds. [ABSTRACT FROM AUTHOR]

A bin (or spectral) model is developed to investigate the sensitivity of warm rain initiation to cloud condensation nuclei (CCN). It explicitly represents CCN with a formula whose parameters come from the Twomey relationship (or CCN measurements). By seamlessly integrating CCN activation and drop collection with thousands of bins, the model can replicate the effect of CCN on rain initiation, providing a benchmark to test the process parameterizations in rain initiation. The model is used to simulate two extreme cases with CCN parameters of maritime and continental clouds, respectively, where other actual cases usually lie between these two extreme cases. Its simulations show that rain can initiate within half an hour or less as observed in cumulus clouds. The fast rain initiation modeled is attributed mainly to a new process: the condensational conversion of cloud drops to raindrops via collision–coalescence initiators (or drops with radius between 28 and 100 μm). Since the new process is more important in rain initiation than the autoconversion of cloud drops to raindrops when large CCN exist, it is suggested that the process be parameterized into the weather and climate models to better represent CCN and subsequently remove the common bias of "too dense clouds." Significance Statement: The current weather and climate models represent aerosols via implicit parameterizations and have a bias of "too dense clouds." Their implicit parameterizations of aerosols usually overlook (or misrepresent) some cloud processes. In this paper and its preceding part (Zeng and Li 2020) we proposed a new framework to explicitly parameterize one subset of aerosols: cloud condensation nuclei (CCN). To embody an explicit parameterization of CCN, we still need quantitative information to connect CCN activation and rain initiation, which motivates this study. In the study we developed an accurate microphysical model to simulate the growth of small CCN to large raindrops, providing information on the sensitivity of rain initiation to CCN. We performed many sensitivity simulations and found the condensational conversion of cloud drops to raindrops via collision–coalescence initiators is a vital process in warm rain initiation. Since the process has been overlooked by all the weather and climate models, the study suggests that the process be introduced in the weather and climate models to properly represent the fast warm rain initiation observed and subsequently remove the bias of "too dense clouds." [ABSTRACT FROM AUTHOR]

The Arctic is warming at more than twice the rate of the global average. This warming is influenced by clouds, which modulate the solar and terrestrial radiative fluxes and, thus, determine the surface energy budget. However, the interactions among clouds, aerosols, and radiative fluxes in the Arctic are still poorly understood. To address these uncertainties, the Ny-Ålesund Aerosol Cloud Experiment (NASCENT) study was conducted from September 2019 to August 2020 in Ny-Ålesund, Svalbard. The campaign's primary goal was to elucidate the life cycle of aerosols in the Arctic and to determine how they modulate cloud properties throughout the year. In situ and remote sensing observations were taken on the ground at sea level, at a mountaintop station, and with a tethered balloon system. An overview of the meteorological and the main aerosol seasonality encountered during the NASCENT year is introduced, followed by a presentation of first scientific highlights. In particular, we present new findings on aerosol physicochemical and molecular properties. Further, the role of cloud droplet activation and ice crystal nucleation in the formation and persistence of mixed-phase clouds, and the occurrence of secondary ice processes, are discussed and compared to the representation of cloud processes within the regional Weather Research and Forecasting Model. The paper concludes with research questions that are to be addressed in upcoming NASCENT publications. [ABSTRACT FROM AUTHOR]

This paper examines the impact of cloud-base turbulence on activation of cloud condensation nuclei (CCN). Following our previous studies, we contrast activation within a nonturbulent adiabatic parcel and an adiabatic parcel filled with turbulence. The latter is simulated by applying a forced implicit large-eddy simulation within a triply periodic computational domain of 643 m3. We consider two monodisperse CCN. Small CCN have a dry radius of 0.01 μm and a corresponding activation (critical) radius and critical supersaturation of 0.6 μm and 1.3%, respectively. Large CCN have a dry radius of 0.2 μm and feature activation radius of 5.4 μm and critical supersaturation 0.15%. CCN are assumed in 200-cm−3 concentration in all cases. Mean cloud-base updraft velocities of 0.33, 1, and 3 m s−1 are considered. In the nonturbulent parcel, all CCN are activated and lead to a monodisperse droplet size distribution above the cloud base, with practically the same droplet size in all simulations. In contrast, turbulence can lead to activation of only a fraction of all CCN with a nonzero spectral width above the cloud base, of the order of 1 μm, especially in the case of small CCN and weak mean cloud-base ascent. We compare our results to studies of the turbulent single-size CCN activation in the Pi chamber. Sensitivity simulations that apply a smaller turbulence intensity, smaller computational domain, and modified initial conditions document the impact of specific modeling assumptions. The simulations call for a more realistic high-resolution modeling of turbulent cloud-base activation. [ABSTRACT FROM AUTHOR]

This paper presents an introduction to the Southern Hemisphere High Altitude Experiment on Particle Nucleation and Growth (SALTENA). This field campaign took place between December 2017 and June 2018 (wet to dry season) at Chacaltaya (CHC), a GAW (Global Atmosphere Watch) station located at 5,240 m MSL in the Bolivian Andes. Concurrent measurements were conducted at two additional sites in El Alto (4,000 m MSL) and La Paz (3,600 m MSL). The overall goal of the campaign was to identify the sources, understand the formation mechanisms and transport, and characterize the properties of aerosol at these stations. State-of-the-art instruments were brought to the station complementing the ongoing permanent GAW measurements, to allow a comprehensive description of the chemical species of anthropogenic and biogenic origin impacting the station and contributing to new particle formation. In this overview we first provide an assessment of the complex meteorology, airmass origin, and boundary layer–free troposphere interactions during the campaign using a 6-month high-resolution Weather Research and Forecasting (WRF) simulation coupled with Flexible Particle dispersion model (FLEXPART). We then show some of the research highlights from the campaign, including (i) chemical transformation processes of anthropogenic pollution while the air masses are transported to the CHC station from the metropolitan area of La Paz–El Alto, (ii) volcanic emissions as an important source of atmospheric sulfur compounds in the region, (iii) the characterization of the compounds involved in new particle formation, and (iv) the identification of long-range-transported compounds from the Pacific or the Amazon basin. We conclude the article with a presentation of future research foci. The SALTENA dataset highlights the importance of comprehensive observations in strategic high-altitude locations, especially the undersampled Southern Hemisphere. [ABSTRACT FROM AUTHOR]

A 30-yr time series (4 February 1990–4 February 2020) of aerosol optical depth (AOD) of the atmosphere, total precipitable water (TPW), and total column ozone has been conducted in central Texas using simple, highly stable instruments. All three parameters in this ongoing measurement series exhibited robust annual cycles. They also responded to many atmospheric events, including the historic volcanic eruption of Mount Pinatubo (1991), a record El Niño (1998), an unprecedented biomass smoke event (1998), and La Niña that caused the driest drought in recorded Texas history (2011). Reduced air pollution caused mean AOD to decline from 0.175 to 0.14. The AOD trend measured for 30 years by a light-emitting diode (LED) sun photometer, the first of its kind, parallels the trend from 20 years of measurements by a modified Microtops II. While TPW responded to El Niño–Southern Oscillation conditions, TPW exhibited no trend over the 30 years. The TPW data compare favorably with 4.5 years of simultaneous measurements by a nearby NOAA GPS (r2 = 0.78). The 30 years of ozone measurements compare favorably with those from a series of NASA ozone satellites (r2 = 0.78). In 2016, 194 comparisons of Microtops II and world standard ozone instrument Dobson 83 at the Mauna Loa Observatory agreed within 1.9% (r2 = 0.81). The paper concludes by observing that students and citizen scientists can collect scientifically useful atmospheric data with simple sun photometers that use one or more LEDs as spectrally selective photodiodes. [ABSTRACT FROM AUTHOR]

Clouds play an important role in Arctic amplification. This term represents the recently observed enhanced warming of the Arctic relative to the global increase of near-surface air temperature. However, there are still important knowledge gaps regarding the interplay between Arctic clouds and aerosol particles, and surface properties, as well as turbulent and radiative fluxes that inhibit accurate model simulations of clouds in the Arctic climate system. In an attempt to resolve this so-called Arctic cloud puzzle, two comprehensive and closely coordinated field studies were conducted: the Arctic Cloud Observations Using Airborne Measurements during Polar Day (ACLOUD) aircraft campaign and the Physical Feedbacks of Arctic Boundary Layer, Sea Ice, Cloud and Aerosol (PASCAL) ice breaker expedition. Both observational studies were performed in the framework of the German Arctic Amplification: Climate Relevant Atmospheric and Surface Processes, and Feedback Mechanisms (AC) project. They took place in the vicinity of Svalbard, Norway, in May and June 2017. ACLOUD and PASCAL explored four pieces of the Arctic cloud puzzle: cloud properties, aerosol impact on clouds, atmospheric radiation, and turbulent dynamical processes. The two instrumented Polar 5 and Polar 6 aircraft; the icebreaker Research Vessel (R/V) Polarstern; an ice floe camp including an instrumented tethered balloon; and the permanent ground-based measurement station at Ny-Ålesund, Svalbard, were employed to observe Arctic low- and mid-level mixed-phase clouds and to investigate related atmospheric and surface processes. The Polar 5 aircraft served as a remote sensing observatory examining the clouds from above by downward-looking sensors; the Polar 6 aircraft operated as a flying in situ measurement laboratory sampling inside and below the clouds. Most of the collocated Polar 5/6 flights were conducted either above the R/V Polarstern or over the Ny-Ålesund station, both of which monitored the clouds from below using similar but upward-looking remote sensing techniques as the Polar 5 aircraft. Several of the flights were carried out underneath collocated satellite tracks. The paper motivates the scientific objectives of the ACLOUD/PASCAL observations and describes the measured quantities, retrieved parameters, and the applied complementary instrumentation. Furthermore, it discusses selected measurement results and poses critical research questions to be answered in future papers analyzing the data from the two field campaigns. [ABSTRACT FROM AUTHOR]

Sea salt aerosol (SSA) plays a significant role in the atmosphere through aerosol direct and indirect effects, and in atmospheric chemistry as a source of tropospheric bromine. In situ measurements of coarse-mode SSA particles are limited because of their low concentration and relatively large sizes (dry radius rd > 0.5 μm). With this in mind, a new, low-cost, easily usable method for sampling coarse-mode SSA particles in the marine boundary layer was developed. An SSA particle sampler that uses an impaction method was designed and built using 3D printing and Arduino microcontrollers and sensors. It exposes polycarbonate slides to ambient airflow remotely on a kite-based platform to capture coarse-mode SSA particles. Because it is a smaller version of the Giant Nucleus Impactor (GNI), designed for use on aircraft, it is named the miniature Giant Nucleus Impactor (miniGNI). After sample collection, the same optical microscope methodology utilized by the GNI was used to analyze the wetted salt particles that impacted onto the slides. In this proof-of-concept study, multiple miniGNIs were attached serially to a kite string, allowing for sampling at multiple altitudes simultaneously. The robustness of the results from this new instrument and methodology for sampling at ambient RH (~75%) the SSA particle size distribution with rd > 3.3 μm are compared with a similar study. We find that the SSA particle number concentration decreases weakly with altitude and shows no correlation to instantaneous U10 wind speed along the windward coastline of Oʻahu in the Hawaiian Islands. Significance Statement: The goal of our work is to determine the size distribution of large (dry salt radius > 3.3 μm) sea salt aerosol (SSA) particles in the atmosphere. Understanding the number concentration and size distribution of SSA particles is important because they play a role in many atmospheric processes, affecting visibility, atmospheric chemistry, cloud properties, precipitation formation, etc. We designed, built, and tested a new low-cost instrument for sampling large SSA particles. In this paper we compare our results to a similar prior study to give insight into the observations made with the new instrument. We flew the instrument on a kite for sampling, but future work could explore using the instrument on other platforms, such as a drone or unmanned aircraft system (UAS). [ABSTRACT FROM AUTHOR]

This paper shows that joint temperature-precipitation information over a global domain provides a more accurate estimate of aerosol forced responses in climate models than does any other combination of temperature, precipitation, or sea level pressure. This fact is demonstrated using a new quantity called potential detectability, which measures the extent to which a forced response can be detected in a model. In particular, this measure can be evaluated independently of observations and therefore permits efficient exploration of a large number of variable combinations before performing optimal fingerprinting on observations. This paper also shows that the response to anthropogenic aerosol forcing can be separated from that of other forcings using only spatial structure alone, leaving the time variation of the response to be inferred from data, thereby demonstrating that temporal information is not necessary for detection. The spatial structure of the forced response is derived by maximizing the signal-to-noise ratio. For single variables, the north-south hemispheric gradient and equator-to-pole latitudinal gradient are important spatial structures for detecting anthropogenic aerosols in some models but not all. Sea level pressure is not an independent detection variable because it is derived partly from surface temperature. In no case does sea level pressure significantly enhance potential detectability beyond that already possible using surface temperature. Including seasonal or land-sea contrast information does not significantly enhance detectability of anthropogenic aerosol responses relative to annual means over global domains. [ABSTRACT FROM AUTHOR]

During late summer 2020, large wildfires over the Pacific Northwest produced dense smoke that impacted the region for an extended period. During this period of poor air quality, persistent low-level cloud coverage was poorly forecast by operational numerical weather prediction models, which dissipated clouds too quickly or produced insufficient cloud coverage extent. This deficiency raises questions about the influence of wildfire smoke on low-level clouds in the marine environment of the Pacific Northwest. This paper investigates the effects of wildfire smoke on the properties of low-level clouds, including their formation, microphysical properties, and dissipation. A case study from 12 to 14 September 2020 is used as a testbed to evaluate the impact of wildfire smoke on such clouds. Observations from satellites and surface observing sites, coupled with mesoscale model simulations, are applied to understand the influence of wildfire smoke during this event. Results indicate that the presence of thick smoke over Washington led to decreased temperatures in the lower troposphere, which enhanced low-level cloud coverage, with smoke particles altering the microphysical structure of clouds to favor high concentrations of small droplets. Thermodynamic changes due to smoke are found to be the primary driver of enhanced cloud lifetime during these events, with microphysical changes to clouds as a secondary contributing factor. However, both the thermodynamic and microphysical effects are necessary to produce a realistic simulation. [ABSTRACT FROM AUTHOR]

A practical method for instrumental calibration and aerosol optical properties retrieval based on coherent Doppler lidar (CDL) and sun photometer is presented in this paper. To verify its feasibility and accuracy, this method is applied into three field experiments in 2019 and 2020. In this method, multiwavelength (440, 670, 870, and 1020 nm) aerosol optical depth (AOD) from sun-photometer measurements are used to estimate AOD at 1550 nm and calibrate integrated CDL backscatter signal. Then it is validated by comparing the retrieved calibrated AOD at 1550 nm from CDL signal and that from sun-photometer measurements. Good agreement between them with the correlation of 0.96, the RMSE of 0.0085, and the mean relative error of 22% is found. From the comparison results of these three experiments, sun photometer is verified to be an effective reference instrument for the calibration of CDL return signal and the aerosol optical properties measurement with CDL is feasible. It is expected to promote the study on the aerosol flux and transport mechanism in the planetary boundary layer with the widely deployed CDLs. Significance Statement: A practical method to calibrate and retrieve the vertical profiles of aerosol optical properties with coherent Doppler lidar (CDL) is proposed. Besides the wind field measurement ability, the extended capability of CDL in observing the aerosol optical properties is developed. In this method, a collocated sun photometer is operated as the reference instrument to calibrate and validate the aerosol optical properties from CDL. Since sun photometers and CDLs are world-widely deployed, this method has significant practical value. Additionally, once a CDL is well calibrated, it is promising to mount it on various platforms for simultaneous observations of aerosol optical properties and wind fields. Consequently, the CDL has the potential to measure the aerosol fluxes and vertical transport within the planetary boundary layers. [ABSTRACT FROM AUTHOR]

C-FOG is a comprehensive bi-national project dealing with the formation, persistence, and dissipation (life cycle) of fog in coastal areas (coastal fog) controlled by land, marine, and atmospheric processes. Given its inherent complexity, coastal-fog literature has mainly focused on case studies, and there is a continuing need for research that integrates across processes (e.g., air--sea--land interactions, environmental flow, aerosol transport, and chemistry), dynamics (two-phase flow and turbulence), microphysics (nucleation, droplet characterization), and thermodynamics (heat transfer and phase changes) through field observations and modeling. Central to C-FOG was a field campaign in eastern Canada from 1 September to 8 October 2018, covering four land sites in Newfoundland and Nova Scotia and an adjacent coastal strip transected by the Research Vessel Hugh R. Sharp. An array of in situ, path-integrating, and remote sensing instruments gathered data across a swath of space--time scales relevant to fog life cycle. Satellite and reanalysis products, routine meteorological observations, numerical weather prediction model (WRF and COAMPS) outputs, large-eddy simulations, and phenomenological modeling underpin the interpretation of field observations in a multiscale and multiplatform framework that helps identify and remedy numerical model deficiencies. An overview of the C-FOG field campaign and some preliminary analysis/findings are presented in this paper. [ABSTRACT FROM AUTHOR]

Here we elaborate on the deficiencies associated with the theoretical arguments and model simulations in a paper by Grabowski and Morrison (2020, hereafter GM20) that argued convective invigoration by aerosols does not exist. We show that the invigoration can be supported by both accurate theoretical analysis and explicit physics modeling with prognostic supersaturation and aerosols. Negligible invigoration by aerosols via drop freezing in GM20 was explained by a complete compensation between the heating effect from the freezing of extra liquid water and the extra loading effect during droplet ascending. But the reality is that droplet ascending then freezing occur at different locations and time scales, producing complex nonlinear responses that depend on the duration and location of the forcing. Also, this argument neglects the effect of off-loading of precipitating ice particles, increases in condensation during ascending, and riming and deposition accompanying droplet freezing. Regarding the warm-phase invigoration, the quasi-steady assumption for supersaturation as adopted in GM20 makes condensation independent of droplet number and size, therefore an incorrect interpretation of warm-phase invigoration. We illustrate that the quasi-steady assumption is invalid for updrafts of deep convective clouds in clean conditions because of the high acceleration of vertical velocity and the fast depletion of droplets by raindrop formation and accretion. Any assumption imposed on supersaturation, such as quasi-steady approximation and saturation adjustment, leads to errors in the evaluation of aerosol effects on diffusional growth and related buoyancy. Furthermore, we demonstrate that the piggybacking approach they used cannot prove or disprove the convective invigoration. [ABSTRACT FROM AUTHOR]

We report on the Azores Stratocumulus Measurements of Radiation, Turbulence and Aerosols (ACORES) campaign, which took place around Graciosa and Pico Islands/Azores in July 2017. The main objective was to investigate the vertical distribution of aerosol particles, stratocumulus microphysical and radiative properties, and turbulence parameters in the eastern North Atlantic. The vertical exchange of mass, momentum, and energy between the free troposphere (FT) and the cloudy marine boundary layer (MBL) was explored over a range of scales from submeters to kilometers. To cover these spatial scales with appropriate measurements, helicopterborne observations with unprecedented high resolution were realized using the Airborne Cloud Turbulence Observation System (ACTOS) and Spectral Modular Airborne Radiation Measurement System--Helicopter-Borne Observations (SMART-HELIOS) instrumental payloads. The helicopterborne observations were combined with ground-based aerosol measurements collected at two continuously running field stations on Pico Mountain (2,225 m above sea level, in the FT), and at the Atmospheric Radiation Measurement (ARM) station on Graciosa (at sea level). First findings from the ACORES observations we are discussing in the paper are as follows: (i) we have observed a high variability of the turbulent cloud-top structure on horizontal scales below 100 m with local temperature gradients of up to 4 K over less than 1 m vertical distance, (ii) we have collected strictly collocated radiation measurements supporting the relevance of small-scale processes by revealing significant inhomogeneities in cloud-top brightness temperature to scales well below 100 m, and (iii) we have concluded that aerosol properties are completely different in the MBL and FT with often-complex stratification and frequently observed burst-like new particle formation. [ABSTRACT FROM AUTHOR]

Atmospheric rivers (AR) are narrow bands of strong horizontal transport of water vapor in the midlatitudes that can cause extreme precipitation, which contributes to beneficial water supply and sometimes flooding. The precipitation productivity of an AR is affected by microphysical processes, including the influence of aerosols. Earlier case studies have shown that some ARs over the North Pacific Ocean contain dust from Africa and Asia that can strongly influence precipitation by acting as ice nuclei. This paper explores how commonly dust and ARs occur together, or in close proximity. A ''dust score'' is introduced to characterize the dustiness of the environment associated with ARs by using satellite-based observations. This method is applied to days on which one or more ARs made landfall along the west coast of the United States between 2001 and 2018. The dust score is used to describe the seasonality and year-to-year variability of dustyenvironment ARs. Dusty ARs occur primarily in the early spring (March-April), and dust is preferentially found within the warm sector of AR-associated extratropical cyclones and is also enhanced in the cold sector. Year-to-year variability in dust score is dependent more on year-to-year variability in dust than on the frequency ofARdays. This year-to-year variability is also strongly related to correlations between the frequency of ARs and the dustiness of the northeastern Pacific, motivating additional investigation into potential dynamical association between dust and ARs. [ABSTRACT FROM AUTHOR]

To explore the various couplings across space and time and between ecosystems in a consistent manner, atmospheric modeling is moving away from the fractured limited-scale modeling strategy of the past toward a unification of the range of scales inherent in the Earth system. This paper describes the forward-looking Multi-Scale Infrastructure for Chemistry and Aerosols (MUSICA), which is intended to become the next-generation community infrastructure for research involving atmospheric chemistry and aerosols. MUSICA will be developed collaboratively by the National Center for Atmospheric Research (NCAR) and university and government researchers, with the goal of serving the international research and applications communities. The capability of unifying various spatiotemporal scales, coupling to other Earth system components, and process-level modularization will allow advances in both fundamental and applied research in atmospheric composition, air quality, and climate and is also envisioned to become a platform that addresses the needs of policy makers and stakeholders. [ABSTRACT FROM AUTHOR]

The Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), updates NASA's previous satellite-era (1980 onward) reanalysis system to include additional observations and improvements to the Goddard Earth Observing System, version 5 (GEOS-5), Earth system model. As a major step toward a full Integrated Earth Systems Analysis (IESA), in addition to meteorological observations, MERRA-2 now includes assimilation of aerosol optical depth (AOD) from various ground- and space-based remote sensing platforms. Here, in the first of a pair of studies, the MERRA-2 aerosol assimilation is documented, including a description of the prognostic model (GEOS-5 coupled to the GOCART aerosol module), aerosol emissions, and the quality control of ingested observations. Initial validation and evaluation of the analyzed AOD fields are provided using independent observations from ground, aircraft, and shipborne instruments. The positive impact of the AOD assimilation on simulated aerosols is demonstrated by comparing MERRA-2 aerosol fields to an identical control simulation that does not include AOD assimilation. After showing the AOD evaluation, this paper takes a first look at aerosol-climate interactions by examining the shortwave, clear-sky aerosol direct radiative effect. The companion paper (Part II) evaluates and validates available MERRA-2 aerosol properties not directly impacted by the AOD assimilation (e.g., aerosol vertical distribution and absorption). Importantly, while highlighting the skill of the MERRA-2 aerosol assimilation products, both studies point out caveats that must be considered when using this new reanalysis product for future studies of aerosols and their interactions with weather and climate. [ABSTRACT FROM AUTHOR]

This paper examines hydrological variability and its changes in two different versions of a coupled ocean–atmosphere general circulation model developed at the National Oceanic and Atmospheric Administration/Geophysical Fluid Dynamics Laboratory and forced with estimates of future increases of greenhouse gas and aerosol concentrations. This paper is the second part, documenting potential changes in variability as greenhouse gases increase. The variance changes are examined using an ensemble of 8 transient integrations for an older model version and 10 transient integrations for a newer model. Monthly and annual data are used to compute the mean and variance changes. Emphasis is placed on computing and analyzing the variance changes for the middle of the twenty-first century and compared with those found in the respective control integrations. The hydrologic cycle intensifies because of the increase of greenhouse gases. In general, precipitation variance increases in most places. This is the case virtually everywhere the mean precipitation rate increases and many places where the precipitation decreases. The precipitation rate variance decreases in the subtropics, where the mean precipitation rate also decreases. The increased precipitation rate and variance, in middle to higher latitudes during late fall, winter, and early spring leads to increased runoff and its variance during that period. On the other hand, the variance changes of soil moisture are more complicated, because soil moisture has both a lower and upper bound that tends to reduce its fluctuations. This is particularly true in middle to higher latitudes during winter and spring, when the soil moisture is close to its saturation value at many locations. Therefore, changes in its variance are limited. Soil moisture variance change is positive during the summer, when the mean soil moisture decreases and is close to the middle of its allowable range. In middle to high northern latitudes, an increase in runoff and its variance during late winter and spring plus the decrease in soil moisture and its variance during summer lend support to the hypothesis stated in other publications that a warmer climate can cause an increasing frequency of both excessive discharge and drier events, depending on season and latitude. [ABSTRACT FROM AUTHOR]

This paper presents a novel method based on the application of interpolation techniques to the multicomponent aerosol–cloud parameterization for global climate modeling. Quantifying the aerosol indirect effect still remains a difficult task, and thus developing parameterizations for general circulation models (GCMs) of the microphysics of clouds and their interactions with aerosols is a major challenge for climate modelers. Three aerosol species are considered in this paper—namely sulfate, sea salt, and biomass smoke—and a detailed microphysical chemical parcel model is used to obtain a dataset of points relating the cloud droplet number concentration (CDNC) to the three aerosol input masses. The resulting variation of CDNC with the aerosol mass has some nonlinear features that require a complex but efficient parameterization to be easily incorporated into GCMs. In bicomponent systems, simple interpolation techniques may be sufficient to relate the CDNC to the aerosol mass, but with increasing components, simple methods fail. The parameterization technique proposed in this study employs either the modified Shepard interpolation method or the Hardy multiquadrics interpolation method, and the numerical results obtained show that both methods provide realistic results for a wide range of aerosol mass loadings. This is the first application of these two interpolation techniques to aerosol–cloud interaction studies. [ABSTRACT FROM AUTHOR]

The North China Plain (NCP) is becoming one of the most polluted areas characterized by a high frequency of haze pollution. However, the spatial and temporal evolutions of aerosol chemical compositions in such a highly polluted region are not well understood due to the lack of a long-term and comprehensive observation-based network. China's National Aerosol Composition Monitoring Network (NACMON) has conducted comprehensive offline and online measurements of compositions and optical properties of airborne aerosols in order to systematically investigate the formation process, source apportionments of haze, and interactions between haze pollution and climate change. The objective of the observations is to provide information for policy makers to make strategies for the alleviation of haze occurrence. In this paper, we present instrumentations and methodologies as well as the preliminary results of the offline observations in NACMON stations over the NCP region. The implications and future perspectives of the network are also summarized. Benefiting from simultaneous observations from this network, we found that secondary aerosols were the dominant component in haze pollution. High anthropogenic emissions, low wind speed, and high relative humidity (RH) facilitated gas-to-particle transformation and resulted in high PM2.5 formation (PM2.5 is particulate matter that is smaller than 2.5 μm in diameter). Sulfate-dominant or nitrate-dominant aerosols during the haze period were driven by ambient RH. Moreover, the contributions of coal combustion and biomass burning to PM2.5 revealed downward trends, whereas secondary aerosols showed upward trends over the last decade. Thus, we highlighted that strict control of anthropogenic emissions of precursor gases, such as NOx, NH3, and volatile organic compounds (VOCs), will be an important way to decrease PM2.5 pollution in the NCP region. [ABSTRACT FROM AUTHOR]

To mark the publication of the special collection in honor of Robert (Bob) A. Duce in the Journal of the Atmospheric Sciences, we have summarized his most important contributions to the subject of biogeochemical coupling between the atmosphere and ocean. Here we have divided these contributions into four themes--deposition from the atmosphere and its effects on the oceans, volatile elements emitted from the oceans, sea surface biology and aerosol formation, and marine aerosols and clouds. It is our intent that this summary along with the papers in this special collection provide an overview of the enormous contributions that Bob Duce has made to the subject during his distinguished scientific career. [ABSTRACT FROM AUTHOR]

Hydrological sensitivity is the change in global-mean precipitation per degree of global-mean temperature change. This paper shows that the hydrological sensitivity of the response to anthropogenic aerosol forcing is distinct from that of the combined response to all other forcings and that this difference is sufficient to infer the associated cooling in global-mean temperature. This result is demonstrated using temperature and precipitation data generated by climate models and is robust across different climate models. Remarkably, greenhouse gas warming and aerosol cooling can be estimated in a model without using any spatial or temporal gradient information in the response, provided temperature data are augmented by precipitation data. Over the late twentieth century, the hydrological sensitivities of climate models differ significantly from that of observations. Whether this discrepancy can be attributed to observational error, which is substantial as different estimates of global-mean precipitation are not even significantly correlated with each other, or to model error is unclear. The results highlight the urgency to construct accurate estimates of global precipitation from past observations and for reducing model uncertainty in hydrological sensitivity. This paper also clarifies that previous estimates of hydrological sensitivity are limited in that standard regression methods neglect temperature-precipitation relations that occur through internal variability. An alternative method for estimating hydrological sensitivity that overcomes this limitation is presented. [ABSTRACT FROM AUTHOR]

During the Cloud System Evolution in the Trades (CSET) field study, 14 research flights of the National Science Foundation G-V sampled the stratocumulus–cumulus transition between Northern California and Hawaii and its synoptic variability. The G-V made vertically resolved measurements of turbulence, cloud microphysics, aerosol characteristics, and trace gases. It also carried dropsondes and a vertically pointing W-band radar and lidar. This paper summarizes these observations with the goals of fostering novel comparisons with theory, models and reanalyses, and satellite-derived products. A longitude–height binning and compositing strategy mitigates limitations of sparse sampling and spatiotemporal variability. Typically, a 1-km-deep decoupled stratocumulus-capped boundary layer near California evolved into 2-km-deep precipitating cumulus clusters surrounded by patches of thin stratus that dissipated toward Hawaii. Low cloud cover was correlated with estimated inversion strength more than with cloud droplet number, even though the thickest clouds were generally precipitating and ultraclean layers indicative of aerosol–cloud–precipitation interaction were common west of 140°W. Accumulation-mode aerosol concentration correlated well with collocated cloud droplet number concentration and was typically largest near the surface. Aitken mode aerosol concentration was typically larger in the free troposphere. Wildfire smoke produced spikes of aerosol and trace gases on some flights. CSET data are compared with space–time collocated output from MERRA-2 reanalysis and from the CAM6 climate model run with winds and temperature nudged toward this reanalysis. The reanalysis compares better with the observed relative humidity than does nudged CAM6. Both vertically diffuse the stratocumulus cloud layer versus observations. MERRA-2 slightly underestimates in situ carbon monoxide measurements and underestimates ozone depletion within the boundary layer. [ABSTRACT FROM AUTHOR]

Influence of pollution on dynamics of deep convection continues to be a controversial topic. Arguably, only carefully designed numerical simulations can clearly separate the impact of aerosols from the effects of meteorological factors that affect moist convection. This paper argues that such a separation is virtually impossible using observations because of the insufficient accuracy of atmospheric measurements and the fundamental nature of the interaction between deep convection and its environment. To support this conjecture, results from numerical simulations are presented that apply modeling methodology previously developed by the author. The simulations consider small modifications, difficult to detect in observations, of the initial sounding, surface fluxes, and large-scale forcing tendencies. All these represent variations of meteorological conditions that affect deep convective dynamics independently of aerosols. The setup follows the case of daytime convective development over land based on observations during the Large-Scale Biosphere–Atmosphere (LBA) field project in Amazonia. The simulated observable macroscopic changes of convection, such as the surface precipitation and upper-tropospheric cloudiness, are similar to or larger than those resulting from changes of cloud condensation nuclei from pristine to polluted conditions studied previously using the same modeling case. Observations from Phase III of the Global Atmospheric Research Program Atlantic Tropical Experiment (GATE) are also used to support the argument concerning the impact of the large-scale forcing. The simulations suggest that the aerosol impacts on dynamics of deep convection cannot be isolated from meteorological effects, at least for the daytime development of unorganized deep convection considered in this study. [ABSTRACT FROM AUTHOR]

This article discusses the impact of anthropogenic greenhouse gases and aerosols on the 2022 Central Andes spring drought. Climate models suggest that human activity has a weak contribution to the drought, with compensating effects between greenhouse gases and aerosols. The Central Andes region is vulnerable to hydroclimatic extremes, and this study aims to assess the anthropogenic contribution to the drought and provide information for climate change mitigation and adaptation strategies. The study finds that the observed drought frequency has been increasing since 2010, with aerosol forcing having a marginal contribution to droughts in 2022, while greenhouse gas forcing has likely decreased the probability of droughts. Further research is needed to understand the combined impact of aerosol and greenhouse gas forcing under different sea surface conditions. The document is a list of references that cover various topics related to climate change, drought, and precipitation in South America, particularly in the Andean region. These sources can be valuable for library patrons conducting research on these specific topics. [Extracted from the article]

A framework for an empirical parameterization (EP) of heterogeneous nucleation of ice crystals by multiple species of aerosol material in clouds was proposed in a 2008 paper by the authors. The present paper reports improvements to specification of a few of its empirical parameters. These include temperatures for onset of freezing, baseline surface areas of aerosol observed in field campaigns over Colorado, and new parameters for properties of black carbon, such as surface hydrophilicity and organic coatings. The EP's third group of ice nucleus (IN) aerosols is redefined as that of primary biological aerosol particles (PBAPs), replacing insoluble organic aerosols. A fourth group of IN is introduced-namely, soluble organic aerosols. The new EP predicts IN concentrations that agree well with aircraft data from selected traverses of shallow wave clouds observed in five flights (1, 3, 4, 6, and 12) of the 2007 Ice in Clouds Experiment-Layer Clouds (ICE-L). Selected traverses were confined to temperatures between about −25° and −29°C in layer cloud without homogeneously nucleated ice from aloft. Some of the wave clouds were affected by carbonaceous aerosols from biomass burning and by dust from dry lakebeds and elsewhere. The EP predicts a trend between number concentrations of heterogeneously nucleated ice crystals and apparent black carbon among the five wave clouds, observed by aircraft in ICE-L. It is predicted in terms of IN activity of black carbon. The EP's predictions are consistent with laboratory and field observations not used in its construction, for black carbon, dust, primary biological aerosols, and soluble organics. The EP's prediction of biological ice nucleation is validated using coincident field observations of PBAP IN and PBAPs in Colorado. [ABSTRACT FROM AUTHOR]

The instantaneous top-of-atmosphere (TOA) radiance-to-flux conversion for the broadband radiometer (BBR) on board the Earth Clouds, Aerosols, and Radiation Explorer (EarthCARE) was assessed in Part I of this paper, by developing theoretical angular distribution models (ADMs) specifically designed for the instrument viewing configuration. This paper validates the BBR ADMs by comparing derived flux estimates with flux retrievals obtained from the Clouds and the Earth's Radiant Energy System (CERES) Terra models. A CERES BBR-like database is employed in the assessment, which is an optimum dataset to validate the BBR algorithms and to determine the benefits of the multiangular conversion procedures in the BBR instrument. The validation of theoretical results with empirical data is essential to prepare the conversion algorithms prior to the launch of EarthCARE. This paper demonstrates that the application of a linear combination method is not recommended when outgoing radiances do not follow the response modeled in the radiative transfer calculations. An effective radiance averaged model outperforms all other developed models, in terms of the coefficient of variation of the root-mean-square error, in the validation study of the shortwave (SW) regime (clear sky 1.9%; cloudy 7.1%) while an effective radiance along-track model obtains the best comparisons for the long-wave (LW) regime (clear sky 1.4%; cloudy 1.5%). The evaluation of the multiangular models with scenes with high anisotropy shows that multiview flux conversion algorithms can statistically improve CERES ADM results when CERES flux discrepancies of a target are higher than 4 W m-2 in the LW domain and SW clear-sky scenes and higher than 20 W m-2 in scenes with cloudy conditions. [ABSTRACT FROM AUTHOR]

In this paper, accurate UV polarization measurements are performed on a volcanic ash cloud after long-range transport at Lyon, France (45.76°N, 4.83°E). The volcanic particles are released from the mid-April 2010 eruption of the Eyjafjallajökull Icelandic volcano (63.63°N, 19.62°W). The aerosol UV depolarization, which arises from nonspherical volcanic ash particles, serves as an independent means to discriminate ash from nonash particles in the volcanic cloud. This discrimination is only feasible if the intrinsic ash particle depolarization ration δash is accurately determined. In this paper, the δash value [δash == (40.5 ± 2.0)%%] is derived from literature laboratory measurements on a scattering matrix to ensure ash particle specificity. It is shown that traditional approaches, based on direct lidar depolarization ratio δ a measurements, are only valid very close to the source region, because δ a may be very different from δash, when nonash particles are present. For the first time, observed lidar depolarization ratios, in the range from a few percent to 40%%, are hence interpreted in comparison with δash taken as a reference. It is then shown how to use the sensitive and accurate UV polarization measurements to access to the size-averaged number concentration vertical profile of volcanic ash particles in the troposphere. Vertical profiles of the backscattering coefficient specific to volcanic ash particles, providing altitude-resolved ash particle number concentrations, are presented in the troposphere after optical scattering computation. This new methodology can be applied to other aerosols events and for other optical remote sensing experiments. [ABSTRACT FROM AUTHOR]

A full understanding of the causes of the severe drought seen in the Sahel in the latter part of the twentieth-century remains elusive some 25 yr after the height of the event. Previous studies have suggested that this drying trend may be explained by either decadal modes of natural variability or by human-driven emissions (primarily aerosols), but these studies lacked a sufficiently large number of models to attribute one cause over the other. In this paper, signatures of both aerosol and greenhouse gas changes on Sahel rainfall are illustrated. These idealized responses are used to interpret the results of historical Sahel rainfall changes from two very large ensembles of fully coupled climate models, which both sample uncertainties arising from internal variability and model formulation. The sizes of these ensembles enable the relative role of human-driven changes and natural variability on historic Sahel rainfall to be assessed. The paper demonstrates that historic aerosol changes are likely to explain most of the underlying 1940-80 drying signal and a notable proportion of the more pronounced 1950-80 drying. [ABSTRACT FROM AUTHOR]

The recently developed GFDL Atmospheric Model version 3 (AM3), an atmospheric general circulation model (GCM), incorporates a prognostic treatment of cloud drop number to simulate the aerosol indirect effect. Since cloud drop activation depends on cloud-scale vertical velocities, which are not reproduced in present-day GCMs, additional assumptions on the subgrid variability are required to implement a local activation parameterization into a GCM. This paper describes the subgrid activation assumptions in AM3 and explores sensitivities by constructing alternate configurations. These alternate model configurations exhibit only small differences in their present-day climatology. However, the total anthropogenic radiative flux perturbation (RFP) between present-day and preindustrial conditions varies by ±±50%% from the reference, because of a large difference in the magnitude of the aerosol indirect effect. The spread in RFP does not originate directly from the subgrid assumptions but indirectly through the cloud retuning necessary to maintain a realistic radiation balance. In particular, the paper shows a linear correlation between the choice of autoconversion threshold radius and the RFP. Climate sensitivity changes only minimally between the reference and alternate configurations. If implemented in a fully coupled model, these alternate configurations would therefore likely produce substantially different warming from preindustrial to present day. [ABSTRACT FROM AUTHOR]

The four-parameter modified gamma distribution (MGD) is the most general mathematically convenient model for size distributions of particle types ranging from aerosols and cloud droplets or ice particles to liquid and frozen precipitation. The common three-parameter gamma distribution, the exponential distribution (e.g., Marshall--Palmer), and power-law distribution (e.g., Junge) are all special cases. Depending on the context, the particle ''size'' used in a given formulation may be the actual geometric diameter, the volume- or area-equivalent spherical diameter, the actual or equivalent radius, the projected or surface area, or the mass. For microphysical and radiative transfer calculations, it is often necessary to convert from one size representation to another, especially when comparing or utilizing distribution parameters obtained from a variety of sources. Furthermore, when the mass scales with Db, with b < 3, as is typical for snow and ice and other particles having a quasi-fractal structure, an exponential or gamma distribution expressed in terms of one size parameter becomes an MGD when expressed in terms of another. The MGD model is therefore more fundamentally relevant to size distributions of nonspherical particles than is often appreciated. The central purpose of this paper is to serve as a concise single-source reference for the mathematical properties of, and conversions between, atmospheric particle size distributions that can expressed as MGDs, including exponential and gamma distributions as special cases. For illustrative purposes, snow particle size distributions published by Sekhon and Srivastava, Braham, and Field et al. are converted to a common representation and directly compared for identical snow water content, allowing large differences in their properties to be discerned and quantified in a way that is not as easily achieved without such conversion. [ABSTRACT FROM AUTHOR]

Breaking waves play an important role in air--sea interaction, enhancing momentum flux from the atmosphere to the ocean, dissipating wave energy that is then available for turbulent mixing, injecting aerosols and sea spray into the atmosphere, and affecting air--sea gas transfer due to air entrainment. In this paper observations are presented of the occurrence of breaking waves under conditions of strong winds (10--25 m s−−1) and fetch-limited seas (0--500 km) in the Gulf of Tehuantepec Experiment (GOTEX) in 2004. An airborne nadir-looking video camera, along with a global positioning system (GPS) and inertial motion unit (IMU), provided digital videos of the breaking sea surface and position in an earth frame. In particular, the authors present observations of ΛΛ( c), which is the distribution of breaking wave crest lengths per unit sea surface area, per unit increment in velocity c or scalar speed c, first introduced by O. M. Phillips. In another paper, the authors discuss the effect of processing methodology on the resulting shape of the ΛΛ( c) distribution. In this paper, the elemental method of measuring breaking crests is used to investigate the ΛΛ( c) distributions under a variety of wind and wave conditions. The integral and the first two moments of the ΛΛ( c) distributions are highly correlated with the active breaking rate and the active whitecap coverage. The computation of whitecap coverage yields a larger observational dataset from which the variability of whitecap coverage with wind speed, friction velocity, wave age, and wave slope is presented and compared to previous observations. The dependence of the active breaking rate on the spectral peak steepness is in agreement with previous studies. Dimensional analysis of ΛΛ( c) indicates that scaling with friction velocity and gravity, as in the classical fetch relations, collapses the breaking distributions more effectively than scaling with dominant wave parameters. Significant wave breaking is observed at speeds near the spectral peak in young seas only, consistent with previous studies. The fourth and fifth moments of ΛΛ( c) are related to the flux of momentum transferred by breaking waves to the underlying water and the rate of wave energy dissipation, respectively. The maximum in the fourth moment occurs at breaking speeds of 5--5.5 m s−−1, and the maximum in the fifth moment occurs at 5.8--6.8 m s−−1, apparently independent of wave age. However, when nondimensionalized by the phase speed at the peak of the local wave spectrum cp, the maxima in the nondimensionalized fourth and fifth moments show a decreasing trend with wave age, obtaining the maxima at dimensionless speeds c/ cp near unity at smaller wave ages and moving to lower dimensionless speeds c/ cp ≪≪ 1 at larger wave ages. The angular dependence of ΛΛ( c) is predominantly unimodal and better aligned with the wind direction than the dominant wave direction. However, the directional distribution of ΛΛ( c) is broadest for small c and often exhibits a bimodal structure for slow breaking speeds under developing seas. An asymmetry in the directional distribution is also observed for moderately developed seas. Observations are compared to the Phillips model for ΛΛ( c) in the equilibrium range of the wave spectrum. Although the ensemble of ΛΛ( c) distributions appears consistent with a c−−6 function, the distributions are not described by a constant power-law exponent. However, the ΛΛ( c) observations are described well by the Rayleigh distribution for slow and intermediate speeds, yet fall above the Rayleigh distribution for the fastest breaking speeds. From the Rayleigh description, it is found that the dimensionless width of the ΛΛ( c) distribution increases weakly with dimensionless fetch, s/ u** e == 1.69 χχ0.06, where s is the Rayleigh parameter, u** e is the effective friction velocity, and the dimensionless fetch is a function of the fetch X and gravitational acceleration g. The nondimensionalized total length of breaking per unit sea surface area is found to decrease with dimensionless fetch for intermediate to fully developed seas, , where A is the total length of breaking crests per unit sea surface area. [ABSTRACT FROM AUTHOR]

The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) is a two-wavelength polarization lidar that performs global profiling of aerosols and clouds in the troposphere and lower stratosphere. CALIOP is the primary instrument on the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite, which has flown in formation with the NASA A-train constellation of satellites since May 2006. The global, multiyear dataset obtained from CALIOP provides a new view of the earth’s atmosphere and will lead to an improved understanding of the role of aerosols and clouds in the climate system. A suite of algorithms has been developed to identify aerosol and cloud layers and to retrieve a variety of optical and microphysical properties. CALIOP represents a significant advance over previous space lidars, and the algorithms that have been developed have many innovative aspects to take advantage of its capabilities. This paper provides a brief overview of the CALIPSO mission, the CALIOP instrument and data products, and an overview of the algorithms used to produce these data products. [ABSTRACT FROM AUTHOR]

This is the second of two companion papers on modeling of mesoscale cellular structures and drizzle in marine stratocumulus. In the first, aerosol–cloud–precipitation interactions and dynamical feedbacks were investigated to study the formation and evolution of open and closed cellular structures separately. In this paper, coexisting open and closed cells and how they influence one another are examined in a model domain of 180 × 60 × 1.5 km3. Simulations show that gradients in aerosol at the open–closed-cell boundary cause gradients in precipitation that generate a mesoscale circulation. The circulation promotes precipitation in the polluted closed cells but suppresses it in open cells by transporting water vapor to the closed-cell regime and carrying drier air and aerosol back to the open cells. The strength of this circulation depends on the contrast in precipitation under clean and polluted conditions at the boundary. Ship plumes emitted into clean, precipitating regions, simulated as a special case of a clean–polluted boundary, develop a similar circulation. Drizzle in the ship track is first suppressed by the increase in aerosol particles but later recovers and becomes even stronger because the local circulation enhances liquid water path owing to the convergence of water vapor from the region adjacent to the track. This circulation modifies the transport and mixing of ship plumes and enhances their dispersal. Finally, results show that whereas ship emissions do increase cloud albedo in regions of open cells, even the addition of very large aerosol concentrations cannot transform an open cellular structure to a closed one, for the case considered. [ABSTRACT FROM AUTHOR]

This study explores how the Atlanta, Georgia (United States), urban region influences warm-season (May through September) cloud-to-ground lightning flashes and precipitation. Eight years (1995–2003) of flashes from the National Lightning Detection Network and mean accumulated precipitation from the North American Regional Reanalysis model were mapped under seven different wind speed and direction combinations derived from cluster analysis. Overlays of these data affirmed a consistent coupling of lightning and precipitation enhancement around Atlanta. Maxima in precipitation and lightning shifted in response to changes in wind direction. Differences in the patterns of flash metrics (flash counts versus thunderstorm counts), the absence of any strong urban signal in the flashes of individual thunderstorms, and the scales over which flashes and precipitation enhancement developed are discussed in light of their support for land-cover- and aerosol-based mechanisms of urban weather modification. This study verifies Atlanta’s propensity to conjointly enhance cloud-to-ground lightning and precipitation production in the absence of strong synoptic forcing. However, because of variability in aerosol characteristics and the dynamics of land use change, it may be a simplification to assume that this observed enhancement will be persistent across all scales of analysis. [ABSTRACT FROM AUTHOR]

Demands for Monte Carlo radiative transfer modeling have grown with the increase in computational power in recent decades. This method provides realistic simulations of radiation processes for various types of application, including radiation budgets in cloudy conditions and remote measurements of clouds, aerosols, and gases. Despite many advantages, such as explicit treatment of three-dimensional radiative transfer, issues of numerical efficiency can make the method intractable, especially in radiance calculations. The commonly used local estimation method requires computationally intensive ray tracing at each collision. Furthermore, the realistic phase function of Mie scattering by cloud and aerosol particles has very sharp peaks in the forward direction. Radiance computations by Monte Carlo methods are inefficient for such spiky phase functions because of significant noise. Moreover, in optically thin regions, sampling of radiance contributions is so rare that long computing times are required to reduce noise. To solve these issues, several variance reduction methods have been proposed. This paper discusses a modified local estimation method, a truncation approximation for a highly anisotropic phase function, a collision-forcing method for optically thin media, a numerical diffusion technique, and several related topics. Numerical experiments demonstrated significant improvements in efficiency for solar radiance calculations in a limited number of cloudy cases. [ABSTRACT FROM AUTHOR]

There are two important problems in the aerosol optical depth (AOD) retrievals from hourly/daily/monthly accumulated pyrheliometer data, that is, how to select a suitable cosine of the solar zenith angle (μ[sub 0] ) and how to eliminate or minimize cloud effects. In this paper, two models of &ldquo=uivalent” μ[sub 0] are developed for two cases of hourly and daily pyrheliometer data. As shown in retrieval simulations, relative standard errors of 0.75-μm-wavelength AOD solutions caused by the model uncertainties are, respectively, 0.77% and 1.93% in the two cases. Then, an approach is proposed to select AOD data from the total optical depths retrieved from hourly/daily pyrheliometer data probably containing cloud contribution. The approach uses additional cloud fraction, surface visibility, and relative humidity data to constrain the AOD upper limit and then to minimize the cloud effect on the monthly/yearly mean AOD estimations. The limit decreases with an increase of cloud fraction. Furthermore, in the case of the AOD retrieval using joint data of total monthly direct solar radiation and sunshine duration, two error factors, that is, the optically thin (solar transparent) cirrus cloud effect and the difference between radiation limits of pyrheliometer and sunshine recorder, are analyzed and an improved inversion method is proposed. The AOD selection approach is tested in two kinds of practical AOD retrieval comparisons. Eleven representative meteorological observatories are selected in the first kind of comparisons of AODs from hourly/daily/monthly pyrheliometer data during 1993–2000. It is found that the AOD selection approach is available to minimize the cloud effect for stable and reasonable monthly/yearly mean AOD estimations. In the case of hourly pyrheliometer data for 1995, the maximum relative deviation between yearly mean AODs, retrieved by using different cloud fraction limits from 0.0 to 60%, is less than 7.9% for all 11 sites. Another kind of comparison between AODs from sun photometer and pyrheliometer data also shows the effectiveness of the AOD selection approach to minimize the cloud effect. [ABSTRACT FROM AUTHOR]

In determining the optical properties of the atmosphere, the measurement of light absorption by aerosols is particularly challenging, and yet it is important because of the influence of strongly absorbing black carbon on climate and atmospheric visibility. The photoacoustic method obtains aerosol light absorption in situ, without use of filters, by acoustic measurement of the heat generated from aerosol light absorption, and its transfer to the surrounding air. However, in the general case, volatile aerosols heated by light absorption may also cool by evaporation (mass transfer). In this paper, the limiting case of the photoacoustic response of a volatile aerosol is compared with that of a dry aerosol to further the understanding of the data obtained with photoacoustic instruments. While the theory of photoacoustics of volatile aerosols for low-frequency, nonresonant cells has already been developed, current methods employ high-frequency, acoustically resonant photoacoustic instruments for quantifying atmospheric aerosol light absorption and vehicle exhaust mass concentration associated with black carbon. In this paper, a complete theory of photoacoustics for volatile aerosols is developed that includes additional terms to allow for higher-frequency devices, large particles, and high particle densities. Numerical calculations are used to determine the limits of various approximations. [ABSTRACT FROM AUTHOR]

The Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), is NASA's latest reanalysis for the satellite era (1980 onward) using the Goddard Earth Observing System, version 5 (GEOS-5), Earth system model. MERRA-2 provides several improvements over its predecessor (MERRA-1), including aerosol assimilation for the entire period. MERRA-2 assimilates bias-corrected aerosol optical depth (AOD) from the Moderate Resolution Imaging Spectroradiometer and the Advanced Very High Resolution Radiometer instruments. Additionally, MERRA-2 assimilates (non bias corrected) AOD from the Multiangle Imaging SpectroRadiometer over bright surfaces and AOD from Aerosol Robotic Network sunphotometer stations. This paper, the second of a pair, summarizes the efforts to assess the quality of the MERRA-2 aerosol products. First, MERRA-2 aerosols are evaluated using independent observations. It is shown that the MERRA-2 absorption aerosol optical depth (AAOD) and ultraviolet aerosol index (AI) compare well with Ozone Monitoring Instrument observations. Next, aerosol vertical structure and surface fine particulate matter (PM2.5) are evaluated using available satellite, aircraft, and ground-based observations. While MERRA-2 generally compares well to these observations, the assimilation cannot correct for all deficiencies in the model (e.g., missing emissions). Such deficiencies can explain many of the biases with observations. Finally, a focus is placed on several major aerosol events to illustrate successes and weaknesses of the AOD assimilation: the Mount Pinatubo eruption, a Saharan dust transport episode, the California Rim Fire, and an extreme pollution event over China. The article concludes with a summary that points to best practices for using the MERRA-2 aerosol reanalysis in future studies. [ABSTRACT FROM AUTHOR]

Kretzschmar et al., in a comment in 2017, use the spread in the output of aerosol-climate models to argue that the models refute the hypothesis (presented in a paper by Stevens in 2015) that for the mid-twentieth-century warming to be consistent with observations, then the present-day aerosol forcing, must be less negative than −1 W m−2. The main point of contention is the nature of the relationship between global SO2 emissions and In contrast to the concave (log-linear) relationship used by Stevens and in earlier studies, whereby becomes progressively less sensitive to SO2 emissions, some models suggest a convex relationship, which would imply a less negative lower bound. The model that best exemplifies this difference, and that is most clearly in conflict with the hypothesis of Stevens, does so because of an implausible aerosol response to the initial rise in anthropogenic aerosol precursor emissions in East and South Asia-already in 1975 this model's clear-sky reflectance from anthropogenic aerosol over the North Pacific exceeds present-day estimates of the clear-sky reflectance by the total aerosol. The authors perform experiments using a new (observationally constrained) climatology of anthropogenic aerosols to further show that the effects of changing patterns of aerosol and aerosol precursor emissions during the late twentieth century have, for the same global emissions, relatively little effect on These findings suggest that the behavior Kretzschmar et al. identify as being in conflict with the lower bound in Stevens arises from an implausible relationship between SO2 emissions and and thus provides little basis for revising this lower bound. [ABSTRACT FROM AUTHOR]

The Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), is the latest atmospheric reanalysis of the modern satellite era produced by NASA's Global Modeling and Assimilation Office (GMAO). MERRA-2 assimilates observation types not available to its predecessor, MERRA, and includes updates to the Goddard Earth Observing System (GEOS) model and analysis scheme so as to provide a viable ongoing climate analysis beyond MERRA's terminus. While addressing known limitations of MERRA, MERRA-2 is also intended to be a development milestone for a future integrated Earth system analysis (IESA) currently under development at GMAO. This paper provides an overview of the MERRA-2 system and various performance metrics. Among the advances in MERRA-2 relevant to IESA are the assimilation of aerosol observations, several improvements to the representation of the stratosphere including ozone, and improved representations of cryospheric processes. Other improvements in the quality of MERRA-2 compared with MERRA include the reduction of some spurious trends and jumps related to changes in the observing system and reduced biases and imbalances in aspects of the water cycle. Remaining deficiencies are also identified. Production of MERRA-2 began in June 2014 in four processing streams and converged to a single near-real-time stream in mid-2015. MERRA-2 products are accessible online through the NASA Goddard Earth Sciences Data Information Services Center (GES DISC). [ABSTRACT FROM AUTHOR]

The rising emissions of reactive nitrogen (Nr) from transport, industrial, and agricultural sectors in India have resulted in its consequent interactions with the removal mechanism of the atmospheric dust. This study, therefore, reports the fluxes of reactive nitrogen along with other inorganic species through dustfall over six sites of Delhi-National Capital Region (NCR) characterized by the changing dynamics of its different land-use pattern. The highest Nr fluxes were observed at site SMA Industrial estate (SMA; NO3− = 16.45 ± 10.17 mg m−2 day−1, NH4+ = 16.33 ± 16.00 mg m−2 day−1) and lowest at site Chuchchakwas village (CV; NO3− = 1.24 ± 0.16 mg m−2 day−1, NH4+ = 0 mg m−2 day−1). Sites Mukherjee Nagar (MN), Peeragarhi Chowk (PC), Jawaharlal Nehru University (JNU), and Noida Phase II (N-II), on the other hand, showed 3.59 ± 1.00, 3.39 ± 0.61, 2.98 ± 0.84, and 3.36 ± 0.78 mg m−2 day−1 of NO3− fluxes and 0.30 ± 0.06, 0.22 ± 0.04, 0.21 ± 0.04, and 0.22 ± 0.05 mg m−2 day−1 of NH4+ fluxes, respectively. The fraction of the total ions in the water soluble extract of the dustfall was also noticed to be the highest at the SMA site (22.2%) and lowest at the CV site (1.5%) with MN, PC, JNU, and N-II showing 3.5%, 3.7%, 2.9%, and 3.9% of their respective contributions. Relative abundances of Ca2+ and SO42− in the dustfall substantiated the stoichiometric reactions involved in Nr scavenging. The role of Ca2+ in the spatiotemporal variability of Nr fluxes was established with the help of neutralization ratios and regression plots. Morphological and particle size analysis further confirmed the anthropogenic-induced crustal interferences in the summertime dustfall fluxes of Nr species. [ABSTRACT FROM AUTHOR]

The negative effects of relative humidity to measurements of particulate matter (PM) due to hygroscopic growth are often not inherently handled by low-cost optical particle counters (OPCs). This study presents a new approach in constructing a miniaturized diffusion dryer, for use with an OPC mounted on an uncrewed aircraft system (UAS), namely, the DJI S900 (weight of 7.5 kg and flight endurance of 20 min) for short-term measurements under humid conditions. In this work, an OPC of type N3 (Alphasense) was employed alongside the dryer, with experiments both in the laboratory and outdoors. Evaluation of the dryer's performance in a fog tank showed effective drying from almost saturated air to 41% relative humidity for 35 min, which is longer than the endurance of the UAS, and therefore sufficient. Changes in the flow rate through the OPC-N3 with the dryer showed a 17% reduction compared to an absent dryer, but the measured PM values remained unaffected. Airborne measurements were taken from four hovering flights near a governmental air pollution station (Mannheim-Nord, Germany) under humid conditions (88%–93%) where the system gave agreeable concentrations when the dryer was in place, but significantly overestimated all PM types without it. At a rural area near the Boundary Layer Field Site Falkenberg (Lindenberg, Germany), operated by the German Meteorological Service (DWD), vertical profiles inside a low-altitude cloud showed sharp increase in concentrations when the UAS entered the cloud layer, demonstrating its capability to accurately detect the layer base. [ABSTRACT FROM AUTHOR]

The long-range transport of bioaerosols by dust events significantly impacts ecological and meteorological networks of the atmosphere, biosphere, and anthroposphere. Bioaerosols not only cause significant public health risks, but also act as efficient ice nuclei for inducing cloud formation and precipitation in the hydrological cycle. To establish risk management for bioaerosol impacts on the Earth system, a large-scale investigation of bioaerosols must be performed under different environmental conditions. For this purpose, a Dust–Bioaerosol (DuBi) field campaign was conducted to investigate the distribution of bioaerosols by collecting ∼950 samples at 39 sites across East Asia from 2016 to 2021. Concentrations and community structures of bioaerosols were further analyzed using fluorescence microscopic observations and high-throughput DNA sequencing, and these factors were compared to environmental factors, such as PM10 and aridity. The results indicated that microbial concentrations at dryland sites were statistically higher than those at humid sites, while the microbe-to-total-particle ratio was statistically lower in drylands than in humid regions. Microbial cells per microgram of PM10 decreased when PM10 increased. The proportion of airborne particles at each site did not vary substantially with season. The richness and diversity of airborne bacteria were significantly higher in drylands than in semiarid regions, while the community structures were stable among all sampling sites. The DuBi field campaign improves our understanding of bioaerosol characteristic variations along the dust transport pathway in East Asia and the changes of bioaerosols under the trend of climate warming, supporting the efforts to reduce public health risks. SIGNIFICANCE STATEMENT: We first conducted large-scale Dust–Bioaerosol (DuBi) field observations in East Asia from 2016 to 2021. We used unified sampling and analysis methods to collect 950 samples at 39 sites and analyzed bioaerosols' concentration and community structure. This study aims to find the relationship between bioaerosols with atmospheric particles and aridity, which fills gaps in the field. These results improve our understanding of bioaerosols' impacts on ecological and meteorological networks of the atmosphere, biosphere, and anthroposphere. The comprehensive observations will promote prediction of bioaerosol change under the trend of climate warming, supporting the efforts to reduce global climate, ecological security, and public health risks in the future. [ABSTRACT FROM AUTHOR]

Volcanic super-eruptions have been theorized to cause severe global cooling, with the 74 kya Toba eruption purported to have driven humanity to near-extinction. However, this eruption left little physical evidence of its severity and models diverge greatly on the magnitude of post-eruption cooling. A key factor controlling the super-eruption climate response is the size of volcanic sulfate aerosol, a quantity that left no physical record and is poorly constrained by models. Here we show that this knowledge gap severely limits confidence in model-based estimates of super-volcanic cooling, and accounts for much of the disagreement among prior studies. By simulating super-eruptions over a range of aerosol sizes, we obtain global mean responses varying from extreme cooling all the way to the previously unexplored scenario of widespread warming. We also use an interactive aerosol model to evaluate the scaling between injected sulfur mass and aerosol size. Combining our model results with the available paleoclimate constraints applicable to large eruptions, we estimate that global volcanic cooling is unlikely to exceed 1.5°C no matter how massive the stratospheric injection. Super-eruptions, we conclude, may be incapable of altering global temperatures substantially more than the largest Common Era eruptions. This lack of exceptional cooling could explain why no single super-eruption event has resulted in firm evidence of widespread catastrophe for humans or ecosystems. Significance Statement: Whether volcanic super-eruptions pose a threat to humanity remains a subject of debate, with climate models disagreeing on the magnitude of global post-eruption cooling. We demonstrate that this disagreement primarily stems from a lack of constraint on the size of volcanic sulfate aerosol particles. By evaluating the range of aerosol size scenarios, we demonstrate that eruptions may be incapable of causing more than 1.5°C cooling no matter how much sulfur they inject into the stratosphere. This could explain why archaeological records provide no evidence of increased human mortality following the Toba super-eruption. Further, we raise the unexplored possibility that the largest super-eruptions could cause global-scale warming. [ABSTRACT FROM AUTHOR]

Stratospheric aerosols are greatly influenced by medium-to-large volcanic eruptions. Over the last few years, extreme wildfires have been identified as new sources of stratospheric particles, in the form of carbonaceous aerosols injected by pyrocumulonimbus (pyroCb) events in the upper troposphere and lower stratosphere, associated with significant impacts on climate and ozone chemistry. To assess the impact of wildfires and volcanic eruptions on stratospheric aerosol loadings in the Northern Hemisphere, the Rapid Balloon Experiments for Sudden Aerosol Injection in the Stratosphere (REAS) project has been initiated. REAS is an international initiative that aims to respond to sudden events impacting stratospheric aerosol composition. Seventeen balloons were launched from Reims, eastern France, between November 2021 and January 2022 to quantify the atmospheric content for both aerosols and trace/greenhouse gases from the ground up to stratospheric levels. The main measurements concerned trace gases (CO/CO2 as tracers of smoke) and aerosol together with ozone using instruments such as a gas collector, optical particle counters, backscatter sondes, an aerosol sampler, an aerosol impactor, and ozonesondes. The Groupe de Spectrométrie Moléculaire et Atmosphérique (GSMA) launch facility provided unique possibilities of combining multiple measurements in one flight thanks to medium flights (corresponding to a 6 kg payload). While no major event impacted the stratosphere during the campaign, we particularly discuss the influence of the aged volcanic plume from La Soufrière volcano (Saint Vincent island) and smoke particles from series of pyroCb events that took place in North America. The burden as well as the optical and microphysical properties of the observed aerosols are quantified from these in situ observations in association with various satellite data. [ABSTRACT FROM AUTHOR]