1. Mineral replacement rate of olivine by chrysotile and brucite under high alkaline conditions
- Author
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Rodica Chiriac, François Toche, Romain Lafay, German Montes-Hernandez, Nathaniel Findling, Emilie Janots, Institut des Sciences de la Terre (ISTerre), Université Joseph Fourier - Grenoble 1 (UJF)-Institut Français des Sciences et Technologies des Transports, de l'Aménagement et des Réseaux (IFSTTAR)-Institut national des sciences de l'Univers (INSU - CNRS)-Institut de recherche pour le développement [IRD] : UR219-PRES Université de Grenoble-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Centre National de la Recherche Scientifique (CNRS), Institut fûr Mineralogie, Westfälische Wilhelms-Universität Münster = University of Münster (WWU), Institute of Geological Sciences [Bern], University of Bern, Laboratoire des Multimatériaux et Interfaces (LMI), Université Claude Bernard Lyon 1 (UCBL), Université de Lyon-Université de Lyon-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS), Laboratoire de géologie de l'ENS (LGENS), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Département des Géosciences - ENS Paris, École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS-PSL), Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL), Centre National de la Recherche Scientifique (CNRS)-PRES Université de Grenoble-Université Joseph Fourier - Grenoble 1 (UJF)-Institut Français des Sciences et Technologies des Transports, de l'Aménagement et des Réseaux (IFSTTAR)-Institut national des sciences de l'Univers (INSU - CNRS)-Institut de recherche pour le développement [IRD] : UR219-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry]), Westfälische Wilhelms-Universität Münster (WWU), École normale supérieure - Paris (ENS Paris), and Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-École normale supérieure - Paris (ENS Paris)
- Subjects
Thermogravimetric analysis ,010504 meteorology & atmospheric sciences ,Mineralogy ,[SDU.STU]Sciences of the Universe [physics]/Earth Sciences ,engineering.material ,010502 geochemistry & geophysics ,01 natural sciences ,Inorganic Chemistry ,Chrysotile ,Materials Chemistry ,TG analyses ,Porosity ,Dissolution ,Alkaline medium ,0105 earth and related environmental sciences ,Chrysotile nanotubes ,Olivine ,Mineral ,Brucite ,Chemistry ,Serpentinization ,Mineral replacement rate ,Condensed Matter Physics ,Grain size ,Chemical engineering ,13. Climate action ,engineering ,[SDU.STU.MI]Sciences of the Universe [physics]/Earth Sciences/Mineralogy - Abstract
International audience; Olivine mineral replacement by serpentine is one major alteration reaction of oceanic hydrothermalism. In the present experimental study, olivine grains were replaced by chrysotile and brucite under high alkaline conditions. In our study, olivine replacement implied a spatial and temporal coupling of dissolution and precipitation reactions at the interface between olivine and chrysotile-brucite minerals. Coupled dissolution-precipitation led to the alteration of starting olivine grains (so-called primary or parent mineral) to a porous mineral assemblage of chrysotile and brucite with preservation of the initial olivine morphology. This mineral replacement reaction of olivine (serpentinization) has been characterized using XRD, FESEM and FTIR measurements. Moreover, a simple and novel method is here proposed to quantify the mineral replacement rate (or serpentinization rate) of olivine by using thermogravimetric (TG) and differential TG (DTG) analyses. Serpentinization extent depends on the grain size: it is complete after 30 days of reaction for the smallest olivine grains (
- Published
- 2012
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