1. Collisions of ultracold molecules in bright and dark optical dipole traps
- Author
-
Arthur Christianen, Marcel Duda, Andreas Schindewolf, Xing-Yan Chen, Xin-Yu Luo, Tijs Karman, Roman Bause, Goulven Quéméner, Immanuel Bloch, Renhao Tao, Max-Planck-Institut für Quantenoptik (MPQ), Max-Planck-Gesellschaft, Munich Center for Quantum Science and Technology (MCQST), Laboratoire Aimé Cotton (LAC), Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Radboud University Nijmegen, Institute for Molecules and Materials, Radboud university [Nijmegen], Fakultat fur Physik, Ludwig-Maximilians-Universitat, and ANR-17-CE30-0015,FEW2MANY-SHIELD,Ecrantage collisionnel à petit et grand nombre de corps de molécules dipolaires ultrafroides(2017)
- Subjects
Physics ,[PHYS.COND.GAS]Physics [physics]/Condensed Matter [cond-mat]/Quantum Gases [cond-mat.quant-gas] ,[PHYS.PHYS.PHYS-ATOM-PH]Physics [physics]/Physics [physics]/Atomic Physics [physics.atom-ph] ,Atomic Physics (physics.atom-ph) ,Degrees of freedom (physics and chemistry) ,FOS: Physical sciences ,Trapping ,01 natural sciences ,Physics - Atomic Physics ,010305 fluids & plasmas ,3. Good health ,Photoexcitation ,Quantum technology ,Dipole ,Orders of magnitude (time) ,[PHYS.QPHY]Physics [physics]/Quantum Physics [quant-ph] ,Quantum Gases (cond-mat.quant-gas) ,0103 physical sciences ,Molecule ,Atomic physics ,Condensed Matter - Quantum Gases ,Theoretical Chemistry ,010306 general physics ,Order of magnitude - Abstract
Understanding collisions between ultracold molecules is crucial for making stable molecular quantum gases and harnessing their rich internal degrees of freedom for quantum engineering. Transient complexes can strongly influence collisional physics, but in the ultracold regime, key aspects of their behavior have remained unknown. To explain experimentally observed loss of ground-state molecules from optical dipole traps, it was recently proposed that molecular complexes can be lost due to photo-excitation. By trapping molecules in a repulsive box potential using laser light near a narrow molecular transition, we are able to test this hypothesis with light intensities three orders of magnitude lower than what is typical in red-detuned dipole traps. This allows us to investigate light-induced collisional loss in a gas of nonreactive fermionic $^{23}$Na$^{40}$K molecules. Even for the lowest intensities available in our experiment, our results are consistent with universal loss, meaning unit loss probability inside the short-range interaction potential. Our findings disagree by at least two orders of magnitude with latest theoretical predictions, showing that crucial aspects of molecular collisions are not yet understood, and provide a benchmark for the development of new theories., 13 pages, 11 figures
- Published
- 2021