1. Dynamical polarizability of graphene with spatial dispersion
- Author
-
Jian-Sheng Wang, Mauro Antezza, Tao Zhu, National University of Singapore (NUS), Laboratoire Charles Coulomb (L2C), Université de Montpellier (UM)-Centre National de la Recherche Scientifique (CNRS), Théorie du rayonnement matière et phénomènes quantiques, and Université de Montpellier (UM)-Centre National de la Recherche Scientifique (CNRS)-Université de Montpellier (UM)-Centre National de la Recherche Scientifique (CNRS)
- Subjects
[PHYS.COND.GAS]Physics [physics]/Condensed Matter [cond-mat]/Quantum Gases [cond-mat.quant-gas] ,Dirac (software) ,Ab initio ,FOS: Physical sciences ,02 engineering and technology ,7. Clean energy ,01 natural sciences ,law.invention ,[PHYS.QPHY]Physics [physics]/Quantum Physics [quant-ph] ,law ,Polarizability ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,0103 physical sciences ,Physics::Atomic and Molecular Clusters ,Physics::Chemical Physics ,010306 general physics ,Electronic band structure ,Wave function ,Physics ,[PHYS.PHYS.PHYS-OPTICS]Physics [physics]/Physics [physics]/Optics [physics.optics] ,Condensed Matter - Materials Science ,[PHYS.PHYS.PHYS-ATOM-PH]Physics [physics]/Physics [physics]/Atomic Physics [physics.atom-ph] ,Condensed Matter - Mesoscale and Nanoscale Physics ,Condensed matter physics ,Graphene ,Screening effect ,[PHYS.PHYS.PHYS-ATM-PH]Physics [physics]/Physics [physics]/Atomic and Molecular Clusters [physics.atm-clus] ,Materials Science (cond-mat.mtrl-sci) ,021001 nanoscience & nanotechnology ,0210 nano-technology ,Random phase approximation - Abstract
We perform a detailed analysis of electronic polarizability of graphene with different theoretical approaches. From Kubo's linear response formalism, we give a general expression of frequency and wave-vector dependent polarizability within the random phase approximation. Four theoretical approaches have been applied to the single-layer graphene and their differences are on the band-overlap of wavefunctions. By comparing with the \textit{ab initio} calculation, we discuss the validity of methods used in literature. Our results show that the tight-binding method is as good as the time-demanding \textit{ab initio} approach in calculating the polarizability of graphene. Moreover, due to the special Dirac-cone band structure of graphene, the Dirac model reproduces results of the tight-binding method for energy smaller than \SI{3}{\electronvolt}. For doped graphene, the intra-band transitions dominate at low energies and can be described by the Lindhard formula for two-dimensional electron gases. At zero temperature and long-wavelength limit, with the relaxation time approximation, all theoretical methods reduce to a long-wave analytical formula and the intra-band contributions agree to the Drude polarizability of graphene. Effects of electrical doping and temperature are also discussed. This work may provide a solid reference for researches and applications of the screening effect of graphene., 10 pages, 6 figures
- Published
- 2021
- Full Text
- View/download PDF