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The Mars 2020 “Perseverance” rover’s SuperCam instrument suite [1,2,3] provides a wide variety of active and passive remote sensing techniques [4, 5, 6, 7] including passive visible & near-infrared (“VISIR”) spectroscopy [8]. Here we present our plans to use the VISIR technique for atmospheric science by observing solar radiation scattered by the Martian sky, similar to the “passive sky” technique demonstrated with ChemCam on the Mars Science Laboratory (MSL) rover [9]. Our presentation will focus on the objectives and techniques of SuperCam VISIR atmospheric science, but we will also present initial atmospheric science results or relevant instrument performance validation results to the extent that such are available at the time of the conference.The objectives of VISIR atmospheric science are O2, CO, and H2O vapor column abundances, and aerosol particle sizes and composition. These objectives are motivated by unexpected seasonal and interannual variability in the O2mixing ratio that is argued to be so large as to require O2 sources and sinks in surface soils [10], by evidence of surface-atmosphere exchange of H2O [11], by the potential significance of O2 and H2O volatiles as field context for returned samples due to their active exchanges with surface materials, and by the Mars 2020 mission [12] objectives of characterizing dust and validating global atmospheric models to prepare for human explorationThe SuperCam spectrometers used for VISIR mode are a ChemCam-heritage reflection spectrometer covering 385–465 nm with < 0.2 nm res. [2], an intensified transmission spectrometer covering 536–853 nm with 0.3–0.7 nm res. [2], and an acousto-optic-tunable-filter (AOTF) -based IR spectrometer covering 1300–2600 nm with 20–30 cm-1 res. [1, 8]. Our primary observing strategy is the same approach used for MSL ChemCam “passive sky” observations [9]: ratioing instrument signals from the two pointing positions with different elevation angles eliminates solar spectrum and instrument response uncertainties that are ~100x and ~10x larger than signals of interest for the transmission and AOTF IR spectrometers, respectively. We will also make use of single pointings directed at the white SuperCam calibration target for less-resource-intensive water vapor and aerosol monitoring, and of multiple-pointing lower-signal-to-noise sky scans to better constrain aerosol size and shape. Sky radiance is fit with a discrete ordinates multiple scattering radiative transfer model identical to that of [9]. As in [9] gas abundances are made robust to aerosol scattering uncertainties by fitting CO2 absorption bands with an aerosol vertical profile parameter.References: [1] Maurice S. et al. (2020) SSR, in press. [2] Wiens R.C. et al. (2021) SSR 217, 4. [3] Manrique J.-A. et al. (2020) SSR 216, 138. [4] Ollila A.M. et al. (2021), this meeting. [5] Ollila A.M. et al. (2018) LPSC 49, 2786. [6] Forni O. et al. (2021), this meeting. [7] Lanza N. L. et al. (2021), this meeting. [8] Johnson J.R et al. (2021), this meeting. [9] McConnochie T.H et al. (2018), Icarus 307, 294. [10] Trainer M.G. et al. (2019), JGR 124, 3000. [11] Savijärvi H. et al. (2016), Icarus 265, 63. [12] Farley K.A. et al. (2020), SSR 216, 142.

The SuperCam Instrument Suite [1-4], a US-French-Spanish-Danish collaboration, consists of three separate units: the Body Unit (BU) within the Rover [2], the Mast Unit (MU) at the top of the Perseverance Remote Sensing Mast [3], and Calibration Targets [4] located on the rover deck. SuperCam includes a passive visible/near-infrared (VISIR) spectroscopy system that will identify minerals near the rover (mm-scale) to distant outcrops (m-scale) over an extended wavelength range (0.385-0.465 µm, 0.536-0.853 µm, 1.3-2.6 µm) that is diagnostic for most mineral classes.The infrared spectrometer (IRS) in the MU [5] uses an acousto-optic tunable filter (AOTF) excited by a RF signal to successively diffract up to 256 different wavelengths ranging between 1.3 and 2.6 µm on one of two available photodiodes to produce a single spectrum in about 80 seconds at a spectral resolution of 5-20 nm. The field-of-view (FOV) of the IRS is 1.15 mrad and is co-aligned with the RMI boresight. The visible (VIS) system in the BU comprises three spectrometers covering the UV (245 – 340 nm), violet (385 – 465 nm), and visible and near-infrared (VNIR, 536–853 nm). The spectrometers are fed by light collected by the telescope in the MU through an optical fiber connecting the MU and BU. The violet spectrometer has a spectral resolution of 0.12 nm, and the VNIR transmission spectrometer has a spectral resolution of 0.35 – 0.70 nm. The VIS FOV is 0.74 mrad and co-aligned with the IR FOV.Several SuperCam calibration targets (SCCT) are dedicated to VISIR spectroscopy, including an AluWhite white target, an Aeroglaze Z307 black target, and red, cyan, and green color targets [4]. Several of the other targets whose primary purpose is for other techniques exhibit useful VISIR spectral features and will be observed [5].Raw data will be converted to radiance (W/m2/sr/µm) with calibrated wavelengths using the instrument transfer function [6-7]. Relative reflectance spectra will be generated by dividing the calibrated radiance spectrum by either (1) a Mars atmospheric transmission spectrum and then by a modeled solar irradiance spectrum; or (2) a radiance spectrum of the white SCCT taken close in time to the surface observation, as is done with Mastcam-Z calibration [8].This poster will show initial VISIR data acquired on Mars, compared with test and performance data obtained at Paris Observatory, LANL, and JPL. As of this writing, the planned observations during the first ~30 sols include spectra of the white and black SCCTs, and at least one Mars target spectrum.[1] Farley et al. (2020), Space Sci. Rev. 216, 142. [2] Wiens et al. (2020) Space Sci. Rev. 216, in press, [3] Maurice et al. (2020) Space Sci. Rev. 216,in press, [4] Manrique et al. (2020) Space Sci. Rev. 216, 8, 1-27; [5] Cousin et al. (2021) this meeting [6] Fouchet et al. (2021) Icarus, in prep. [7] Royer et al. (2020) Rev. Scient. Instrum. 91, 063105. [8] Bell, J.F. et al. (2021), Space Sci. Rev, in press.