1. 240 Pu/ 239 Pu signatures allow refining the chronology of radionuclide fallout in South America.
- Author
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Chaboche PA, Pointurier F, Sabatier P, Foucher A, Tiecher T, Minella JPG, Tassano M, Hubert A, Morera S, Guédron S, Ardois C, Boulet B, Cossonnet C, Cabral P, Cabrera M, Chalar G, and Evrard O
- Subjects
- Chile, Radioisotopes analysis, Soil, Plutonium analysis, Radiation Monitoring, Soil Pollutants, Radioactive analysis, Water Pollutants, Radioactive analysis
- Abstract
Atmospheric nuclear tests (1945-1980) have led to radioactive fallout across the globe. French tests in Polynesia (1966-1974) may influence the signature of fallout in South America in addition to those conducted by USA and former USSR until 1963 in the Northern hemisphere. Here, we compiled the
240 Pu/239 Pu atom ratios reported for soils of South America and conducted additional measurements to examine their latitudinal distributions across this continent. Significantly lower ratio values were found in the 20-45° latitudinal band (0.04 to 0.13) compared to the rest of the continent (up to 0.20) and attributed to the contribution of the French atmospheric tests to the ultra-trace plutonium levels found in these soils. Based on sediment cores collected in lakes of Chile and Uruguay, we show the added value of measuring240 Pu/239 Pu atom ratios to refine the age models of environmental archives in this region of the world., Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2022 Elsevier B.V. All rights reserved.)- Published
- 2022
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