1. Field-induced quantum criticality in the Kitaev system α−RuCl3
- Author
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Konstantin Nenkov, Seung-Hwan Do, L. T. Corredor, Th. Doert, Stephan Schönecker, A. U. B. Wolter, Jens Hunger, Matthias Vojta, Lukas Janssen, K.-Y. Choi, Ralf Albrecht, and Bernd Büchner
- Subjects
Physics ,Condensed matter physics ,Specific heat ,Order (ring theory) ,Field (mathematics) ,02 engineering and technology ,021001 nanoscience & nanotechnology ,01 natural sciences ,Condensed Matter - Strongly Correlated Electrons ,Quantum critical point ,0103 physical sciences ,Antiferromagnetism ,Condensed Matter::Strongly Correlated Electrons ,Quantum spin liquid ,010306 general physics ,0210 nano-technology ,Quantum ,Excitation - Abstract
$\alpha$-RuCl$_3$ has attracted enormous attention since it has been proposed as a prime candidate to study fractionalized magnetic excitations akin to Kitaev's honeycomb-lattice spin liquid. We have performed a detailed specific-heat investigation at temperatures down to $0.4$ K in applied magnetic fields up to $9$ T for fields parallel to the $ab$ plane. We find a suppression of the zero-field antiferromagnetic order, together with an increase of the low-temperature specific heat, with increasing field up to $\mu_0H_c\approx 6.9$ T. Above $H_c$, the magnetic contribution to the low-temperature specific heat is strongly suppressed, implying the opening of a spin-excitation gap. Our data point toward a field-induced quantum critical point (QCP) at $H_c$; this is supported by universal scaling behavior near $H_c$. Remarkably, the data also reveal the existence of a small characteristic energy scale well below $1$~meV above which the excitation spectrum changes qualitatively. We relate the data to theoretical calculations based on a $J_1$--$K_1$--$\Gamma_1$--$J_3$ honeycomb model., Comment: 5 pages, 4 figures (main text), plus Supplemental Material
- Published
- 2017
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