Search

In the lower/middle troposphere, {H2O,δD} pairs are good proxies for moisture pathways; however, their observation, in particular when using remote sensing techniques, is challenging. The project MUSICA (MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water) addresses this challenge by integrating the remote sensing with in situ measurement techniques. The aim is to retrieve calibrated tropospheric {H2O,δD} pairs from the middle infrared spectra measured from ground by FTIR (Fourier transform infrared) spectrometers of the NDACC (Network for the Detection of Atmospheric Composition Change) and the thermal nadir spectra measured by IASI (Infrared Atmospheric Sounding Interferometer) aboard the MetOp satellites. In this paper, we present the final MUSICA products, and discuss the characteristics and potential of the NDACC/FTIR and MetOp/IASI {H2O,δD} data pairs. First, we briefly resume the particularities of an {H2O,δD} pair retrieval. Second, we show that the remote sensing data of the final product version are absolutely calibrated with respect to H2O and δD in situ profile references measured in the subtropics, between 0 and 7 km. Third, we reveal that the {H2O,δD} pair distributions obtained from the different remote sensors are consistent and allow distinct lower/middle tropospheric moisture pathways to be identified in agreement with multi-year in situ references. Fourth, we document the possibilities of the NDACC/FTIR instruments for climatological studies (due to long-term monitoring) and of the MetOp/IASI sensors for observing diurnal signals on a quasi-global scale and with high horizontal resolution. Fifth, we discuss the risk of misinterpreting {H2O,δD} pair distributions due to incomplete processing of the remote sensing products. [ABSTRACT FROM AUTHOR]

In this work we present an analysis of aerosol microphysical properties during a mineral dust event taking advantage of the combination of different state-of-theart retrieval techniques applied to active and passive remote sensing measurements and the evaluation of some of those techniques using independent data acquired from in situ aircraft measurements. Data were collected in a field campaign performed during a mineral dust outbreak at the Granada, Spain, experimental site (37.16° N, 3.61°W, 680ma.s.l.) on 27 June 2011. Column-integrated properties are provided by sun- and star-photometry, which allows for a continuous reveal the presence of dust layers between 3 and 5 km a.s.l. with volume concentrations of the coarse spheroid mode up to 60 μm3 cm-3. The combined use of the regularization and LIRIC methods reveals the night-to-day evolution of the vertical structure of the mineral dust microphysical properties and offers complementary information to that from column-integrated variables retrieved from passive remote sensing. Additionally, lidar depolarization profiles and LIRIC retrieved volume concentration are compared with aircraft in situ measurements. This study presents for the first time a comparison of the total volume concentration retrieved with LIRIC with independent in situ measurements, obtaining agreement within the estimated uncertainties for both methods and quite good agreement for the vertical distribution of the aerosol layers. Regarding the depolarization, the first published data set of the CAS-POL for polarization ratios is presented here and qualitatively compared with the lidar technique. [ABSTRACT FROM AUTHOR]