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Based on the 18 realizations of three state-of-the-art climate models participated in the Coupled Model Intercomparison Project phase 6 (CMIP6), this paper examines the changes in climatology and trends of winter diurnal temperature range (DTR) over East Asia in response to natural and anthropogenic forcings. In the observation, the climatology of DTR during 1979–2014 displays a horizontal tile from southwest to northeast over East Asia. In addition, the observed DTR also presents an obviously declining trend in recent decades, with the magnitude of roughly −0.10 °C decade−1. The historical all-forcing simulations well reproduce the geographical distributions and magnitude of climatology and trends of winter DTR over East Asia in 1979–2014. Furthermore, the winter DTR exhibits a continuous declining trend from the historical scenario to the future SSP245 scenario over East Asia, with the most significant declining during the first half of twenty-first century (i.e., 2021–2060). Based on the individual forcing experiments, it suggests that the greenhouse gases forcing plays a primary role in driving the climatology and trends of DTR over East Asia, especially for the SSP245 scenario. Further analysis indicates that the increasing precipitation under greenhouse gases forcing largely explain the declining DTR trends over East Asia, especially over the northern East Asia both in historical and SSP245 scenarios. • The observed decreasing DTR trends are reasonably captured in the all-forcing historical simulations in CMIP6 models. • The greenhouse gas forcing plays a primary role in driving the declining DTR trends over East Asia • The declining of DTR is partly attributed to the increasing precipitation over East Asia in the greenhouse gas forcing. [ABSTRACT FROM AUTHOR]

An advanced modeling system with a “one-atmosphere” perspective, Models-3/Community Multi-scale Air Quality (CMAQ) modeling system, driven by MM5/NCEP reanalysis data as the meteorology, and GEOS-Chem outputs as boundary values was applied to simulate the O3, and other gaseous pollutants (SO2 and NO2) evolution among other atmospheric chemicals for July 2001. Comparisons had been made with other models in the MICS-II exercise for the same period. Statistics of both monthly and daily means show that the model skill is very good in reproducing O3 and SO2 with small to moderate RMSE. The model species capture the day-to-day and spatial variability of the observations. The same O3 model concentrations that overpredict most of the EANET observations in the MICS-II study may have underpredicted ones from monitoring networks in Beijing area that is not included in this paper. Vertical O3 profiles at 4 ozonesonde sites are well predicted in July 2001. In fact, our model is among the best of those MICS-II models within the 2-km surface layer. The meteorology near surface and lower troposphere is well reproduced. Compared to SO2 and O3, the NO2 gas concentrations are simulated less well, but the correlation coefficient is still significant. The choice of reanalysis meteorological fields and different boundary conditions generated by different global models may result in diverse spatial patterns exhibited by MICS-II models and ours. Our spatial distributions of O3 shows a high concentration patch covering Beijing, a moderate to high pattern across Korea and Japan Sea, and a low but extensive pattern enclosing southern China, Taiwan, and East Sea. Extension of the pattern to southern China coincides with the existence of pollution problems in Guangdong and Taiwan, but overprediction of O3 over the region deserves further improvement by various factors. One of them can be the grid resolution to resolve the complex orography in or close to the ocean. Another factor can be the refinement of local land use data that changes the micro-meteorology in favor of more air pollution events. [Copyright &y& Elsevier]

In the framework of the model intercomparison study—Asia Phase II (MICS2), where eight models are compared over East Asia, this paper studies the influence of different parameterizations used in the aerosol module on the aerosol concentrations of sulfate and nitrate in . An intracomparison of aerosol concentrations is done for March 2001 using different configurations of the aerosol module of one of the model used for the intercomparison. Single modifications of a reference setup for model configurations are performed and compared to a reference case. These modifications concern the size distribution, i.e. the number of sections, and physical processes, i.e. coagulation, condensation/evaporation, cloud chemistry, heterogeneous reactions and sea-salt emissions. Comparing monthly averaged concentrations at different stations, the importance of each parameterization is first assessed. It is found that sulfate concentrations are little sensitive to sea-salt emissions and to whether condensation is computed dynamically or by assuming thermodynamic equilibrium. Nitrate concentrations are little sensitive to cloud chemistry. However, a very high sensitivity to heterogeneous reactions is observed. Thereafter, the variability of the aerosol concentrations to the use of different chemistry transport models (CTMs) and the variability to the use of different parameterizations in the aerosol module are compared. For sulfate, the variability to the use of different parameterizations in the aerosol module is lower than the variability to the use of different CTMs. However, for nitrate, for monthly averaged concentrations averaged over four stations, these two variabilities have the same order of magnitude. [Copyright &y& Elsevier]