1. Tropical sources and sinks of carbonyl sulfide observed from space
- Author
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Glatthor, N., Höpfner, M., Baker, I. T., Berry, J, Campbell, J. E., Kawa, S. R., Krysztofiak, G, Leyser, A., Sinnhuber, B.-M., Stiller, G. P., Stinecipher, J, Von Clarmann, T, Karlsruher Institut für Technologie (KIT), Department of Atmospheric Science [Fort Collins], Colorado State University [Fort Collins] (CSU), Department of Global Ecology [Carnegie] (DGE), Carnegie Institution for Science [Washington], Sierra Nevada Research Institute, University of California, NASA Goddard Space Flight Center (GSFC), Laboratoire de Physique et Chimie de l'Environnement et de l'Espace (LPC2E), Observatoire des Sciences de l'Univers en région Centre (OSUC), Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université d'Orléans (UO)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire de Paris, Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Université d'Orléans (UO)-Centre National de la Recherche Scientifique (CNRS)-Centre National d’Études Spatiales [Paris] (CNES), Environmental Systems Graduate Group, University of California [Merced], and University of California-University of California
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[SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere ,tropical sources and sinks of COS - Abstract
International audience; According to current budget estimations the seasonal variation of carbonyl sulfide (COS) is governed by oceanic release and vegetation uptake. Its assimilation by plants is assumed to be similar to the photosynthetic uptake of CO 2 but, contrary to the latter process, to be irreversible. Therefore, COS has been suggested as cotracer of the carbon cycle. Observations of COS, however, are sparse, especially in tropical regions. We use the comprehensive data set of spaceborne measurements of the Michelson Interferometer for Passive Atmospheric Sounding to analyze its global distribution. Two major features are observed in the tropical upper troposphere around 250 hPa: enhanced amounts over the western Pacific and the Maritime Continent, peaking around 550 parts per trillion by volume (pptv) in boreal summer, and a seasonally varying depletion of COS extending from tropical South America to Africa. The large-scale COS depletion, which in austral summer amounts up to −40 pptv as compared to the rest of the respective latitude band, has not been observed before and reveals the seasonality of COS uptake through tropical vegetation. The observations can only be reproduced by global models, when a large vegetation uptake and a corresponding increase in oceanic emissions as proposed in several recent publications are assumed.
- Published
- 2015
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